Barlin Das , Binita Pathak , Uday Bhattacharjee , Partha Jyoti Sahu , Arundhati Kundu , Arup Borgohain , Mukunda M. Gogoi , Shyam S. Kundu , Kalyan Bhuyan , Pradip K. Bhuyan
{"title":"喜马拉雅山麓东部城市地区npf诱导的CCN增强:一项基于运动的研究","authors":"Barlin Das , Binita Pathak , Uday Bhattacharjee , Partha Jyoti Sahu , Arundhati Kundu , Arup Borgohain , Mukunda M. Gogoi , Shyam S. Kundu , Kalyan Bhuyan , Pradip K. Bhuyan","doi":"10.1016/j.atmosenv.2025.121524","DOIUrl":null,"url":null,"abstract":"<div><div>The New Particle Formation (NPF) mechanism plays a significant role in regulating the cloud condensation nuclei (CCN). Here, we present results from a campaign mode study during 3 January - 4 February 2023 obtained from simultaneous measurements of particle number concentration within a size range 10–300 nm (N<sub>10-300</sub>) using the scanning mobility particle sizer (SMPS) and CCN concentrations (N<sub>CCN</sub>) using a CCN Counter (CCNc) over an urban location, Dibrugarh, in the Eastern Himalayan Foothills. The mean diurnal variation of N<sub>CCN</sub> at supersaturations (SS) 0.2 %–1.0 % exhibits similar variation to the total number concentration of aerosols (N<sub>10-300</sub>) measured by the SMPS. Both exhibit higher concentrations during nighttime and lower during daytime, primarily influenced by atmospheric boundary layer (ABL) dynamics. We have identified four NPF events during the study period. The new particle burst appeared below 25 nm, while the growth process sustained for 12 to 17 h at the growth rate from 4.5 to 7.2 nm h<sup>−1</sup>. The growth process begins with coagulation, followed by condensation, which becomes the dominant mechanism in the formation of CCN. Further, the enhancement factor of CCN due to NPF (E_N<sub>CCN</sub>) was estimated to examine the aerosol-CCN interaction. E_N<sub>CCN</sub> was found to vary between 2 and 8 for the four NPF events at the SS range 0.2–1 %, which are comparable to those over many urban places across the globe.</div></div>","PeriodicalId":250,"journal":{"name":"Atmospheric Environment","volume":"362 ","pages":"Article 121524"},"PeriodicalIF":3.7000,"publicationDate":"2025-09-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"NPF-induced CCN enhancement over an urban location in Eastern Himalayan Foothills: A campaign-based study\",\"authors\":\"Barlin Das , Binita Pathak , Uday Bhattacharjee , Partha Jyoti Sahu , Arundhati Kundu , Arup Borgohain , Mukunda M. Gogoi , Shyam S. Kundu , Kalyan Bhuyan , Pradip K. Bhuyan\",\"doi\":\"10.1016/j.atmosenv.2025.121524\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The New Particle Formation (NPF) mechanism plays a significant role in regulating the cloud condensation nuclei (CCN). Here, we present results from a campaign mode study during 3 January - 4 February 2023 obtained from simultaneous measurements of particle number concentration within a size range 10–300 nm (N<sub>10-300</sub>) using the scanning mobility particle sizer (SMPS) and CCN concentrations (N<sub>CCN</sub>) using a CCN Counter (CCNc) over an urban location, Dibrugarh, in the Eastern Himalayan Foothills. The mean diurnal variation of N<sub>CCN</sub> at supersaturations (SS) 0.2 %–1.0 % exhibits similar variation to the total number concentration of aerosols (N<sub>10-300</sub>) measured by the SMPS. Both exhibit higher concentrations during nighttime and lower during daytime, primarily influenced by atmospheric boundary layer (ABL) dynamics. We have identified four NPF events during the study period. The new particle burst appeared below 25 nm, while the growth process sustained for 12 to 17 h at the growth rate from 4.5 to 7.2 nm h<sup>−1</sup>. The growth process begins with coagulation, followed by condensation, which becomes the dominant mechanism in the formation of CCN. Further, the enhancement factor of CCN due to NPF (E_N<sub>CCN</sub>) was estimated to examine the aerosol-CCN interaction. 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NPF-induced CCN enhancement over an urban location in Eastern Himalayan Foothills: A campaign-based study
The New Particle Formation (NPF) mechanism plays a significant role in regulating the cloud condensation nuclei (CCN). Here, we present results from a campaign mode study during 3 January - 4 February 2023 obtained from simultaneous measurements of particle number concentration within a size range 10–300 nm (N10-300) using the scanning mobility particle sizer (SMPS) and CCN concentrations (NCCN) using a CCN Counter (CCNc) over an urban location, Dibrugarh, in the Eastern Himalayan Foothills. The mean diurnal variation of NCCN at supersaturations (SS) 0.2 %–1.0 % exhibits similar variation to the total number concentration of aerosols (N10-300) measured by the SMPS. Both exhibit higher concentrations during nighttime and lower during daytime, primarily influenced by atmospheric boundary layer (ABL) dynamics. We have identified four NPF events during the study period. The new particle burst appeared below 25 nm, while the growth process sustained for 12 to 17 h at the growth rate from 4.5 to 7.2 nm h−1. The growth process begins with coagulation, followed by condensation, which becomes the dominant mechanism in the formation of CCN. Further, the enhancement factor of CCN due to NPF (E_NCCN) was estimated to examine the aerosol-CCN interaction. E_NCCN was found to vary between 2 and 8 for the four NPF events at the SS range 0.2–1 %, which are comparable to those over many urban places across the globe.
期刊介绍:
Atmospheric Environment has an open access mirror journal Atmospheric Environment: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review.
Atmospheric Environment is the international journal for scientists in different disciplines related to atmospheric composition and its impacts. The journal publishes scientific articles with atmospheric relevance of emissions and depositions of gaseous and particulate compounds, chemical processes and physical effects in the atmosphere, as well as impacts of the changing atmospheric composition on human health, air quality, climate change, and ecosystems.