{"title":"非中心对称半导体单层中周期性反铁磁斯基米子的场驱动演化","authors":"Liyenda Gogoi, P. Deb","doi":"10.1039/d5nr03229f","DOIUrl":null,"url":null,"abstract":"Antiferromagnetic skyrmions are topologically protected, stable nanoscale spin textures with countable particle-like properties, which are resistant to skyrmion Hall effect, and suitable for high-density data storage spintronic applications. However, the absence of long-range periodic antiferromagnetic skyrmion order in dynamically stable single-layer semiconducting materials hinders the compatibility and integrability of skyrmion-based devices with existing semiconductor-based technologies. Here, in this work, we demonstrate the nucleation of periodic antiferromagnetic skyrmions in a Janus non-centrosymmetric semiconducting monolayer, MnBrCl. In the Janus monolayer with a unique antiferromagnetic double-stranded helical ground state configuration of magnetic moments, a periodic antiferromagnetic skyrmion is nucleated under a magnetic field, which has not been reported previously. We have thoroughly investigated the microscopic origin of this periodic, topologically protected structure and propose a four-sublattice framework that explains the field-driven nucleation of antiferromagnetic skyrmions. This mechanism of antiferromagnetic skyrmion evolution, based on the four-sublattice framework, offers a new perspective on the formation of periodic antiferromagnetic skyrmions. Our analysis also provides deeper insight into the controllability of magnetic topology in Janus non-centrosymmetric material. Further, the magnetic tunability of the nucleated periodic AFM skyrmions suggests suitability of the materials for parallel processing applications in multi-state memory devices and neuromorphic computing, thereby enriching the domain of AFM skyrmion based spintronic.","PeriodicalId":92,"journal":{"name":"Nanoscale","volume":"17 1","pages":""},"PeriodicalIF":5.1000,"publicationDate":"2025-09-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Field driven evolution of periodic antiferromagnetic skyrmion in non-centrosymmetric semiconducting monolayer\",\"authors\":\"Liyenda Gogoi, P. Deb\",\"doi\":\"10.1039/d5nr03229f\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Antiferromagnetic skyrmions are topologically protected, stable nanoscale spin textures with countable particle-like properties, which are resistant to skyrmion Hall effect, and suitable for high-density data storage spintronic applications. However, the absence of long-range periodic antiferromagnetic skyrmion order in dynamically stable single-layer semiconducting materials hinders the compatibility and integrability of skyrmion-based devices with existing semiconductor-based technologies. Here, in this work, we demonstrate the nucleation of periodic antiferromagnetic skyrmions in a Janus non-centrosymmetric semiconducting monolayer, MnBrCl. In the Janus monolayer with a unique antiferromagnetic double-stranded helical ground state configuration of magnetic moments, a periodic antiferromagnetic skyrmion is nucleated under a magnetic field, which has not been reported previously. We have thoroughly investigated the microscopic origin of this periodic, topologically protected structure and propose a four-sublattice framework that explains the field-driven nucleation of antiferromagnetic skyrmions. This mechanism of antiferromagnetic skyrmion evolution, based on the four-sublattice framework, offers a new perspective on the formation of periodic antiferromagnetic skyrmions. Our analysis also provides deeper insight into the controllability of magnetic topology in Janus non-centrosymmetric material. Further, the magnetic tunability of the nucleated periodic AFM skyrmions suggests suitability of the materials for parallel processing applications in multi-state memory devices and neuromorphic computing, thereby enriching the domain of AFM skyrmion based spintronic.\",\"PeriodicalId\":92,\"journal\":{\"name\":\"Nanoscale\",\"volume\":\"17 1\",\"pages\":\"\"},\"PeriodicalIF\":5.1000,\"publicationDate\":\"2025-09-29\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nanoscale\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1039/d5nr03229f\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nanoscale","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1039/d5nr03229f","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Field driven evolution of periodic antiferromagnetic skyrmion in non-centrosymmetric semiconducting monolayer
Antiferromagnetic skyrmions are topologically protected, stable nanoscale spin textures with countable particle-like properties, which are resistant to skyrmion Hall effect, and suitable for high-density data storage spintronic applications. However, the absence of long-range periodic antiferromagnetic skyrmion order in dynamically stable single-layer semiconducting materials hinders the compatibility and integrability of skyrmion-based devices with existing semiconductor-based technologies. Here, in this work, we demonstrate the nucleation of periodic antiferromagnetic skyrmions in a Janus non-centrosymmetric semiconducting monolayer, MnBrCl. In the Janus monolayer with a unique antiferromagnetic double-stranded helical ground state configuration of magnetic moments, a periodic antiferromagnetic skyrmion is nucleated under a magnetic field, which has not been reported previously. We have thoroughly investigated the microscopic origin of this periodic, topologically protected structure and propose a four-sublattice framework that explains the field-driven nucleation of antiferromagnetic skyrmions. This mechanism of antiferromagnetic skyrmion evolution, based on the four-sublattice framework, offers a new perspective on the formation of periodic antiferromagnetic skyrmions. Our analysis also provides deeper insight into the controllability of magnetic topology in Janus non-centrosymmetric material. Further, the magnetic tunability of the nucleated periodic AFM skyrmions suggests suitability of the materials for parallel processing applications in multi-state memory devices and neuromorphic computing, thereby enriching the domain of AFM skyrmion based spintronic.
期刊介绍:
Nanoscale is a high-impact international journal, publishing high-quality research across nanoscience and nanotechnology. Nanoscale publishes a full mix of research articles on experimental and theoretical work, including reviews, communications, and full papers.Highly interdisciplinary, this journal appeals to scientists, researchers and professionals interested in nanoscience and nanotechnology, quantum materials and quantum technology, including the areas of physics, chemistry, biology, medicine, materials, energy/environment, information technology, detection science, healthcare and drug discovery, and electronics.