Patrick Franke, Markus Schubert, Uwe Hampel, Eugeny Y. Kenig
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A rate-based model for reactive separation columns with sandwich packings
Sandwich packings are assembled from two conventional structured packings with different geometrical surface areas stacked alternatingly within a separation column. When operated under partially flooded conditions, they provide significant mass transfer improvement compared to common structured packings. In this work, a rate-based model including novel mass transfer correlations is presented and validated using a comprehensive experimental database for the reactive absorption of CO2 into aqueous monoethanolamine. The proposed rate-based approach is capable of accounting for axial dispersion, thereby enabling the evaluation of the effect of liquid-phase backmixing on the mass transfer performance. The validated rate-based model is used to evaluate the separation performance of sandwich packings. Compared with structured packings, up to 10 % higher mass transfer rates are obtained.
期刊介绍:
Chemical engineering enables the transformation of natural resources and energy into useful products for society. It draws on and applies natural sciences, mathematics and economics, and has developed fundamental engineering science that underpins the discipline.
Chemical Engineering Science (CES) has been publishing papers on the fundamentals of chemical engineering since 1951. CES is the platform where the most significant advances in the discipline have ever since been published. Chemical Engineering Science has accompanied and sustained chemical engineering through its development into the vibrant and broad scientific discipline it is today.