{"title":"基于程序升温解吸技术的高选择性MEMS气体传感器。","authors":"Junming Shao,Renjun Si,Hongze Jiang,Shaofeng Chen,Jiabao Ding,Zheng Wang,Shunping Zhang","doi":"10.1021/acssensors.5c01413","DOIUrl":null,"url":null,"abstract":"Aiming at the issue of poor selectivity in metal oxide gas sensors, a novel MEMS gas sensor structure was designed, comprising an adsorption unit and a sensing unit. Based on this design, a gas-sensing method utilizing on-chip programmable temperature analysis technology was developed. By quantifying the gas-sensitive response, we successfully extracted the peak signal of temperature-dependent resistance with high selectivity. The performance results show that ZSM-5, as the adsorbent material, exhibits desorption peak positions at different temperatures for four types of alcohol gases, and the peak height is correlated with the adsorption concentration. The essence of its high selectivity lies in the fact that materials have different desorption activation energies for different gases under the same conditions. This study proposes a new selective MEMS device testing method for identifying gas types and concentrations.","PeriodicalId":24,"journal":{"name":"ACS Sensors","volume":"69 1","pages":""},"PeriodicalIF":9.1000,"publicationDate":"2025-09-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Highly Selective MEMS Gas Sensor Based on Temperature-Programmed Desorption Technology.\",\"authors\":\"Junming Shao,Renjun Si,Hongze Jiang,Shaofeng Chen,Jiabao Ding,Zheng Wang,Shunping Zhang\",\"doi\":\"10.1021/acssensors.5c01413\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Aiming at the issue of poor selectivity in metal oxide gas sensors, a novel MEMS gas sensor structure was designed, comprising an adsorption unit and a sensing unit. Based on this design, a gas-sensing method utilizing on-chip programmable temperature analysis technology was developed. By quantifying the gas-sensitive response, we successfully extracted the peak signal of temperature-dependent resistance with high selectivity. The performance results show that ZSM-5, as the adsorbent material, exhibits desorption peak positions at different temperatures for four types of alcohol gases, and the peak height is correlated with the adsorption concentration. The essence of its high selectivity lies in the fact that materials have different desorption activation energies for different gases under the same conditions. This study proposes a new selective MEMS device testing method for identifying gas types and concentrations.\",\"PeriodicalId\":24,\"journal\":{\"name\":\"ACS Sensors\",\"volume\":\"69 1\",\"pages\":\"\"},\"PeriodicalIF\":9.1000,\"publicationDate\":\"2025-09-30\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Sensors\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://doi.org/10.1021/acssensors.5c01413\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, ANALYTICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Sensors","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1021/acssensors.5c01413","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, ANALYTICAL","Score":null,"Total":0}
Highly Selective MEMS Gas Sensor Based on Temperature-Programmed Desorption Technology.
Aiming at the issue of poor selectivity in metal oxide gas sensors, a novel MEMS gas sensor structure was designed, comprising an adsorption unit and a sensing unit. Based on this design, a gas-sensing method utilizing on-chip programmable temperature analysis technology was developed. By quantifying the gas-sensitive response, we successfully extracted the peak signal of temperature-dependent resistance with high selectivity. The performance results show that ZSM-5, as the adsorbent material, exhibits desorption peak positions at different temperatures for four types of alcohol gases, and the peak height is correlated with the adsorption concentration. The essence of its high selectivity lies in the fact that materials have different desorption activation energies for different gases under the same conditions. This study proposes a new selective MEMS device testing method for identifying gas types and concentrations.
期刊介绍:
ACS Sensors is a peer-reviewed research journal that focuses on the dissemination of new and original knowledge in the field of sensor science, particularly those that selectively sense chemical or biological species or processes. The journal covers a broad range of topics, including but not limited to biosensors, chemical sensors, gas sensors, intracellular sensors, single molecule sensors, cell chips, and microfluidic devices. It aims to publish articles that address conceptual advances in sensing technology applicable to various types of analytes or application papers that report on the use of existing sensing concepts in new ways or for new analytes.