{"title":"环境应用的mxene基复合材料:最新进展","authors":"Navid Rabiee","doi":"10.1016/j.jece.2025.119521","DOIUrl":null,"url":null,"abstract":"<div><div>MXene-based composites have emerged as revolutionary materials for environmental applications, offering unprecedented capabilities in water treatment, air purification, and resource recovery. This review presents a comprehensive assessment of recent advances, spanning sustainable synthesis innovations to advanced composite design strategies. The unique combination of metallic conductivity, hydrophilic surface chemistry, and tunable interlayer spacing positions MXenes as highly versatile platforms for tackling critical environmental challenges. Significant progress has been demonstrated in heavy metal removal, with adsorption capacities exceeding 1000 mg/g, and in organic pollutant degradation via photocatalytic and Fenton-like pathways. Emerging synthesis approaches, including fluoride-free etching and electrochemical methods, have improved both scalability and material performance. MXene-based membranes are highlighted for their superior ion selectivity and dye rejection, while integration with metal–organic frameworks, layered double hydroxides, and polymer matrices has generated multifunctional composites with enhanced stability, selectivity, and durability. Photocatalytic applications further demonstrate outstanding hydrogen evolution and CO<sub>2</sub> reduction efficiencies, while MXene-based sensors achieve detection limits ranging from ppb to ppq levels for high-priority contaminants. The novelty of this review lies in its multi-dimensional performance analysis and integrative perspective, which unify experimental findings, theoretical models, and application prospects into a predictive framework. This approach reveals structure–property–function relationships, cross-cutting design principles, and optimization strategies across diverse environmental technologies, offering actionable insights for tailored composite development. By combining critical evaluation with forward-looking strategies, this review not only highlights the transformative potential of MXenes but also defines clear research pathways toward scalable and sustainable environmental technologies.</div></div>","PeriodicalId":15759,"journal":{"name":"Journal of Environmental Chemical Engineering","volume":"13 6","pages":"Article 119521"},"PeriodicalIF":7.2000,"publicationDate":"2025-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"MXene-based composites for environmental applications: Recent advances\",\"authors\":\"Navid Rabiee\",\"doi\":\"10.1016/j.jece.2025.119521\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>MXene-based composites have emerged as revolutionary materials for environmental applications, offering unprecedented capabilities in water treatment, air purification, and resource recovery. This review presents a comprehensive assessment of recent advances, spanning sustainable synthesis innovations to advanced composite design strategies. The unique combination of metallic conductivity, hydrophilic surface chemistry, and tunable interlayer spacing positions MXenes as highly versatile platforms for tackling critical environmental challenges. Significant progress has been demonstrated in heavy metal removal, with adsorption capacities exceeding 1000 mg/g, and in organic pollutant degradation via photocatalytic and Fenton-like pathways. Emerging synthesis approaches, including fluoride-free etching and electrochemical methods, have improved both scalability and material performance. MXene-based membranes are highlighted for their superior ion selectivity and dye rejection, while integration with metal–organic frameworks, layered double hydroxides, and polymer matrices has generated multifunctional composites with enhanced stability, selectivity, and durability. Photocatalytic applications further demonstrate outstanding hydrogen evolution and CO<sub>2</sub> reduction efficiencies, while MXene-based sensors achieve detection limits ranging from ppb to ppq levels for high-priority contaminants. The novelty of this review lies in its multi-dimensional performance analysis and integrative perspective, which unify experimental findings, theoretical models, and application prospects into a predictive framework. This approach reveals structure–property–function relationships, cross-cutting design principles, and optimization strategies across diverse environmental technologies, offering actionable insights for tailored composite development. By combining critical evaluation with forward-looking strategies, this review not only highlights the transformative potential of MXenes but also defines clear research pathways toward scalable and sustainable environmental technologies.</div></div>\",\"PeriodicalId\":15759,\"journal\":{\"name\":\"Journal of Environmental Chemical Engineering\",\"volume\":\"13 6\",\"pages\":\"Article 119521\"},\"PeriodicalIF\":7.2000,\"publicationDate\":\"2025-09-25\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Environmental Chemical Engineering\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2213343725042174\",\"RegionNum\":2,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Environmental Chemical Engineering","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2213343725042174","RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
MXene-based composites for environmental applications: Recent advances
MXene-based composites have emerged as revolutionary materials for environmental applications, offering unprecedented capabilities in water treatment, air purification, and resource recovery. This review presents a comprehensive assessment of recent advances, spanning sustainable synthesis innovations to advanced composite design strategies. The unique combination of metallic conductivity, hydrophilic surface chemistry, and tunable interlayer spacing positions MXenes as highly versatile platforms for tackling critical environmental challenges. Significant progress has been demonstrated in heavy metal removal, with adsorption capacities exceeding 1000 mg/g, and in organic pollutant degradation via photocatalytic and Fenton-like pathways. Emerging synthesis approaches, including fluoride-free etching and electrochemical methods, have improved both scalability and material performance. MXene-based membranes are highlighted for their superior ion selectivity and dye rejection, while integration with metal–organic frameworks, layered double hydroxides, and polymer matrices has generated multifunctional composites with enhanced stability, selectivity, and durability. Photocatalytic applications further demonstrate outstanding hydrogen evolution and CO2 reduction efficiencies, while MXene-based sensors achieve detection limits ranging from ppb to ppq levels for high-priority contaminants. The novelty of this review lies in its multi-dimensional performance analysis and integrative perspective, which unify experimental findings, theoretical models, and application prospects into a predictive framework. This approach reveals structure–property–function relationships, cross-cutting design principles, and optimization strategies across diverse environmental technologies, offering actionable insights for tailored composite development. By combining critical evaluation with forward-looking strategies, this review not only highlights the transformative potential of MXenes but also defines clear research pathways toward scalable and sustainable environmental technologies.
期刊介绍:
The Journal of Environmental Chemical Engineering (JECE) serves as a platform for the dissemination of original and innovative research focusing on the advancement of environmentally-friendly, sustainable technologies. JECE emphasizes the transition towards a carbon-neutral circular economy and a self-sufficient bio-based economy. Topics covered include soil, water, wastewater, and air decontamination; pollution monitoring, prevention, and control; advanced analytics, sensors, impact and risk assessment methodologies in environmental chemical engineering; resource recovery (water, nutrients, materials, energy); industrial ecology; valorization of waste streams; waste management (including e-waste); climate-water-energy-food nexus; novel materials for environmental, chemical, and energy applications; sustainability and environmental safety; water digitalization, water data science, and machine learning; process integration and intensification; recent developments in green chemistry for synthesis, catalysis, and energy; and original research on contaminants of emerging concern, persistent chemicals, and priority substances, including microplastics, nanoplastics, nanomaterials, micropollutants, antimicrobial resistance genes, and emerging pathogens (viruses, bacteria, parasites) of environmental significance.