{"title":"利用金纳米金字塔增强超薄倒置钙钛矿太阳能电池性能:光学和电学模拟研究","authors":"Danping Zhang, Chuyuan Yang","doi":"10.1007/s11468-025-02771-5","DOIUrl":null,"url":null,"abstract":"<div><p>In recent years, the development of ultra-thin perovskite solar cells has attracted attention due to their potential for producing flexible and less toxic solar cells. However, the use of perovskite thin films results in lower efficiency due to inadequate light harvesting. This paper proposes and numerically investigates the incorporation of Au nanopyramids within the 200 nm thick perovskite layer of inverted perovskite solar cells to enhance light harvesting. The effects of the size and periodicity of the nanopyramids on light absorption in the active layer are examined to achieve optimum cell performance. The mechanisms behind the improvement in absorption are analyzed through Mie resonance and near-field distribution. The optimized Au nanopyramids embedded in the perovskite layer led to a 19.48% increase in perovskite layer absorption. Additionally, devices based on Cu, Al, and Ag are studied to investigate the significance of the materials used in the plasmonic structures. The effects of Au nanopyramids in solar cells with perovskite layer thicknesses of 100 nm and 300 nm are also examined. Electrical analysis is performed on all optimized structures, and photovoltaic parameters are extracted. The findings of our research facilitate the design of high-performance, ultra-thin, and stable perovskite solar cells.</p></div>","PeriodicalId":736,"journal":{"name":"Plasmonics","volume":"20 9","pages":"7369 - 7379"},"PeriodicalIF":4.3000,"publicationDate":"2025-01-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Enhancement of Ultra-Thin Inverted Perovskite Solar Cell Performance Using Au Nanopyramids: An Optical and Electrical Simulation Study\",\"authors\":\"Danping Zhang, Chuyuan Yang\",\"doi\":\"10.1007/s11468-025-02771-5\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>In recent years, the development of ultra-thin perovskite solar cells has attracted attention due to their potential for producing flexible and less toxic solar cells. However, the use of perovskite thin films results in lower efficiency due to inadequate light harvesting. This paper proposes and numerically investigates the incorporation of Au nanopyramids within the 200 nm thick perovskite layer of inverted perovskite solar cells to enhance light harvesting. The effects of the size and periodicity of the nanopyramids on light absorption in the active layer are examined to achieve optimum cell performance. The mechanisms behind the improvement in absorption are analyzed through Mie resonance and near-field distribution. The optimized Au nanopyramids embedded in the perovskite layer led to a 19.48% increase in perovskite layer absorption. Additionally, devices based on Cu, Al, and Ag are studied to investigate the significance of the materials used in the plasmonic structures. The effects of Au nanopyramids in solar cells with perovskite layer thicknesses of 100 nm and 300 nm are also examined. Electrical analysis is performed on all optimized structures, and photovoltaic parameters are extracted. The findings of our research facilitate the design of high-performance, ultra-thin, and stable perovskite solar cells.</p></div>\",\"PeriodicalId\":736,\"journal\":{\"name\":\"Plasmonics\",\"volume\":\"20 9\",\"pages\":\"7369 - 7379\"},\"PeriodicalIF\":4.3000,\"publicationDate\":\"2025-01-31\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Plasmonics\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s11468-025-02771-5\",\"RegionNum\":4,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Plasmonics","FirstCategoryId":"101","ListUrlMain":"https://link.springer.com/article/10.1007/s11468-025-02771-5","RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Enhancement of Ultra-Thin Inverted Perovskite Solar Cell Performance Using Au Nanopyramids: An Optical and Electrical Simulation Study
In recent years, the development of ultra-thin perovskite solar cells has attracted attention due to their potential for producing flexible and less toxic solar cells. However, the use of perovskite thin films results in lower efficiency due to inadequate light harvesting. This paper proposes and numerically investigates the incorporation of Au nanopyramids within the 200 nm thick perovskite layer of inverted perovskite solar cells to enhance light harvesting. The effects of the size and periodicity of the nanopyramids on light absorption in the active layer are examined to achieve optimum cell performance. The mechanisms behind the improvement in absorption are analyzed through Mie resonance and near-field distribution. The optimized Au nanopyramids embedded in the perovskite layer led to a 19.48% increase in perovskite layer absorption. Additionally, devices based on Cu, Al, and Ag are studied to investigate the significance of the materials used in the plasmonic structures. The effects of Au nanopyramids in solar cells with perovskite layer thicknesses of 100 nm and 300 nm are also examined. Electrical analysis is performed on all optimized structures, and photovoltaic parameters are extracted. The findings of our research facilitate the design of high-performance, ultra-thin, and stable perovskite solar cells.
期刊介绍:
Plasmonics is an international forum for the publication of peer-reviewed leading-edge original articles that both advance and report our knowledge base and practice of the interactions of free-metal electrons, Plasmons.
Topics covered include notable advances in the theory, Physics, and applications of surface plasmons in metals, to the rapidly emerging areas of nanotechnology, biophotonics, sensing, biochemistry and medicine. Topics, including the theory, synthesis and optical properties of noble metal nanostructures, patterned surfaces or materials, continuous or grated surfaces, devices, or wires for their multifarious applications are particularly welcome. Typical applications might include but are not limited to, surface enhanced spectroscopic properties, such as Raman scattering or fluorescence, as well developments in techniques such as surface plasmon resonance and near-field scanning optical microscopy.