{"title":"反向多元校准作为非加性吸光度混合光谱中相似分析物的分离测定仪器","authors":"I. V. Vlasova, A. A. Matusevich, V. I. Vershinin","doi":"10.1134/S1061934825700248","DOIUrl":null,"url":null,"abstract":"<p>Multivariate calibrations are used in spectrophotometric analysis to determine multiple analytes in multicomponent solutions. These calibrations relate generalized signals measured at multiple wavelengths with concentrations of the analytes. The aim of this study was to assess the applicability of inverted multivariate calibrations (IMCs) for the separate determination of similar analytes under conditions of nonadditive absorbance. The test samples were model aqueous solutions simultaneously containing Cu(II), Co(II), Ni(II), Zn(II), and Pb(II) along with an excess of the photometric reagent 4-(2-pyridylazo)resorcinol. In these solutions, statistically significant deviations from additive absorbance were observed, likely due to a shift in the complexation equilibrium. The input data for constructing the IMC were the spectra of model mixtures from the training set. The number of analytical wavelengths (<i>m</i>) and the number of mixtures in the training set (<i>n</i>) were varied during the experiment. The metal concentrations in the mixtures of the test set were calculated individually by multiple linear regression, using different spectral regions and different IMCs. The best results were obtained with <i>m</i> = 16 and <i>n</i> = 30. The determination errors for Co, Ni, and Zn in single mixtures did not exceed 25 rel % (in modulo), while the generalized errors (RMSEP) were 10–15 rel %. The determination errors for copper and lead were significantly higher. The experiment demonstrated that IMCs allow to determine the separate components of mixtures with similar but nonadditive spectra. However, the amount of the input data required must be significantly larger than in assessing the total amount of the same analytes, the accuracy of the results will be lower, and the correct determination of all analytes cannot be guaranteed.</p>","PeriodicalId":606,"journal":{"name":"Journal of Analytical Chemistry","volume":"80 5","pages":"856 - 863"},"PeriodicalIF":1.1000,"publicationDate":"2025-06-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Inverted Multivariate Calibrations as an Instrument for the Separate Determination of Similar Analytes from a Mixture Spectrum with Non-Additive Absorbance\",\"authors\":\"I. V. Vlasova, A. A. Matusevich, V. I. Vershinin\",\"doi\":\"10.1134/S1061934825700248\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Multivariate calibrations are used in spectrophotometric analysis to determine multiple analytes in multicomponent solutions. These calibrations relate generalized signals measured at multiple wavelengths with concentrations of the analytes. The aim of this study was to assess the applicability of inverted multivariate calibrations (IMCs) for the separate determination of similar analytes under conditions of nonadditive absorbance. The test samples were model aqueous solutions simultaneously containing Cu(II), Co(II), Ni(II), Zn(II), and Pb(II) along with an excess of the photometric reagent 4-(2-pyridylazo)resorcinol. In these solutions, statistically significant deviations from additive absorbance were observed, likely due to a shift in the complexation equilibrium. The input data for constructing the IMC were the spectra of model mixtures from the training set. The number of analytical wavelengths (<i>m</i>) and the number of mixtures in the training set (<i>n</i>) were varied during the experiment. The metal concentrations in the mixtures of the test set were calculated individually by multiple linear regression, using different spectral regions and different IMCs. The best results were obtained with <i>m</i> = 16 and <i>n</i> = 30. The determination errors for Co, Ni, and Zn in single mixtures did not exceed 25 rel % (in modulo), while the generalized errors (RMSEP) were 10–15 rel %. The determination errors for copper and lead were significantly higher. The experiment demonstrated that IMCs allow to determine the separate components of mixtures with similar but nonadditive spectra. 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引用次数: 0
摘要
多元校准用于分光光度分析,以确定多组分溶液中的多种分析物。这些校准将在多个波长下测量的广义信号与分析物的浓度联系起来。本研究的目的是评估倒置多元校准(IMCs)在非加性吸光度条件下对类似分析物单独测定的适用性。测试样品是同时含有Cu(II), Co(II), Ni(II), Zn(II)和Pb(II)的模型水溶液,以及过量的光度试剂4-(2-吡啶偶氮)间二酚。在这些溶液中,观察到统计学上显著的加法吸光度偏差,可能是由于络合平衡的变化。构建IMC的输入数据是来自训练集的模型混合谱。在实验过程中,分析波长的个数(m)和训练集中的混合物的个数(n)是不同的。采用多元线性回归方法,利用不同的光谱区域和不同的imc分别计算了试验集混合物中的金属浓度。当m = 16, n = 30时效果最佳。单一混合物中Co、Ni和Zn的测定误差不超过25雷尔%(模),而广义误差(RMSEP)为10-15雷尔%。铜和铅的测定误差明显较高。实验表明,IMCs可以确定具有相似但非加性光谱的混合物的单独组分。但是,所需的输入数据量必须明显大于评估相同分析物的总量,结果的准确性会降低,并且不能保证对所有分析物的正确测定。
Inverted Multivariate Calibrations as an Instrument for the Separate Determination of Similar Analytes from a Mixture Spectrum with Non-Additive Absorbance
Multivariate calibrations are used in spectrophotometric analysis to determine multiple analytes in multicomponent solutions. These calibrations relate generalized signals measured at multiple wavelengths with concentrations of the analytes. The aim of this study was to assess the applicability of inverted multivariate calibrations (IMCs) for the separate determination of similar analytes under conditions of nonadditive absorbance. The test samples were model aqueous solutions simultaneously containing Cu(II), Co(II), Ni(II), Zn(II), and Pb(II) along with an excess of the photometric reagent 4-(2-pyridylazo)resorcinol. In these solutions, statistically significant deviations from additive absorbance were observed, likely due to a shift in the complexation equilibrium. The input data for constructing the IMC were the spectra of model mixtures from the training set. The number of analytical wavelengths (m) and the number of mixtures in the training set (n) were varied during the experiment. The metal concentrations in the mixtures of the test set were calculated individually by multiple linear regression, using different spectral regions and different IMCs. The best results were obtained with m = 16 and n = 30. The determination errors for Co, Ni, and Zn in single mixtures did not exceed 25 rel % (in modulo), while the generalized errors (RMSEP) were 10–15 rel %. The determination errors for copper and lead were significantly higher. The experiment demonstrated that IMCs allow to determine the separate components of mixtures with similar but nonadditive spectra. However, the amount of the input data required must be significantly larger than in assessing the total amount of the same analytes, the accuracy of the results will be lower, and the correct determination of all analytes cannot be guaranteed.
期刊介绍:
The Journal of Analytical Chemistry is an international peer reviewed journal that covers theoretical and applied aspects of analytical chemistry; it informs the reader about new achievements in analytical methods, instruments and reagents. Ample space is devoted to problems arising in the analysis of vital media such as water and air. Consideration is given to the detection and determination of metal ions, anions, and various organic substances. The journal welcomes manuscripts from all countries in the English or Russian language.