Haodong Fan , Han Zhang , Geng Li , Xiong Zhang , Zixue Luo , Lin Huang , Shihong Zhang
{"title":"工业生物质流化床气化系统建模及运行条件优化","authors":"Haodong Fan , Han Zhang , Geng Li , Xiong Zhang , Zixue Luo , Lin Huang , Shihong Zhang","doi":"10.1016/j.biombioe.2025.108403","DOIUrl":null,"url":null,"abstract":"<div><div>Carbon emissions from fossil fuel combustion have emerged as a critical constraint on sustainable industrial development. Biomass gasification gas (BGG) represents a promising decarbonization pathway; however, the reliance on single-source biomass cannot ensure the operational reliability of industrial fluidized bed gasifiers. A key challenge to large-scale BGG adoption lies in the limited adaptability of fluidized bed reactors to different biomass, which exhibit heterogeneous physicochemical properties. Moreover, industrial research on the impact of structural parameters on gasification efficiency remains scarce. To investigate the impact of different biomass on gasification performance in fluidized-bed reactors, this study developed an industrial-scale fluidized-bed gasifier model using the Aspen Plus fluidized-bed module, based on an 8 t/h biomass gasifier operating in a regional facility. Key parameters, including equivalence ratio (ER), gasification pressure, and gasification temperature, were systematically evaluated to assess their effects on BGG composition and gasification efficiency. Furthermore, model validity was rigorously validated through computational and experimental data comparisons of critical design parameters. The results demonstrated that gasification temperature and ER are critical factors influencing biomass gasification efficiency. When the gasification temperature increased from 650 to 900 °C, the gas yield variation of corn stover and wooden blocks reached a maximum of 0.17 m<sup>3</sup>/kg. For corn stover gasification, the volumetric fractions of H<sub>2</sub>, CO, CO<sub>2</sub>, and CH<sub>4</sub> exhibited an increasing trend, rising by 11.43 %, 8.41 %, 7.73 %, and 2.24 %, respectively. Notably, biomass briquette gasification showed the most significant increase in H<sub>2</sub> fraction (11.4 %). Balancing operational safety and efficiency, the optimal gasification temperature was identified as 850 °C, with an ER range of 0.15–0.2. Increased biomass moisture content (2 %–25 %) reduced CH<sub>4</sub> concentration from 4.08 % to 2.95 %, lowering the overall BGG calorific value. Air temperature exhibited negligible impacts on gasification performance. Implementation of these findings in industrial biomass gasifiers validated the optimized parameters of the model can accurately predict and guide actual experiments, with <20 % deviation in BGG composition under optimized conditions.</div></div>","PeriodicalId":253,"journal":{"name":"Biomass & Bioenergy","volume":"204 ","pages":"Article 108403"},"PeriodicalIF":5.8000,"publicationDate":"2025-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Modeling of industrial biomass fluidized bed gasification system and optimization of operating conditions\",\"authors\":\"Haodong Fan , Han Zhang , Geng Li , Xiong Zhang , Zixue Luo , Lin Huang , Shihong Zhang\",\"doi\":\"10.1016/j.biombioe.2025.108403\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Carbon emissions from fossil fuel combustion have emerged as a critical constraint on sustainable industrial development. Biomass gasification gas (BGG) represents a promising decarbonization pathway; however, the reliance on single-source biomass cannot ensure the operational reliability of industrial fluidized bed gasifiers. A key challenge to large-scale BGG adoption lies in the limited adaptability of fluidized bed reactors to different biomass, which exhibit heterogeneous physicochemical properties. Moreover, industrial research on the impact of structural parameters on gasification efficiency remains scarce. To investigate the impact of different biomass on gasification performance in fluidized-bed reactors, this study developed an industrial-scale fluidized-bed gasifier model using the Aspen Plus fluidized-bed module, based on an 8 t/h biomass gasifier operating in a regional facility. Key parameters, including equivalence ratio (ER), gasification pressure, and gasification temperature, were systematically evaluated to assess their effects on BGG composition and gasification efficiency. Furthermore, model validity was rigorously validated through computational and experimental data comparisons of critical design parameters. The results demonstrated that gasification temperature and ER are critical factors influencing biomass gasification efficiency. When the gasification temperature increased from 650 to 900 °C, the gas yield variation of corn stover and wooden blocks reached a maximum of 0.17 m<sup>3</sup>/kg. For corn stover gasification, the volumetric fractions of H<sub>2</sub>, CO, CO<sub>2</sub>, and CH<sub>4</sub> exhibited an increasing trend, rising by 11.43 %, 8.41 %, 7.73 %, and 2.24 %, respectively. Notably, biomass briquette gasification showed the most significant increase in H<sub>2</sub> fraction (11.4 %). Balancing operational safety and efficiency, the optimal gasification temperature was identified as 850 °C, with an ER range of 0.15–0.2. Increased biomass moisture content (2 %–25 %) reduced CH<sub>4</sub> concentration from 4.08 % to 2.95 %, lowering the overall BGG calorific value. Air temperature exhibited negligible impacts on gasification performance. Implementation of these findings in industrial biomass gasifiers validated the optimized parameters of the model can accurately predict and guide actual experiments, with <20 % deviation in BGG composition under optimized conditions.