A. Baburajan, R. H. Gaikwad, V. K. Varakhedkar, I. V. Saradhi, A. Vinod Kumar
{"title":"印度Tarapur热带核电站站点陆生植物TFWT和OBT的评估及其与模式计算浓度的比较分析","authors":"A. Baburajan, R. H. Gaikwad, V. K. Varakhedkar, I. V. Saradhi, A. Vinod Kumar","doi":"10.1007/s10967-025-10313-w","DOIUrl":null,"url":null,"abstract":"<div><p>Tritium, a key radionuclide from pressurized heavy water reactors, disperses rapidly and is absorbed by organisms as Tissue-Free Water Tritium (TFWT) and Organically Bound Tritium (OBT). This study examines the measured TFWT and OBT concentrations in terrestrial plants around Nuclear Power Plant (NPP) site at Tarapur, India, from 2016 to 2018 and compared with the computed concentrations. A Gaussian Plume Model (GPM) was used to compute air tritium concentrations, incorporating meteorological data and site-specific model parameters. The key parameters include fractional water content (WCp), water equivalent factor (WEQp), and the OBT-to-TFWT ratio (Rp). Results show higher concentrations near the NPP, with measured values exceeding computed estimates may be due to GPM limitations and environmental variability. A statistical evaluations (mean fractional bias: − 0.095) of computed to measured air tritium (2014 to 2018) confirmed systematic underestimation by computation, highlighting the need for field measurements and site-specific parameterization in tritium transport modelling.</p></div>","PeriodicalId":661,"journal":{"name":"Journal of Radioanalytical and Nuclear Chemistry","volume":"334 8","pages":"5771 - 5783"},"PeriodicalIF":1.6000,"publicationDate":"2025-08-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s10967-025-10313-w.pdf","citationCount":"0","resultStr":"{\"title\":\"Assessment of TFWT and OBT in terrestrial plants at Tarapur, a tropical NPP Site in India, and a comparative analysis with model-computed concentrations\",\"authors\":\"A. Baburajan, R. H. Gaikwad, V. K. Varakhedkar, I. V. Saradhi, A. Vinod Kumar\",\"doi\":\"10.1007/s10967-025-10313-w\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Tritium, a key radionuclide from pressurized heavy water reactors, disperses rapidly and is absorbed by organisms as Tissue-Free Water Tritium (TFWT) and Organically Bound Tritium (OBT). This study examines the measured TFWT and OBT concentrations in terrestrial plants around Nuclear Power Plant (NPP) site at Tarapur, India, from 2016 to 2018 and compared with the computed concentrations. A Gaussian Plume Model (GPM) was used to compute air tritium concentrations, incorporating meteorological data and site-specific model parameters. The key parameters include fractional water content (WCp), water equivalent factor (WEQp), and the OBT-to-TFWT ratio (Rp). Results show higher concentrations near the NPP, with measured values exceeding computed estimates may be due to GPM limitations and environmental variability. A statistical evaluations (mean fractional bias: − 0.095) of computed to measured air tritium (2014 to 2018) confirmed systematic underestimation by computation, highlighting the need for field measurements and site-specific parameterization in tritium transport modelling.</p></div>\",\"PeriodicalId\":661,\"journal\":{\"name\":\"Journal of Radioanalytical and Nuclear Chemistry\",\"volume\":\"334 8\",\"pages\":\"5771 - 5783\"},\"PeriodicalIF\":1.6000,\"publicationDate\":\"2025-08-19\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://link.springer.com/content/pdf/10.1007/s10967-025-10313-w.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Radioanalytical and Nuclear Chemistry\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s10967-025-10313-w\",\"RegionNum\":3,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, ANALYTICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Radioanalytical and Nuclear Chemistry","FirstCategoryId":"92","ListUrlMain":"https://link.springer.com/article/10.1007/s10967-025-10313-w","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, ANALYTICAL","Score":null,"Total":0}
Assessment of TFWT and OBT in terrestrial plants at Tarapur, a tropical NPP Site in India, and a comparative analysis with model-computed concentrations
Tritium, a key radionuclide from pressurized heavy water reactors, disperses rapidly and is absorbed by organisms as Tissue-Free Water Tritium (TFWT) and Organically Bound Tritium (OBT). This study examines the measured TFWT and OBT concentrations in terrestrial plants around Nuclear Power Plant (NPP) site at Tarapur, India, from 2016 to 2018 and compared with the computed concentrations. A Gaussian Plume Model (GPM) was used to compute air tritium concentrations, incorporating meteorological data and site-specific model parameters. The key parameters include fractional water content (WCp), water equivalent factor (WEQp), and the OBT-to-TFWT ratio (Rp). Results show higher concentrations near the NPP, with measured values exceeding computed estimates may be due to GPM limitations and environmental variability. A statistical evaluations (mean fractional bias: − 0.095) of computed to measured air tritium (2014 to 2018) confirmed systematic underestimation by computation, highlighting the need for field measurements and site-specific parameterization in tritium transport modelling.
期刊介绍:
An international periodical publishing original papers, letters, review papers and short communications on nuclear chemistry. The subjects covered include: Nuclear chemistry, Radiochemistry, Radiation chemistry, Radiobiological chemistry, Environmental radiochemistry, Production and control of radioisotopes and labelled compounds, Nuclear power plant chemistry, Nuclear fuel chemistry, Radioanalytical chemistry, Radiation detection and measurement, Nuclear instrumentation and automation, etc.