重庆市铜梁区菜地土壤重金属污染现状、健康风险评价及来源解析

Q2 Environmental Science
Xu Luo, Lin Yang, Xiao-Ge Shen, Xue-Pin Zhan, Jian Fu, Xiao-Zhong Wang, Ran Xiao
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引用次数: 0

摘要

了解蔬菜土壤重金属污染现状及来源,对土壤保护和蔬菜生产安全具有重要意义。本研究对铜梁区典型蔬菜土壤151份表层蔬菜土壤样品中Cr、Cu、Zn、As、Cd 5种重金属的含量进行了测定。通过地积累指数、富集系数和潜在生态风险指数对重金属污染程度进行评价。采用健康风险模型对重金属的致癌性和非致癌性风险进行评价。采用相关分析、主成分分析(PCA)、聚类分析、绝对主成分评分-多元线性回归(APCS-MLR)等定性和定量方法对表层土壤重金属来源进行分析。结果表明,铜梁区菜地土壤中Cu、Zn和As的平均含量分别高出背景值的1.78倍、1.71倍和3.32倍。15.89%、11.26%、4.64%和3.97%的土壤点Cu、Zn、As和Cd含量分别超过风险筛选值。富集因子分析结果显示,a为光污染,62.62%的土壤样品为光污染,20.56%的土壤样品为中度污染。地质堆积指数分析表明,As处于中度污染水平,Cu和Zn处于轻至中度污染水平。潜在生态风险评价表明,研究区主要为中度生态风险,a类生态风险占51.66%。来源分配分析表明,农业自然源、大气沉积源和未知源的平均贡献分别为66.75%、22.06%和11.19%。健康风险评估进一步显示,As的非致癌风险系数超过1,表明成人和儿童均存在潜在的非致癌风险。因此,迫切需要有效的管理和修复策略来解决砷污染,确保该地区蔬菜生产的安全。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
[Current Pollution Status, Health Risk Assessment and Source Apportionment of Heavy Metals in Vegetable Soil in Tongliang District, Chongqin].

Understanding the status and sources of vegetable soil heavy metals pollution has great significance for soil protection and vegetable production safety. In this study, the contents of five heavy metals, Cr, Cu, Zn, As, and Cd, were collected and determined in 151 surface vegetable soil samples from the typical vegetable soil of Tongliang District. The heavy metals pollution degree was evaluated by means of the geoaccumulation index, enrichment factor, and potential ecological risk index. The carcinogenic and non-carcinogenic risks of the heavy metals were evaluated using the health risk model. The sources of the heavy metals in the topsoil were analyzed by correlation analysis, principal component analysis (PCA), cluster analysis, absolute principal component score-multiple linear regression (APCS-MLR), and other qualitative and quantitative methods. The results showed that the average contents of Cu, Zn, and As in the vegetable garden soils of Tongliang District exceed background values, being 1.78, 1.71, and 3.32 times higher, respectively. The contents of Cu, Zn, As, and Cd in 15.89%, 11.26%, 4.64%, and 3.97% of the soil sites exceeded the risk screening values, respectively. Enrichment factor analysis classified As as light pollution, with 62.62% of the soil samples showing light pollution and 20.56% showing moderate pollution levels. The geoaccumulation index analysis revealed that As is at a moderate pollution level, while Cu and Zn fall into the light-to-moderate pollution category. The potential ecological risk assessment suggested that the study area primarily faces moderate ecological hazards, with As contributing 51.66% of the ecological risk. Source apportionment analysis revealed that the average contributions of agricultural-natural sources, atmospheric deposition, and unknown sources are 66.75%, 22.06%, and 11.19%, respectively. The health risk assessment further revealed that the non-carcinogenic risk quotient for As exceeds 1, indicating potential non-carcinogenic risks for both adults and children. Thus, there is an urgent need for effective management and remediation strategies to address As contamination and ensure the safety of vegetable production in the region.

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环境科学
环境科学 Environmental Science-Environmental Science (all)
CiteScore
4.40
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0.00%
发文量
15329
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