{"title":"利用先进的锌基金属有机骨架材料进行燃烧后碳捕获和转化:综述","authors":"Yuhui Jin, Feichao Li, Yun Zheng, Wenqiang Zhang, Shufan Wang, Wei Yan, Bo Yu, Jiujun Zhang","doi":"10.1007/s11708-025-1009-1","DOIUrl":null,"url":null,"abstract":"<div><p>Developing environmentalyl friendly and energy-efficient CO<sub>2</sub> adsorbents for post-combustion capture is a critical step toward achieving toward carbon neutrality. While aqueous amines and metal oxides have play pivotal roles in CO<sub>2</sub> capture, their application is limited by issues such as secondary pollution and high energy consumption. In contrast, Zn-based metal-organic frameworks (Zn-based MOFs) have emerged as a green alternative, offering low toxicity reduced regeneration temperatures, and high efficiency in both CO<sub>2</sub> adsorption and catalytic conversion into valuable fuels and chemicals. This mini review begins with a general introduction to MOFs in CO<sub>2</sub> capture and conversion, followed by an overview of early studies on Zn-based MOFs for CO<sub>2</sub> capture. It then summarizes recent research advancements in Zn-based MOFs for integrated CO<sub>2</sub> capture and conversion. Finally, it discusses key challenges and future research directions for post-combustion CO<sub>2</sub> capture and conversion using Zn-based MOFs.</p></div>","PeriodicalId":570,"journal":{"name":"Frontiers in Energy","volume":"19 3","pages":"300 - 311"},"PeriodicalIF":6.2000,"publicationDate":"2025-05-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Post-combustion carbon capture and conversion using advanced materials of Zn-based metal-organic frameworks: A mini review\",\"authors\":\"Yuhui Jin, Feichao Li, Yun Zheng, Wenqiang Zhang, Shufan Wang, Wei Yan, Bo Yu, Jiujun Zhang\",\"doi\":\"10.1007/s11708-025-1009-1\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Developing environmentalyl friendly and energy-efficient CO<sub>2</sub> adsorbents for post-combustion capture is a critical step toward achieving toward carbon neutrality. While aqueous amines and metal oxides have play pivotal roles in CO<sub>2</sub> capture, their application is limited by issues such as secondary pollution and high energy consumption. In contrast, Zn-based metal-organic frameworks (Zn-based MOFs) have emerged as a green alternative, offering low toxicity reduced regeneration temperatures, and high efficiency in both CO<sub>2</sub> adsorption and catalytic conversion into valuable fuels and chemicals. This mini review begins with a general introduction to MOFs in CO<sub>2</sub> capture and conversion, followed by an overview of early studies on Zn-based MOFs for CO<sub>2</sub> capture. It then summarizes recent research advancements in Zn-based MOFs for integrated CO<sub>2</sub> capture and conversion. Finally, it discusses key challenges and future research directions for post-combustion CO<sub>2</sub> capture and conversion using Zn-based MOFs.</p></div>\",\"PeriodicalId\":570,\"journal\":{\"name\":\"Frontiers in Energy\",\"volume\":\"19 3\",\"pages\":\"300 - 311\"},\"PeriodicalIF\":6.2000,\"publicationDate\":\"2025-05-15\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Frontiers in Energy\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s11708-025-1009-1\",\"RegionNum\":4,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ENERGY & FUELS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Frontiers in Energy","FirstCategoryId":"5","ListUrlMain":"https://link.springer.com/article/10.1007/s11708-025-1009-1","RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
Post-combustion carbon capture and conversion using advanced materials of Zn-based metal-organic frameworks: A mini review
Developing environmentalyl friendly and energy-efficient CO2 adsorbents for post-combustion capture is a critical step toward achieving toward carbon neutrality. While aqueous amines and metal oxides have play pivotal roles in CO2 capture, their application is limited by issues such as secondary pollution and high energy consumption. In contrast, Zn-based metal-organic frameworks (Zn-based MOFs) have emerged as a green alternative, offering low toxicity reduced regeneration temperatures, and high efficiency in both CO2 adsorption and catalytic conversion into valuable fuels and chemicals. This mini review begins with a general introduction to MOFs in CO2 capture and conversion, followed by an overview of early studies on Zn-based MOFs for CO2 capture. It then summarizes recent research advancements in Zn-based MOFs for integrated CO2 capture and conversion. Finally, it discusses key challenges and future research directions for post-combustion CO2 capture and conversion using Zn-based MOFs.
期刊介绍:
Frontiers in Energy, an interdisciplinary and peer-reviewed international journal launched in January 2007, seeks to provide a rapid and unique platform for reporting the most advanced research on energy technology and strategic thinking in order to promote timely communication between researchers, scientists, engineers, and policy makers in the field of energy.
Frontiers in Energy aims to be a leading peer-reviewed platform and an authoritative source of information for analyses, reviews and evaluations in energy engineering and research, with a strong focus on energy analysis, energy modelling and prediction, integrated energy systems, energy conversion and conservation, energy planning and energy on economic and policy issues.
Frontiers in Energy publishes state-of-the-art review articles, original research papers and short communications by individual researchers or research groups. It is strictly peer-reviewed and accepts only original submissions in English. The scope of the journal is broad and covers all latest focus in current energy research.
High-quality papers are solicited in, but are not limited to the following areas:
-Fundamental energy science
-Energy technology, including energy generation, conversion, storage, renewables, transport, urban design and building efficiency
-Energy and the environment, including pollution control, energy efficiency and climate change
-Energy economics, strategy and policy
-Emerging energy issue