</div></div>\",\"PeriodicalId\":253,\"journal\":{\"name\":\"Biomass & Bioenergy\",\"volume\":\"204 \",\"pages\":\"Article 108403\"},\"PeriodicalIF\":5.8000,\"publicationDate\":\"2025-09-25\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Biomass & Bioenergy\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0961953425008141\",\"RegionNum\":2,\"RegionCategory\":\"生物学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"AGRICULTURAL ENGINEERING\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Biomass & Bioenergy","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0961953425008141","RegionNum":2,"RegionCategory":"生物学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"AGRICULTURAL ENGINEERING","Score":null,"Total":0}
Modeling of industrial biomass fluidized bed gasification system and optimization of operating conditions
Carbon emissions from fossil fuel combustion have emerged as a critical constraint on sustainable industrial development. Biomass gasification gas (BGG) represents a promising decarbonization pathway; however, the reliance on single-source biomass cannot ensure the operational reliability of industrial fluidized bed gasifiers. A key challenge to large-scale BGG adoption lies in the limited adaptability of fluidized bed reactors to different biomass, which exhibit heterogeneous physicochemical properties. Moreover, industrial research on the impact of structural parameters on gasification efficiency remains scarce. To investigate the impact of different biomass on gasification performance in fluidized-bed reactors, this study developed an industrial-scale fluidized-bed gasifier model using the Aspen Plus fluidized-bed module, based on an 8 t/h biomass gasifier operating in a regional facility. Key parameters, including equivalence ratio (ER), gasification pressure, and gasification temperature, were systematically evaluated to assess their effects on BGG composition and gasification efficiency. Furthermore, model validity was rigorously validated through computational and experimental data comparisons of critical design parameters. The results demonstrated that gasification temperature and ER are critical factors influencing biomass gasification efficiency. When the gasification temperature increased from 650 to 900 °C, the gas yield variation of corn stover and wooden blocks reached a maximum of 0.17 m3/kg. For corn stover gasification, the volumetric fractions of H2, CO, CO2, and CH4 exhibited an increasing trend, rising by 11.43 %, 8.41 %, 7.73 %, and 2.24 %, respectively. Notably, biomass briquette gasification showed the most significant increase in H2 fraction (11.4 %). Balancing operational safety and efficiency, the optimal gasification temperature was identified as 850 °C, with an ER range of 0.15–0.2. Increased biomass moisture content (2 %–25 %) reduced CH4 concentration from 4.08 % to 2.95 %, lowering the overall BGG calorific value. Air temperature exhibited negligible impacts on gasification performance. Implementation of these findings in industrial biomass gasifiers validated the optimized parameters of the model can accurately predict and guide actual experiments, with <20 % deviation in BGG composition under optimized conditions.
期刊介绍:
Biomass & Bioenergy is an international journal publishing original research papers and short communications, review articles and case studies on biological resources, chemical and biological processes, and biomass products for new renewable sources of energy and materials.
The scope of the journal extends to the environmental, management and economic aspects of biomass and bioenergy.
Key areas covered by the journal:
• Biomass: sources, energy crop production processes, genetic improvements, composition. Please note that research on these biomass subjects must be linked directly to bioenergy generation.
• Biological Residues: residues/rests from agricultural production, forestry and plantations (palm, sugar etc), processing industries, and municipal sources (MSW). Papers on the use of biomass residues through innovative processes/technological novelty and/or consideration of feedstock/system sustainability (or unsustainability) are welcomed. However waste treatment processes and pollution control or mitigation which are only tangentially related to bioenergy are not in the scope of the journal, as they are more suited to publications in the environmental arena. Papers that describe conventional waste streams (ie well described in existing literature) that do not empirically address ''new'' added value from the process are not suitable for submission to the journal.
• Bioenergy Processes: fermentations, thermochemical conversions, liquid and gaseous fuels, and petrochemical substitutes
• Bioenergy Utilization: direct combustion, gasification, electricity production, chemical processes, and by-product remediation
• Biomass and the Environment: carbon cycle, the net energy efficiency of bioenergy systems, assessment of sustainability, and biodiversity issues.