{"title":"低密度煤辅助下微波等离子体炬系统的CO2减排研究。","authors":"Yannick Kumona Balue, Hugues Nkomba Museba, Dzeyewir Divine Nyuyki, Bongju Lee","doi":"10.1080/09593330.2025.2560590","DOIUrl":null,"url":null,"abstract":"<p><p>Greenhouse gas emissions are abundantly produced every year by human activities. They are the main cause of global warming and the changes observed in the climate. In this study, we used the microwave plasma torch system (MPT) to drive the conversion of CO<sub>2</sub> through the Boudouard reaction pathway. The necessary microwave power applied has efficiently activated the coal used as a reductant agent to initiate the chemical decomposition of CO2. The specific energy consumption reached 94 kJ/mol to ensure the continuous decomposition process of carbon dioxide under microwave plasma torch technology at atmospheric pressure. Experimentally, the conversion rate of 20 lpm of CO<sub>2</sub> under the MPT developed in this research reached 64% at a moderate temperature of 680°C with a specific recipe composed of the operating conditions coupled to the geometry of the designed reactor. In addition, the numerical model built in Aspen Plus V12 supported the experimental results by producing similar patterns in the conversion of CO<sub>2</sub> as a function of microwave power. Thus, the entire process tends to be energy-saving and an efficient solution for greenhouse gas mitigation for a clean and sustainable environment.</p>","PeriodicalId":12009,"journal":{"name":"Environmental Technology","volume":" ","pages":"1-12"},"PeriodicalIF":2.0000,"publicationDate":"2025-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Abatement of CO2 under the microwave plasma torch system assisted with low-density coal.\",\"authors\":\"Yannick Kumona Balue, Hugues Nkomba Museba, Dzeyewir Divine Nyuyki, Bongju Lee\",\"doi\":\"10.1080/09593330.2025.2560590\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Greenhouse gas emissions are abundantly produced every year by human activities. They are the main cause of global warming and the changes observed in the climate. In this study, we used the microwave plasma torch system (MPT) to drive the conversion of CO<sub>2</sub> through the Boudouard reaction pathway. The necessary microwave power applied has efficiently activated the coal used as a reductant agent to initiate the chemical decomposition of CO2. The specific energy consumption reached 94 kJ/mol to ensure the continuous decomposition process of carbon dioxide under microwave plasma torch technology at atmospheric pressure. Experimentally, the conversion rate of 20 lpm of CO<sub>2</sub> under the MPT developed in this research reached 64% at a moderate temperature of 680°C with a specific recipe composed of the operating conditions coupled to the geometry of the designed reactor. In addition, the numerical model built in Aspen Plus V12 supported the experimental results by producing similar patterns in the conversion of CO<sub>2</sub> as a function of microwave power. Thus, the entire process tends to be energy-saving and an efficient solution for greenhouse gas mitigation for a clean and sustainable environment.</p>\",\"PeriodicalId\":12009,\"journal\":{\"name\":\"Environmental Technology\",\"volume\":\" \",\"pages\":\"1-12\"},\"PeriodicalIF\":2.0000,\"publicationDate\":\"2025-09-25\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Environmental Technology\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://doi.org/10.1080/09593330.2025.2560590\",\"RegionNum\":4,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ENVIRONMENTAL SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Environmental Technology","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.1080/09593330.2025.2560590","RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
引用次数: 0
摘要
人类活动每年产生大量的温室气体排放。它们是全球变暖和观测到的气候变化的主要原因。在这项研究中,我们使用微波等离子体炬系统(MPT)通过Boudouard反应途径驱动CO2的转化。必要的微波功率有效地激活了用作还原剂的煤,引发了二氧化碳的化学分解。比能耗达到94 kJ/mol,保证了微波等离子体炬技术在常压下对二氧化碳的连续分解过程。实验结果表明,本研究开发的MPT在680°C的中等温度下,20 lpm CO2的转化率达到64%,具体配方由操作条件与设计的反应器几何形状耦合而成。此外,在Aspen Plus V12中建立的数值模型通过产生与微波功率相似的CO2转换模式来支持实验结果。因此,整个过程往往是节能的,是减少温室气体的有效解决办法,以实现清洁和可持续的环境。
Abatement of CO2 under the microwave plasma torch system assisted with low-density coal.
Greenhouse gas emissions are abundantly produced every year by human activities. They are the main cause of global warming and the changes observed in the climate. In this study, we used the microwave plasma torch system (MPT) to drive the conversion of CO2 through the Boudouard reaction pathway. The necessary microwave power applied has efficiently activated the coal used as a reductant agent to initiate the chemical decomposition of CO2. The specific energy consumption reached 94 kJ/mol to ensure the continuous decomposition process of carbon dioxide under microwave plasma torch technology at atmospheric pressure. Experimentally, the conversion rate of 20 lpm of CO2 under the MPT developed in this research reached 64% at a moderate temperature of 680°C with a specific recipe composed of the operating conditions coupled to the geometry of the designed reactor. In addition, the numerical model built in Aspen Plus V12 supported the experimental results by producing similar patterns in the conversion of CO2 as a function of microwave power. Thus, the entire process tends to be energy-saving and an efficient solution for greenhouse gas mitigation for a clean and sustainable environment.
期刊介绍:
Environmental Technology is a leading journal for the rapid publication of science and technology papers on a wide range of topics in applied environmental studies, from environmental engineering to environmental biotechnology, the circular economy, municipal and industrial wastewater management, drinking-water treatment, air- and water-pollution control, solid-waste management, industrial hygiene and associated technologies.
Environmental Technology is intended to provide rapid publication of new developments in environmental technology. The journal has an international readership with a broad scientific base. Contributions will be accepted from scientists and engineers in industry, government and universities. Accepted manuscripts are generally published within four months.
Please note that Environmental Technology does not publish any review papers unless for a specified special issue which is decided by the Editor. Please do submit your review papers to our sister journal Environmental Technology Reviews at http://www.tandfonline.com/toc/tetr20/current