Zehui Shang , Yinan Liu , Chunying Zhu , Taotao Fu , Xiqun Gao , Youguang Ma
{"title":"y型微通道中无阻碍水包水滴破裂动力学","authors":"Zehui Shang , Yinan Liu , Chunying Zhu , Taotao Fu , Xiqun Gao , Youguang Ma","doi":"10.1016/j.ces.2025.122677","DOIUrl":null,"url":null,"abstract":"<div><div>The breakup of water-in-water droplets in a Y-junction microchannel was experimentally investigated, focusing on the unobstructed breakup mode due to its broad applicability. This process was divided into four stages: entering, squeezing, pinch-off, and filament rupture, based on the evolution of the neck width and its thinning rate. In the entering stage, neck thinning accelerates with increasing dispersed-phase flow rate <em>Q</em><sub>d</sub>, droplet length <em>l</em><sub>0</sub>, and two-phase viscosity ratio <em>λ</em>, and slows down with increasing continuous-phase flow rate <em>Q</em><sub>c</sub>. In the squeezing stage, the minimum neck width follows a power-law relation with time. The thinning rate increases with higher <em>Q</em><sub>d</sub>, <em>l</em><sub>0</sub>, and <em>λ</em>, whereas increasing <em>Q</em><sub>c</sub> inhibits thinning. In the pinch-off stage, neck width decreases linearly with time, and the thinning is enhanced by higher <em>Q</em><sub>c</sub>, <em>Q</em><sub>d</sub>, and <em>l</em><sub>0</sub>, but remains nearly independent of <em>λ</em>. The filament rupture stage follows a power-law thinning trend, and exhibits similar parameter dependencies, though satellite droplets may form at high <em>Q</em><sub>d</sub> and <em>Q</em><sub>c</sub>, and show increased instability at low viscosity. These findings offer insights into neck dynamics and interfacial rupture in low interfacial tension systems.</div></div>","PeriodicalId":271,"journal":{"name":"Chemical Engineering Science","volume":"320 ","pages":"Article 122677"},"PeriodicalIF":4.3000,"publicationDate":"2025-09-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Breakup kinetics of water-in-water droplets without obstruction in Y-shaped microchannel\",\"authors\":\"Zehui Shang , Yinan Liu , Chunying Zhu , Taotao Fu , Xiqun Gao , Youguang Ma\",\"doi\":\"10.1016/j.ces.2025.122677\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The breakup of water-in-water droplets in a Y-junction microchannel was experimentally investigated, focusing on the unobstructed breakup mode due to its broad applicability. This process was divided into four stages: entering, squeezing, pinch-off, and filament rupture, based on the evolution of the neck width and its thinning rate. In the entering stage, neck thinning accelerates with increasing dispersed-phase flow rate <em>Q</em><sub>d</sub>, droplet length <em>l</em><sub>0</sub>, and two-phase viscosity ratio <em>λ</em>, and slows down with increasing continuous-phase flow rate <em>Q</em><sub>c</sub>. In the squeezing stage, the minimum neck width follows a power-law relation with time. The thinning rate increases with higher <em>Q</em><sub>d</sub>, <em>l</em><sub>0</sub>, and <em>λ</em>, whereas increasing <em>Q</em><sub>c</sub> inhibits thinning. In the pinch-off stage, neck width decreases linearly with time, and the thinning is enhanced by higher <em>Q</em><sub>c</sub>, <em>Q</em><sub>d</sub>, and <em>l</em><sub>0</sub>, but remains nearly independent of <em>λ</em>. The filament rupture stage follows a power-law thinning trend, and exhibits similar parameter dependencies, though satellite droplets may form at high <em>Q</em><sub>d</sub> and <em>Q</em><sub>c</sub>, and show increased instability at low viscosity. These findings offer insights into neck dynamics and interfacial rupture in low interfacial tension systems.</div></div>\",\"PeriodicalId\":271,\"journal\":{\"name\":\"Chemical Engineering Science\",\"volume\":\"320 \",\"pages\":\"Article 122677\"},\"PeriodicalIF\":4.3000,\"publicationDate\":\"2025-09-23\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemical Engineering Science\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0009250925014988\",\"RegionNum\":2,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Engineering Science","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0009250925014988","RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
Breakup kinetics of water-in-water droplets without obstruction in Y-shaped microchannel
The breakup of water-in-water droplets in a Y-junction microchannel was experimentally investigated, focusing on the unobstructed breakup mode due to its broad applicability. This process was divided into four stages: entering, squeezing, pinch-off, and filament rupture, based on the evolution of the neck width and its thinning rate. In the entering stage, neck thinning accelerates with increasing dispersed-phase flow rate Qd, droplet length l0, and two-phase viscosity ratio λ, and slows down with increasing continuous-phase flow rate Qc. In the squeezing stage, the minimum neck width follows a power-law relation with time. The thinning rate increases with higher Qd, l0, and λ, whereas increasing Qc inhibits thinning. In the pinch-off stage, neck width decreases linearly with time, and the thinning is enhanced by higher Qc, Qd, and l0, but remains nearly independent of λ. The filament rupture stage follows a power-law thinning trend, and exhibits similar parameter dependencies, though satellite droplets may form at high Qd and Qc, and show increased instability at low viscosity. These findings offer insights into neck dynamics and interfacial rupture in low interfacial tension systems.
期刊介绍:
Chemical engineering enables the transformation of natural resources and energy into useful products for society. It draws on and applies natural sciences, mathematics and economics, and has developed fundamental engineering science that underpins the discipline.
Chemical Engineering Science (CES) has been publishing papers on the fundamentals of chemical engineering since 1951. CES is the platform where the most significant advances in the discipline have ever since been published. Chemical Engineering Science has accompanied and sustained chemical engineering through its development into the vibrant and broad scientific discipline it is today.