磁阻Mn2PdIn中费米表面嵌套与反常霍尔效应

IF 19 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Afsar Ahmed, Arnab Bhattacharya, Prashant Singh, Ajay Kumar, Tukai Singha, Anis Biswas, Yaroslav Mudryk, I. Das
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引用次数: 0

摘要

非共线磁体具有接近零的净磁化强度和非平凡的块状电子拓扑结构,在自旋电子应用中具有重要的前景,尽管它们的稀缺性需要深思熟虑的设计策略。在这项工作中,报告了金属Mn2PdIn的拓扑非平凡电子结构,其结晶为逆Heusler结构,并表现出具有淬火磁化的自旋玻璃基态。该系统在费米能级附近具有weyl型带交叉,并揭示了动量-空间嵌套、轨道杂化和自旋-轨道耦合之间的新相互作用。综合磁输运测量揭示了Mn2PdIn中明显的异常霍尔效应(AHE)。观察到的纵向霍尔电阻率和异常霍尔电阻率之间的二次关系突出了本征贝里曲率对AHE的贡献。这些发现确立了逆Heusler合金作为实现承载weyl型半金属或金属相的非共线磁体的引人注目的平台,结合了抑制磁化和强大的电子输运,从而为其无缝集成到下一代自旋电子器件提供了一条有希望的途径。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Fermi Surface Nesting and Anomalous Hall Effect in Magnetically Frustrated Mn2PdIn

Fermi Surface Nesting and Anomalous Hall Effect in Magnetically Frustrated Mn2PdIn
Noncollinear magnets with near-zero net magnetization and nontrivial bulk electronic topology hold significant promise for spintronic applications, though their scarcity necessitates deliberate design strategies. In this work, a topologically nontrivial electronic structure is reported in metallic Mn2PdIn, which crystallizes in the inverse Heusler structure and exhibits a spin-glassy ground state with quenched magnetization. The system features Weyl-type band crossings near the Fermi level and reveals a novel interplay among momentum-space nesting, orbital hybridization, and spin-orbit coupling. Comprehensive magnetotransport measurements reveal a pronounced anomalous Hall effect (AHE) in Mn2PdIn. The observed quadratic relationship between the longitudinal and anomalous Hall resistivities highlights the dominance of the intrinsic Berry curvature contribution to the AHE. These findings establish inverse Heusler alloys as compelling platforms for realizing noncollinear magnets that host Weyl-type semimetallic or metallic phases-combining suppressed magnetization with robust electronic transport-thereby offering a promising route toward their seamless integration into next-generation spintronic devices.
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来源期刊
Advanced Functional Materials
Advanced Functional Materials 工程技术-材料科学:综合
CiteScore
29.50
自引率
4.20%
发文量
2086
审稿时长
2.1 months
期刊介绍: Firmly established as a top-tier materials science journal, Advanced Functional Materials reports breakthrough research in all aspects of materials science, including nanotechnology, chemistry, physics, and biology every week. Advanced Functional Materials is known for its rapid and fair peer review, quality content, and high impact, making it the first choice of the international materials science community.
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