{"title":"基于双环摩擦电纳米发电机的自供电饮用水UV/O3消毒系统","authors":"Ming Li, , , Tianyi Jiang*, , , Haoxiu Sun, , , Liangyu Cao, , , Shanguo Zhang, , , Wenlong Wu, , , Jiachao Tang, , , Yu Li, , and , Hongyuan Jiang, ","doi":"10.1021/acsanm.5c03269","DOIUrl":null,"url":null,"abstract":"<p >Drinking water security is a significant component of public health. However, the majority of disinfection methods depends on a power grid, restricting their application prospects. This work proposes a self-powered combined (UV/O<sub>3</sub>) disinfection system for drinking water based on a double-ring triboelectric nanogenerator (DR-TENG) consisting of an inner-ring TENG (IR-TENG) and an outer-ring TENG (OR-TENG). The artificially introduced air gap in the OR-TENG circuit increases the UV irradiance to 31.63 μW/cm<sup>2</sup>, significantly improving the disinfection efficiency to 12.02 mL/min at 300 rpm. For IR-TENG, an instant voltage of over 31.24 kV and an O<sub>3</sub> concentration of 31.96 mg/m<sup>3</sup> at 500 rpm were achieved. Consequently, a UV/O<sub>3</sub> disinfection method is proposed to enhance the disinfection performance under insufficient UV irradiance such as in high-turbidity environments or large-diameter water reactors. The UV/O<sub>3</sub> disinfection efficiency of <i>E. coli</i> solution with 0.35 McFarland (MCF) and within a 60 mm diameter water reactor is enhanced to 4.43 and 17.23 mL/min, respectively, at 300 rpm. Furthermore, 10 mL of Rhodamine B solution with a concentration of 5 ppm is almost completely degraded by O<sub>3</sub> within 15 min at 300 rpm due to the strong oxidizing properties of O<sub>3</sub>. To expand the function of the O<sub>3</sub> disinfection system, a buck circuit is integrated into the current loop without disturbing the generation of the O<sub>3</sub> to power a water quality detector. In summary, this work provides a strategy for water disinfection and TENGs with high-voltage DC output.</p>","PeriodicalId":6,"journal":{"name":"ACS Applied Nano Materials","volume":"8 38","pages":"18487–18499"},"PeriodicalIF":5.5000,"publicationDate":"2025-09-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"A Self-Powered UV/O3 Disinfection System for Drinking Water Based on a Double-Ring Triboelectric Nanogenerator\",\"authors\":\"Ming Li, , , Tianyi Jiang*, , , Haoxiu Sun, , , Liangyu Cao, , , Shanguo Zhang, , , Wenlong Wu, , , Jiachao Tang, , , Yu Li, , and , Hongyuan Jiang, \",\"doi\":\"10.1021/acsanm.5c03269\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Drinking water security is a significant component of public health. However, the majority of disinfection methods depends on a power grid, restricting their application prospects. This work proposes a self-powered combined (UV/O<sub>3</sub>) disinfection system for drinking water based on a double-ring triboelectric nanogenerator (DR-TENG) consisting of an inner-ring TENG (IR-TENG) and an outer-ring TENG (OR-TENG). The artificially introduced air gap in the OR-TENG circuit increases the UV irradiance to 31.63 μW/cm<sup>2</sup>, significantly improving the disinfection efficiency to 12.02 mL/min at 300 rpm. For IR-TENG, an instant voltage of over 31.24 kV and an O<sub>3</sub> concentration of 31.96 mg/m<sup>3</sup> at 500 rpm were achieved. Consequently, a UV/O<sub>3</sub> disinfection method is proposed to enhance the disinfection performance under insufficient UV irradiance such as in high-turbidity environments or large-diameter water reactors. The UV/O<sub>3</sub> disinfection efficiency of <i>E. coli</i> solution with 0.35 McFarland (MCF) and within a 60 mm diameter water reactor is enhanced to 4.43 and 17.23 mL/min, respectively, at 300 rpm. Furthermore, 10 mL of Rhodamine B solution with a concentration of 5 ppm is almost completely degraded by O<sub>3</sub> within 15 min at 300 rpm due to the strong oxidizing properties of O<sub>3</sub>. To expand the function of the O<sub>3</sub> disinfection system, a buck circuit is integrated into the current loop without disturbing the generation of the O<sub>3</sub> to power a water quality detector. In summary, this work provides a strategy for water disinfection and TENGs with high-voltage DC output.</p>\",\"PeriodicalId\":6,\"journal\":{\"name\":\"ACS Applied Nano Materials\",\"volume\":\"8 38\",\"pages\":\"18487–18499\"},\"PeriodicalIF\":5.5000,\"publicationDate\":\"2025-09-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Nano Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsanm.5c03269\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Nano Materials","FirstCategoryId":"88","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsanm.5c03269","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
A Self-Powered UV/O3 Disinfection System for Drinking Water Based on a Double-Ring Triboelectric Nanogenerator
Drinking water security is a significant component of public health. However, the majority of disinfection methods depends on a power grid, restricting their application prospects. This work proposes a self-powered combined (UV/O3) disinfection system for drinking water based on a double-ring triboelectric nanogenerator (DR-TENG) consisting of an inner-ring TENG (IR-TENG) and an outer-ring TENG (OR-TENG). The artificially introduced air gap in the OR-TENG circuit increases the UV irradiance to 31.63 μW/cm2, significantly improving the disinfection efficiency to 12.02 mL/min at 300 rpm. For IR-TENG, an instant voltage of over 31.24 kV and an O3 concentration of 31.96 mg/m3 at 500 rpm were achieved. Consequently, a UV/O3 disinfection method is proposed to enhance the disinfection performance under insufficient UV irradiance such as in high-turbidity environments or large-diameter water reactors. The UV/O3 disinfection efficiency of E. coli solution with 0.35 McFarland (MCF) and within a 60 mm diameter water reactor is enhanced to 4.43 and 17.23 mL/min, respectively, at 300 rpm. Furthermore, 10 mL of Rhodamine B solution with a concentration of 5 ppm is almost completely degraded by O3 within 15 min at 300 rpm due to the strong oxidizing properties of O3. To expand the function of the O3 disinfection system, a buck circuit is integrated into the current loop without disturbing the generation of the O3 to power a water quality detector. In summary, this work provides a strategy for water disinfection and TENGs with high-voltage DC output.
期刊介绍:
ACS Applied Nano Materials is an interdisciplinary journal publishing original research covering all aspects of engineering, chemistry, physics and biology relevant to applications of nanomaterials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important applications of nanomaterials.