{"title":"多相熔岩的粘度:综合实验室和现场测量的新见解","authors":"M.A. Harris , S. Kolzenburg , M.O. Chevrel","doi":"10.1016/j.epsl.2025.119642","DOIUrl":null,"url":null,"abstract":"<div><div>Laboratory measurements on remelted rocks are the standard technique for characterizing the rheology of lava at eruptive temperatures. This approach enables precise measurements but struggles to recreate natural emplacement conditions. Particularly, lavas erupt as multiphase suspensions (melt + crystals + bubbles), but current laboratory methods cannot retain bubbles, and experiments are limited to two-phase (melt+crystals) suspensions. The oxygen fugacity of lavas is known to influence the kinetics of crystallization, and despite its importance, few studies have considered this factor to date. The only available technique to measure the three-phase viscosity of natural lava is through <em>in-situ</em> measurements while it is flowing. Here, we present the first study that integrates viscosity data from laboratory-derived single (melt) and two-phase (melt+crystals) measurements with data from three-phase (melt + crystals + bubbles) field measurements, using the 2023 Litli-Hrútur eruption in Iceland as a case study. We present a rheological characterization of the remelted lava during crystallization at thermomechanical equilibrium and disequilibrium at log <em>f</em>O<sub>2</sub> = −8.7, and deformation rates of 3.3 s<sup>-1</sup>. These bubble-free laboratory experiments were designed to overlap with field temperatures (1150–1165 °C), enabling direct comparison with the <em>in-situ</em> three-phase field viscosities. We find laboratory and field data overlap in viscosity space (10<sup>2.5</sup> to 10<sup>4.5</sup> Pa s) and at cooling rates of 0.5–1 °C/min. Isothermal experiments successfully recreate crystal phases and volumes comparable to natural samples (∼20–50 vol.% crystals). 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Particularly, lavas erupt as multiphase suspensions (melt + crystals + bubbles), but current laboratory methods cannot retain bubbles, and experiments are limited to two-phase (melt+crystals) suspensions. The oxygen fugacity of lavas is known to influence the kinetics of crystallization, and despite its importance, few studies have considered this factor to date. The only available technique to measure the three-phase viscosity of natural lava is through <em>in-situ</em> measurements while it is flowing. Here, we present the first study that integrates viscosity data from laboratory-derived single (melt) and two-phase (melt+crystals) measurements with data from three-phase (melt + crystals + bubbles) field measurements, using the 2023 Litli-Hrútur eruption in Iceland as a case study. We present a rheological characterization of the remelted lava during crystallization at thermomechanical equilibrium and disequilibrium at log <em>f</em>O<sub>2</sub> = −8.7, and deformation rates of 3.3 s<sup>-1</sup>. These bubble-free laboratory experiments were designed to overlap with field temperatures (1150–1165 °C), enabling direct comparison with the <em>in-situ</em> three-phase field viscosities. We find laboratory and field data overlap in viscosity space (10<sup>2.5</sup> to 10<sup>4.5</sup> Pa s) and at cooling rates of 0.5–1 °C/min. Isothermal experiments successfully recreate crystal phases and volumes comparable to natural samples (∼20–50 vol.% crystals). 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引用次数: 0
摘要
对重熔岩石的实验室测量是描述喷发温度下熔岩流变性的标准技术。这种方法可以实现精确的测量,但很难重现自然就位条件。特别是,熔岩以多相悬浮液(熔体+晶体+气泡)的形式喷发,但目前的实验室方法无法保留气泡,而且实验仅限于两相(熔体+晶体)悬浮液。众所周知,熔岩的氧逸度会影响结晶动力学,尽管它很重要,但迄今为止很少有研究考虑到这一因素。唯一可用的技术来测量天然熔岩的三相粘度是通过现场测量,而它是流动的。在这里,我们提出了第一个将实验室获得的单(熔体)和两相(熔体+晶体)测量数据与三相(熔体+晶体+气泡)现场测量数据相结合的研究,并以2023年Litli-Hrútur冰岛火山喷发为例进行了研究。本文研究了重熔熔岩结晶过程的流变学特征,在log fO2 =−8.7、变形速率为3.3 s-1时处于热力平衡和非平衡状态。这些无气泡的实验室实验与现场温度(1150-1165°C)重叠,可以直接与现场三相场粘度进行比较。我们发现实验室和现场数据在粘度空间(102.5至104.5 Pa s)和冷却速度为0.5-1°C/min时重叠。等温实验成功地重建了与天然样品(~ 20-50体积%晶体)相当的晶体相和体积。这一比较使得对天然熔岩有效粘度的实验室测量的首次现场验证成为可能。
The viscosity of multiphase lava: New insights from integrating laboratory and field measurements
Laboratory measurements on remelted rocks are the standard technique for characterizing the rheology of lava at eruptive temperatures. This approach enables precise measurements but struggles to recreate natural emplacement conditions. Particularly, lavas erupt as multiphase suspensions (melt + crystals + bubbles), but current laboratory methods cannot retain bubbles, and experiments are limited to two-phase (melt+crystals) suspensions. The oxygen fugacity of lavas is known to influence the kinetics of crystallization, and despite its importance, few studies have considered this factor to date. The only available technique to measure the three-phase viscosity of natural lava is through in-situ measurements while it is flowing. Here, we present the first study that integrates viscosity data from laboratory-derived single (melt) and two-phase (melt+crystals) measurements with data from three-phase (melt + crystals + bubbles) field measurements, using the 2023 Litli-Hrútur eruption in Iceland as a case study. We present a rheological characterization of the remelted lava during crystallization at thermomechanical equilibrium and disequilibrium at log fO2 = −8.7, and deformation rates of 3.3 s-1. These bubble-free laboratory experiments were designed to overlap with field temperatures (1150–1165 °C), enabling direct comparison with the in-situ three-phase field viscosities. We find laboratory and field data overlap in viscosity space (102.5 to 104.5 Pa s) and at cooling rates of 0.5–1 °C/min. Isothermal experiments successfully recreate crystal phases and volumes comparable to natural samples (∼20–50 vol.% crystals). This comparison allows the first field validation for laboratory measurements of the effective viscosity of natural lava.
期刊介绍:
Earth and Planetary Science Letters (EPSL) is a leading journal for researchers across the entire Earth and planetary sciences community. It publishes concise, exciting, high-impact articles ("Letters") of broad interest. Its focus is on physical and chemical processes, the evolution and general properties of the Earth and planets - from their deep interiors to their atmospheres. EPSL also includes a Frontiers section, featuring invited high-profile synthesis articles by leading experts on timely topics to bring cutting-edge research to the wider community.