基于硅纳米线的高性能紫外探测器,采用AuNPs/SnO2纳米结构

IF 3.3 3区 材料科学 Q3 CHEMISTRY, PHYSICAL
Silicon Pub Date : 2025-05-07 DOI:10.1007/s12633-025-03331-6
Pooja Singh, Avshish Kumar, Pramod Kumar, V. K. Jain
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引用次数: 0

摘要

在这项工作中,利用基于硅纳米线(SiNWs)的异质结开发了紫外(UV)光电探测器,以获得高性能器件。本文在硅片上的硅纳米线(SiNWs)上制备了金纳米粒子(AuNPs)、氧化锡纳米粒子(SnO2)异质结。采用共沉淀法和Turkevich法分别合成了SnO2 NPs和AuNPs。采用金属辅助化学蚀刻(MACE)技术制备了SiNWs。利用各种技术对制备的材料及其异质结结构进行了表征。在自供电模式下,测量到AuNPs/SnO2NPs@SiNWs异质结结构的光电流响应为60μA。该光电探测器在室温下具有45 mA/W的高响应率和0.25 × 1012 Jones的良好探测率。光电探测器还具有快速上升/衰减时间,分别为~ 60 ms和~ 110 ms。样品按一定的间隔连续检查三组开/关照明。该光电探测器的高性能可归因于等离子体AuNPs与SnO2 NPs的协同效应,其表现出增强的光捕获相互作用,从而最大限度地吸收紫外线辐射。因此,本工作的结果对具有独特功能的高效微型紫外光电探测器的发展具有很大的希望。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Silicon Nanowires Based High Performance Ultraviolet Photodetector Developed using AuNPs/SnO2 Nanostructure

In this work, ultraviolet (UV) photodetector was developed using silicon nanowire (SiNWs) based heterojunction to obtain a high-performance device. Here, a heterojunction was prepared using gold nanoparticles (AuNPs), tin oxide (SnO2) nanoparticles on silicon nanowires (SiNWs) on Si chip. The synthesis of SnO2 NPs and AuNPs was done using the co-precipitation and Turkevich methods, respectively. The SiNWs were developed by using metal assisted chemical etching (MACE) technique. The prepared materials and their heterojunction structures were characterized using various techniques. The photocurrent response of AuNPs/SnO2NPs@SiNWs heterojunction structure was measured to be 60μA under self-powered mode. The photodetector showed a high responsivity of 45 mA/W and good detectivity of 0.25 × 1012 Jones at room temperature. The photodetector also possesses a fast rise/decay time of ~ 60 ms and ~ 110 ms, respectively. The sample was checked continually for three ON/OFF sets of illumination at a regular interval. The high performance of the photodetector can be attributed due to the synergetic effect of plasmonic AuNPs with SnO2 NPs which shows an enhanced light trapping interactions, leading to maximum absorption of UV radiation. Thus, the results presented in this work hold great promise for the advancement of highly effective miniature UV photodetectors with unique features.

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来源期刊
Silicon
Silicon CHEMISTRY, PHYSICAL-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
5.90
自引率
20.60%
发文量
685
审稿时长
>12 weeks
期刊介绍: The journal Silicon is intended to serve all those involved in studying the role of silicon as an enabling element in materials science. There are no restrictions on disciplinary boundaries provided the focus is on silicon-based materials or adds significantly to the understanding of such materials. Accordingly, such contributions are welcome in the areas of inorganic and organic chemistry, physics, biology, engineering, nanoscience, environmental science, electronics and optoelectronics, and modeling and theory. Relevant silicon-based materials include, but are not limited to, semiconductors, polymers, composites, ceramics, glasses, coatings, resins, composites, small molecules, and thin films.
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