ZnO-CuO压电催化剂的合成与效能:高效降解水中有机污染物和抗菌的高性价比催化剂

IF 2.3 4区 化学 Q3 CHEMISTRY, PHYSICAL
Longhao Xiao, Wenxia Ma, Haibo Li, Yunzi Yu, Shuming Liu, Xianglong Zeng, Zheng Fang, Kai Yao, Zhenhui Hu, Yongsheng Yang, Hongjun Liu, Corresponging Yongsheng Yang
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引用次数: 0

摘要

由于环境问题和现实考虑,有机污染物的降解已成为人们关注的焦点。本研究通过原位法合成了一种经济高效的掺杂CuO的ZnO压电催化剂。该研究强调了ZnO-CuO压电催化剂在不同锌铜比下的卓越降解效果,在1:1的比例下达到最佳催化活性。使用有机染料(亚甲基蓝、刚果红和罗丹明B)的降解实验显示了令人印象深刻的结果,在室温、黑暗环境下磁力搅拌90分钟后,亚甲基蓝的降解率约为90%。电化学阻抗谱(EIS)分析表明,催化剂的高压电活性可归因于其低载流子转移阻力,有利于载流子分离的动力学过程。此外,该催化剂还表现出明显的抑菌能力。大规模合成ZnO-CuO压电催化剂为水质修复提供了一条经济、高效、有前景的途径。图形抽象
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Synthesis and Efficacy of ZnO-CuO Piezoelectric Catalysts: A Cost-Effective Catalysts for Efficient Degradation of Organic Pollutants and Antibacterial in Water

The degradation of organic pollutants has become a focal point due to environmental concerns and practical considerations. In this study, a cost-effective and efficient ZnO piezoelectric catalyst doped with CuO was synthesized through an in-situ method. The research highlights the exceptional degradation effectiveness of the ZnO-CuO piezoelectric catalyst across various zinc-copper ratios, with the optimum catalytic activity achieved at a 1:1 ratio. Degradation experiments using organic dyes (Methylene Blue, Congo Red, and Rhodamine B) revealed impressive results, with methylene blue exhibiting a degradation rate of approximately 90% after 90 min under magnetic stirring at room temperature in a dark environment. Electrochemical impedance spectroscopy (EIS) analysis suggested that the catalyst’s high piezoelectric activity can be attributed to its low charge carrier transfer resistance, facilitating the kinetic process of charge carrier separation. Furthermore, the catalyst exhibited notable antibacterial inhibition capabilities. The synthesis of ZnO-CuO piezoelectric catalysts on a large scale offers a promising, economical, and efficient approach for water quality remediation.

Graphical Abstract

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来源期刊
Catalysis Letters
Catalysis Letters 化学-物理化学
CiteScore
5.70
自引率
3.60%
发文量
327
审稿时长
1 months
期刊介绍: Catalysis Letters aim is the rapid publication of outstanding and high-impact original research articles in catalysis. The scope of the journal covers a broad range of topics in all fields of both applied and theoretical catalysis, including heterogeneous, homogeneous and biocatalysis. The high-quality original research articles published in Catalysis Letters are subject to rigorous peer review. Accepted papers are published online first and subsequently in print issues. All contributions must include a graphical abstract. Manuscripts should be written in English and the responsibility lies with the authors to ensure that they are grammatically and linguistically correct. Authors for whom English is not the working language are encouraged to consider using a professional language-editing service before submitting their manuscripts.
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