基于双环摩擦电纳米发电机的自供电饮用水UV/O3消毒系统

IF 5.5 2区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY
Ming Li, , , Tianyi Jiang*, , , Haoxiu Sun, , , Liangyu Cao, , , Shanguo Zhang, , , Wenlong Wu, , , Jiachao Tang, , , Yu Li, , and , Hongyuan Jiang, 
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引用次数: 0

摘要

饮用水安全是公共卫生的一个重要组成部分。然而,大多数消毒方法依赖于电网,限制了它们的应用前景。本工作提出了一种基于双环摩擦电纳米发电机(DR-TENG)的自供电组合(UV/O3)饮用水消毒系统,该系统由内环TENG (IR-TENG)和外环TENG (OR-TENG)组成。在OR-TENG回路中人工引入气隙,使紫外辐照度提高到31.63 μW/cm2,在300 rpm时显著提高消毒效率,达到12.02 mL/min。IR-TENG的瞬时电压超过31.24 kV, O3浓度为31.96 mg/m3,转速为500 rpm。因此,提出了一种UV/O3消毒方法,以提高在高浊度环境或大直径水反应器等紫外线辐照不足情况下的消毒性能。0.35 McFarland (MCF)溶液在60 mm直径的水反应器内,在300 rpm转速下,对大肠杆菌溶液的UV/O3消毒效率分别提高到4.43和17.23 mL/min。此外,由于O3的强氧化性,10ml浓度为5ppm的罗丹明B溶液在300 rpm转速下在15分钟内几乎完全被O3降解。为了扩展O3消毒系统的功能,在不干扰O3产生的情况下,将降压电路集成到电流回路中,为水质检测器供电。综上所述,本工作提供了一种具有高压直流输出的水消毒和teng策略。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

A Self-Powered UV/O3 Disinfection System for Drinking Water Based on a Double-Ring Triboelectric Nanogenerator

A Self-Powered UV/O3 Disinfection System for Drinking Water Based on a Double-Ring Triboelectric Nanogenerator

Drinking water security is a significant component of public health. However, the majority of disinfection methods depends on a power grid, restricting their application prospects. This work proposes a self-powered combined (UV/O3) disinfection system for drinking water based on a double-ring triboelectric nanogenerator (DR-TENG) consisting of an inner-ring TENG (IR-TENG) and an outer-ring TENG (OR-TENG). The artificially introduced air gap in the OR-TENG circuit increases the UV irradiance to 31.63 μW/cm2, significantly improving the disinfection efficiency to 12.02 mL/min at 300 rpm. For IR-TENG, an instant voltage of over 31.24 kV and an O3 concentration of 31.96 mg/m3 at 500 rpm were achieved. Consequently, a UV/O3 disinfection method is proposed to enhance the disinfection performance under insufficient UV irradiance such as in high-turbidity environments or large-diameter water reactors. The UV/O3 disinfection efficiency of E. coli solution with 0.35 McFarland (MCF) and within a 60 mm diameter water reactor is enhanced to 4.43 and 17.23 mL/min, respectively, at 300 rpm. Furthermore, 10 mL of Rhodamine B solution with a concentration of 5 ppm is almost completely degraded by O3 within 15 min at 300 rpm due to the strong oxidizing properties of O3. To expand the function of the O3 disinfection system, a buck circuit is integrated into the current loop without disturbing the generation of the O3 to power a water quality detector. In summary, this work provides a strategy for water disinfection and TENGs with high-voltage DC output.

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来源期刊
CiteScore
8.30
自引率
3.40%
发文量
1601
期刊介绍: ACS Applied Nano Materials is an interdisciplinary journal publishing original research covering all aspects of engineering, chemistry, physics and biology relevant to applications of nanomaterials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important applications of nanomaterials.
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