环境应用的mxene基复合材料:最新进展

IF 7.2 2区 工程技术 Q1 ENGINEERING, CHEMICAL
Navid Rabiee
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引用次数: 0

摘要

基于mxene的复合材料已经成为环境应用的革命性材料,在水处理、空气净化和资源回收方面提供了前所未有的能力。这篇综述提出了一个全面的评估最近的进展,跨越可持续合成创新到先进的复合材料设计策略。MXenes独特的结合了金属导电性、亲水性表面化学和可调层间间距,使其成为应对关键环境挑战的高度通用平台。在重金属去除方面取得了重大进展,吸附量超过1000 mg/g,并通过光催化和Fenton-like途径降解有机污染物。新兴的合成方法,包括无氟蚀刻和电化学方法,提高了可扩展性和材料性能。mxene基膜因其优异的离子选择性和染料抑制性能而被突出,而与金属有机框架、层状双氢氧化物和聚合物基质的集成产生了具有增强稳定性、选择性和耐久性的多功能复合材料。光催化应用进一步展示了出色的析氢和二氧化碳还原效率,而基于mxene的传感器对高优先级污染物的检测极限从ppb到ppq不等。本文的新颖之处在于其多维性能分析和综合视角,将实验结果、理论模型和应用前景统一到一个预测框架中。该方法揭示了结构-性能-功能关系、跨环境技术的横切设计原则和优化策略,为定制复合材料开发提供了可操作的见解。通过将批判性评估与前瞻性战略相结合,本综述不仅突出了MXenes的变革潜力,而且为可扩展和可持续的环境技术定义了明确的研究途径。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
MXene-based composites for environmental applications: Recent advances
MXene-based composites have emerged as revolutionary materials for environmental applications, offering unprecedented capabilities in water treatment, air purification, and resource recovery. This review presents a comprehensive assessment of recent advances, spanning sustainable synthesis innovations to advanced composite design strategies. The unique combination of metallic conductivity, hydrophilic surface chemistry, and tunable interlayer spacing positions MXenes as highly versatile platforms for tackling critical environmental challenges. Significant progress has been demonstrated in heavy metal removal, with adsorption capacities exceeding 1000 mg/g, and in organic pollutant degradation via photocatalytic and Fenton-like pathways. Emerging synthesis approaches, including fluoride-free etching and electrochemical methods, have improved both scalability and material performance. MXene-based membranes are highlighted for their superior ion selectivity and dye rejection, while integration with metal–organic frameworks, layered double hydroxides, and polymer matrices has generated multifunctional composites with enhanced stability, selectivity, and durability. Photocatalytic applications further demonstrate outstanding hydrogen evolution and CO2 reduction efficiencies, while MXene-based sensors achieve detection limits ranging from ppb to ppq levels for high-priority contaminants. The novelty of this review lies in its multi-dimensional performance analysis and integrative perspective, which unify experimental findings, theoretical models, and application prospects into a predictive framework. This approach reveals structure–property–function relationships, cross-cutting design principles, and optimization strategies across diverse environmental technologies, offering actionable insights for tailored composite development. By combining critical evaluation with forward-looking strategies, this review not only highlights the transformative potential of MXenes but also defines clear research pathways toward scalable and sustainable environmental technologies.
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来源期刊
Journal of Environmental Chemical Engineering
Journal of Environmental Chemical Engineering Environmental Science-Pollution
CiteScore
11.40
自引率
6.50%
发文量
2017
审稿时长
27 days
期刊介绍: The Journal of Environmental Chemical Engineering (JECE) serves as a platform for the dissemination of original and innovative research focusing on the advancement of environmentally-friendly, sustainable technologies. JECE emphasizes the transition towards a carbon-neutral circular economy and a self-sufficient bio-based economy. Topics covered include soil, water, wastewater, and air decontamination; pollution monitoring, prevention, and control; advanced analytics, sensors, impact and risk assessment methodologies in environmental chemical engineering; resource recovery (water, nutrients, materials, energy); industrial ecology; valorization of waste streams; waste management (including e-waste); climate-water-energy-food nexus; novel materials for environmental, chemical, and energy applications; sustainability and environmental safety; water digitalization, water data science, and machine learning; process integration and intensification; recent developments in green chemistry for synthesis, catalysis, and energy; and original research on contaminants of emerging concern, persistent chemicals, and priority substances, including microplastics, nanoplastics, nanomaterials, micropollutants, antimicrobial resistance genes, and emerging pathogens (viruses, bacteria, parasites) of environmental significance.
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