Jiaxin Liu , Mengshuai Chen , Rachid Bennacer , Lin Chen
{"title":"多孔切屑内超临界CO2流动的可视化实验与数值分析:传热与多孔结构的影响","authors":"Jiaxin Liu , Mengshuai Chen , Rachid Bennacer , Lin Chen","doi":"10.1016/j.supflu.2025.106788","DOIUrl":null,"url":null,"abstract":"<div><div>Carbon dioxide (CO<sub>2</sub>) geological sequestration is one of the key methods to reduce atmospheric carbon emissions, yet the migration mechanisms of CO₂ within reservoirs remain unclear. This study systematically investigates the flow and heat transfer characteristics of supercritical CO₂ (sCO₂) in porous media through integrated optical visualization experiments and numerical simulations. Experimental results show that under supercritical conditions (pressure: 8.2–8.6 MPa, temperature: 32–34 °C), increasing the outlet pressure enhances momentum exchange but reduces flow uniformity, whereas raising the inlet temperature reduces fluid viscosity and smoothens density gradients, thereby improving flow homogeneity. Numerical simulations further reveal that under supercritical conditions (8.5 MPa, 305.15–318.15 K), boundary parameters including the inlet Reynolds number, inlet temperature, and wall heat flux exhibit non-monotonic influence patterns on the heat transfer coefficient (HTC), with an optimal range identified for each parameter. Exceeding this range leads to a significant reduction in HTC by 75–94 %. Under transcritical conditions (7.5–9.0 MPa, 303.15 K), the structure of the porous media effectively suppresses disturbances caused by thermophysical nonlinearities of sCO₂ through flow inertia, enabling the local heat transfer coefficient to maintain strong robustness against variations in outlet pressure and heat flux.</div></div>","PeriodicalId":17078,"journal":{"name":"Journal of Supercritical Fluids","volume":"228 ","pages":"Article 106788"},"PeriodicalIF":4.4000,"publicationDate":"2025-09-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Visualization experiment and numerical analysis of supercritical CO2 flow inside porous chip: Effect of heat transfer and porous structures\",\"authors\":\"Jiaxin Liu , Mengshuai Chen , Rachid Bennacer , Lin Chen\",\"doi\":\"10.1016/j.supflu.2025.106788\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Carbon dioxide (CO<sub>2</sub>) geological sequestration is one of the key methods to reduce atmospheric carbon emissions, yet the migration mechanisms of CO₂ within reservoirs remain unclear. This study systematically investigates the flow and heat transfer characteristics of supercritical CO₂ (sCO₂) in porous media through integrated optical visualization experiments and numerical simulations. Experimental results show that under supercritical conditions (pressure: 8.2–8.6 MPa, temperature: 32–34 °C), increasing the outlet pressure enhances momentum exchange but reduces flow uniformity, whereas raising the inlet temperature reduces fluid viscosity and smoothens density gradients, thereby improving flow homogeneity. Numerical simulations further reveal that under supercritical conditions (8.5 MPa, 305.15–318.15 K), boundary parameters including the inlet Reynolds number, inlet temperature, and wall heat flux exhibit non-monotonic influence patterns on the heat transfer coefficient (HTC), with an optimal range identified for each parameter. Exceeding this range leads to a significant reduction in HTC by 75–94 %. Under transcritical conditions (7.5–9.0 MPa, 303.15 K), the structure of the porous media effectively suppresses disturbances caused by thermophysical nonlinearities of sCO₂ through flow inertia, enabling the local heat transfer coefficient to maintain strong robustness against variations in outlet pressure and heat flux.</div></div>\",\"PeriodicalId\":17078,\"journal\":{\"name\":\"Journal of Supercritical Fluids\",\"volume\":\"228 \",\"pages\":\"Article 106788\"},\"PeriodicalIF\":4.4000,\"publicationDate\":\"2025-09-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Supercritical Fluids\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S089684462500275X\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Supercritical Fluids","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S089684462500275X","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Visualization experiment and numerical analysis of supercritical CO2 flow inside porous chip: Effect of heat transfer and porous structures
Carbon dioxide (CO2) geological sequestration is one of the key methods to reduce atmospheric carbon emissions, yet the migration mechanisms of CO₂ within reservoirs remain unclear. This study systematically investigates the flow and heat transfer characteristics of supercritical CO₂ (sCO₂) in porous media through integrated optical visualization experiments and numerical simulations. Experimental results show that under supercritical conditions (pressure: 8.2–8.6 MPa, temperature: 32–34 °C), increasing the outlet pressure enhances momentum exchange but reduces flow uniformity, whereas raising the inlet temperature reduces fluid viscosity and smoothens density gradients, thereby improving flow homogeneity. Numerical simulations further reveal that under supercritical conditions (8.5 MPa, 305.15–318.15 K), boundary parameters including the inlet Reynolds number, inlet temperature, and wall heat flux exhibit non-monotonic influence patterns on the heat transfer coefficient (HTC), with an optimal range identified for each parameter. Exceeding this range leads to a significant reduction in HTC by 75–94 %. Under transcritical conditions (7.5–9.0 MPa, 303.15 K), the structure of the porous media effectively suppresses disturbances caused by thermophysical nonlinearities of sCO₂ through flow inertia, enabling the local heat transfer coefficient to maintain strong robustness against variations in outlet pressure and heat flux.
期刊介绍:
The Journal of Supercritical Fluids is an international journal devoted to the fundamental and applied aspects of supercritical fluids and processes. Its aim is to provide a focused platform for academic and industrial researchers to report their findings and to have ready access to the advances in this rapidly growing field. Its coverage is multidisciplinary and includes both basic and applied topics.
Thermodynamics and phase equilibria, reaction kinetics and rate processes, thermal and transport properties, and all topics related to processing such as separations (extraction, fractionation, purification, chromatography) nucleation and impregnation are within the scope. Accounts of specific engineering applications such as those encountered in food, fuel, natural products, minerals, pharmaceuticals and polymer industries are included. Topics related to high pressure equipment design, analytical techniques, sensors, and process control methodologies are also within the scope of the journal.