印度Tarapur热带核电站站点陆生植物TFWT和OBT的评估及其与模式计算浓度的比较分析

IF 1.6 3区 化学 Q3 CHEMISTRY, ANALYTICAL
A. Baburajan, R. H. Gaikwad, V. K. Varakhedkar, I. V. Saradhi, A. Vinod Kumar
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引用次数: 0

摘要

氚是压力重水反应堆中的一种关键放射性核素,扩散迅速,并被生物吸收为无组织水氚(TFWT)和有机结合氚(OBT)。本研究调查了2016年至2018年印度塔拉普尔核电站(NPP)场址周围陆生植物中TFWT和OBT的测量浓度,并与计算浓度进行了比较。采用高斯羽流模型(Gaussian Plume Model, GPM),结合气象数据和特定站点的模型参数计算空气氚浓度。关键参数包括分数含水量(WCp)、水当量因子(WEQp)和OBT-to-TFWT比(Rp)。结果表明,NPP附近的浓度较高,测量值超过计算值,这可能是由于GPM的限制和环境变异性。统计评估(平均分数偏差:- 0.095)计算得出的空气氚(2014年至2018年)证实了计算的系统性低估,强调了在氚输运建模中需要进行现场测量和特定地点参数化。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Assessment of TFWT and OBT in terrestrial plants at Tarapur, a tropical NPP Site in India, and a comparative analysis with model-computed concentrations

Tritium, a key radionuclide from pressurized heavy water reactors, disperses rapidly and is absorbed by organisms as Tissue-Free Water Tritium (TFWT) and Organically Bound Tritium (OBT). This study examines the measured TFWT and OBT concentrations in terrestrial plants around Nuclear Power Plant (NPP) site at Tarapur, India, from 2016 to 2018 and compared with the computed concentrations. A Gaussian Plume Model (GPM) was used to compute air tritium concentrations, incorporating meteorological data and site-specific model parameters. The key parameters include fractional water content (WCp), water equivalent factor (WEQp), and the OBT-to-TFWT ratio (Rp). Results show higher concentrations near the NPP, with measured values exceeding computed estimates may be due to GPM limitations and environmental variability. A statistical evaluations (mean fractional bias: − 0.095) of computed to measured air tritium (2014 to 2018) confirmed systematic underestimation by computation, highlighting the need for field measurements and site-specific parameterization in tritium transport modelling.

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来源期刊
CiteScore
2.80
自引率
18.80%
发文量
504
审稿时长
2.2 months
期刊介绍: An international periodical publishing original papers, letters, review papers and short communications on nuclear chemistry. The subjects covered include: Nuclear chemistry, Radiochemistry, Radiation chemistry, Radiobiological chemistry, Environmental radiochemistry, Production and control of radioisotopes and labelled compounds, Nuclear power plant chemistry, Nuclear fuel chemistry, Radioanalytical chemistry, Radiation detection and measurement, Nuclear instrumentation and automation, etc.
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