喜马拉雅山麓东部城市地区npf诱导的CCN增强:一项基于运动的研究

IF 3.7 2区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES
Barlin Das , Binita Pathak , Uday Bhattacharjee , Partha Jyoti Sahu , Arundhati Kundu , Arup Borgohain , Mukunda M. Gogoi , Shyam S. Kundu , Kalyan Bhuyan , Pradip K. Bhuyan
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引用次数: 0

摘要

新粒子形成(NPF)机制在云凝结核(CCN)中起着重要的调节作用。在这里,我们展示了2023年1月3日至2月4日期间的运动模式研究结果,该研究使用扫描迁移率粒径仪(SMPS)同时测量了10-300 nm (N10-300)范围内的颗粒数浓度,并使用CCN计数仪(CCNc)同时测量了CCN浓度(NCCN),测量地点为东喜马拉雅山麓迪布鲁加尔(Dibrugarh)。在过饱和度(SS) 0.2% ~ 1.0%时,NCCN的平均日变化与SMPS测量的气溶胶总数浓度(N10-300)的变化相似。两者的浓度在夜间较高,白天较低,主要受大气边界层(ABL)动力学的影响。在研究期间,我们确定了四个NPF事件。在25 nm以下出现新粒子爆发,生长速度为4.5 ~ 7.2 nm h−1,持续12 ~ 17 h。生长过程从凝聚开始,然后是凝聚,这成为CCN形成的主要机制。此外,估计了NPF对CCN的增强因子(E_NCCN),以检验气溶胶与CCN的相互作用。在SS范围为0.2 - 1%的4个NPF事件中,E_NCCN在2 - 8之间变化,这与全球许多城市地区的情况相当。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
NPF-induced CCN enhancement over an urban location in Eastern Himalayan Foothills: A campaign-based study
The New Particle Formation (NPF) mechanism plays a significant role in regulating the cloud condensation nuclei (CCN). Here, we present results from a campaign mode study during 3 January - 4 February 2023 obtained from simultaneous measurements of particle number concentration within a size range 10–300 nm (N10-300) using the scanning mobility particle sizer (SMPS) and CCN concentrations (NCCN) using a CCN Counter (CCNc) over an urban location, Dibrugarh, in the Eastern Himalayan Foothills. The mean diurnal variation of NCCN at supersaturations (SS) 0.2 %–1.0 % exhibits similar variation to the total number concentration of aerosols (N10-300) measured by the SMPS. Both exhibit higher concentrations during nighttime and lower during daytime, primarily influenced by atmospheric boundary layer (ABL) dynamics. We have identified four NPF events during the study period. The new particle burst appeared below 25 nm, while the growth process sustained for 12 to 17 h at the growth rate from 4.5 to 7.2 nm h−1. The growth process begins with coagulation, followed by condensation, which becomes the dominant mechanism in the formation of CCN. Further, the enhancement factor of CCN due to NPF (E_NCCN) was estimated to examine the aerosol-CCN interaction. E_NCCN was found to vary between 2 and 8 for the four NPF events at the SS range 0.2–1 %, which are comparable to those over many urban places across the globe.
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来源期刊
Atmospheric Environment
Atmospheric Environment 环境科学-环境科学
CiteScore
9.40
自引率
8.00%
发文量
458
审稿时长
53 days
期刊介绍: Atmospheric Environment has an open access mirror journal Atmospheric Environment: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review. Atmospheric Environment is the international journal for scientists in different disciplines related to atmospheric composition and its impacts. The journal publishes scientific articles with atmospheric relevance of emissions and depositions of gaseous and particulate compounds, chemical processes and physical effects in the atmosphere, as well as impacts of the changing atmospheric composition on human health, air quality, climate change, and ecosystems.
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