中南半岛生物质燃烧对华南沿海对流层臭氧的多尺度影响:来自长期(2000-2024)观测的见解

IF 4.4 2区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES
Zhiheng Liao , Juncheng Zhu , Chunhua Li , Jielan Xie , Zhiqiang Ma
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引用次数: 0

摘要

生物质燃烧是对流层臭氧(O3)的重要来源。利用香港长期(2000-2024年)臭氧探测资料和中南半岛(ICP)卫星火灾反演资料,结合EAC4再分析资料,探讨了中南半岛春季(3 - 4月)生物质燃烧对华南沿海对流层O3变化和趋势的影响。我们发现香港较低的自由对流层O3 (LFTO3)浓度与印度支那的生物质燃烧,特别是与老挝北部两天前的生物质燃烧显著相关(r = 0.57, p < 0.01)。虽然印度支那生物质燃烧对华南沿海地区LFTO3浓度的影响超过30 ppbv,但对地表O3浓度的影响不显著。在研究期间,尽管印度支那生物质燃烧的数量和强度有所下降,但香港春季LFTO3浓度呈显著上升趋势(0.37 ppbv/年)。这种长期的LFTO3增加趋势主要是由印度支那生物质燃烧向东迁移(主要是由于中部ICP地区生物质燃烧的增加)所驱动的,这使得到香港的运输距离缩短了~ 300公里,从而提高了运输效率,最终贡献了香港长期LFTO3增长的~ 90%。这些发现有助于理解中南半岛生物质燃烧运输对华南沿海对流层O3多尺度变化的影响。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Multi-scale impacts of Indochina biomass burnings on tropospheric ozone in coastal South China: Insights from long-term (2000–2024) observations
Biomass burning is an important source of tropospheric ozone (O3). This study explored the impacts of Indochina springtime (March–April) biomass burnings on the variability and trend of tropospheric O3 in coastal South China using long-term (2000–2024) ozonesondes in Hong Kong and satellite fire retrievals in the Indochina Peninsula (ICP), complemented with EAC4 reanalysis data. We find that the lower-free-tropospheric O3 (LFTO3) concentrations in Hong Kong are significantly correlated with the Indochina biomass burnings, particularly with the two-day-ago biomass burnings in northern Laos (r = 0.57, p < 0.01). While Indochina biomass burning contributes more than 30 ppbv enhancements in LFTO3 concentrations over coastal South China, their impacts on surface O3 concentrations are insignificant. During the study period, there is a significant increasing trend in springtime LFTO3 concentrations in Hong Kong (0.37 ppbv/year), despite decreasing quantity and intension of Indochina biomass burnings. This long-term LFTO3 increasing trend is mainly driven by the eastward migration of Indochina biomass burnings (mainly due to the increase in biomass burnings in the central ICP region), which reduces transport distance to Hong Kong by ∼300 km and thereby improves the transport efficiency, ultimately contributing ∼90 % of the long-term LFTO3 increase in Hong Kong. These findings advance understanding of Indochina biomass burning transport impacts on multi-scale tropospheric O3 variability in coastal South China.
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来源期刊
Atmospheric Research
Atmospheric Research 地学-气象与大气科学
CiteScore
9.40
自引率
10.90%
发文量
460
审稿时长
47 days
期刊介绍: The journal publishes scientific papers (research papers, review articles, letters and notes) dealing with the part of the atmosphere where meteorological events occur. Attention is given to all processes extending from the earth surface to the tropopause, but special emphasis continues to be devoted to the physics of clouds, mesoscale meteorology and air pollution, i.e. atmospheric aerosols; microphysical processes; cloud dynamics and thermodynamics; numerical simulation, climatology, climate change and weather modification.
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