基于绿色双钙钛矿qds敏化二维半导体的UVA/ b选择性皮肤激发伤害感受器可靠的人体体感系统模拟。

IF 4.6 2区 化学 Q2 CHEMISTRY, PHYSICAL
Yuchan Wang, Ting Chen, Zihe Liu, Lei Zheng*, Chenhao Xu, Jianzhou Ren, Hongling Guo, Kai Hu*, Wenxia Zhang* and Kailiang Zhang, 
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引用次数: 0

摘要

在单个设备水平上实现UVA/ b选择性、皮肤激发的具有感知和阻断功能的伤害感受器仍然具有挑战性。这是因为该器件需要为每个性能指标提供不同的组件,从而导致复杂的制备工艺和受限的性能,以及缺乏深紫外(UVB及以下)选择性半导体。在这里,为了解决这个问题,我们使用反向ii型Cu2AgSbI6/MoS2异质结构开发了一种结构简化的皮肤激发伤害感受器。它在Cu2AgSbI6中集成了出色的UVA/B敏化增益,在离域和键能方面优于传统的基于cu2agmiiii6的量子点,并表现出高效的多场调制电荷自俘获传输。因此,在365/280 nm紫外光照射下,混合光电晶体管的探测率(30/14倍)和光响应率(6.4/7.2倍)显著提高。此外,它可以可靠地模拟计算能力,对皮肤激发的伤害感受器功能具有不同寻常的适应性,实现了大约52%的不同寻常的神经阻断度。这项工作提出了一种新的方法来设计复杂的仿生功能的二维材料用于先进的神经形态光电子学。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

UVA/B-Selective Skin-Inspired Nociceptors Based on Green Double Perovskite QDs-Sensitized 2D Semiconductor toward Reliable Human Somatosensory System Simulation

UVA/B-Selective Skin-Inspired Nociceptors Based on Green Double Perovskite QDs-Sensitized 2D Semiconductor toward Reliable Human Somatosensory System Simulation

Achieving UVA/B-selective, skin-inspired nociceptors with perception and blockade functions at the single-unit device level remains challenging. This is because the device necessitates distinct components for every performance metric, thereby leading to complex preparation processes and restricted performance, as well as the absence of deep UV (UVB and below)-selective semiconductors. Here, to address this, we develop a structure-simplification skin-inspired nociceptor using a reverse type-II Cu2AgSbI6/MoS2 heterostructure. It integrates excellent UVA/B sensitization gain in Cu2AgSbI6, surpassing traditional Cu2AgMIIII6-based QDs in delocalization and bond energy, and exhibits efficient multifield modulated charge self-trapping transport. Consequently, the hybrid phototransistor shows significant increases in detectivity (30/14 times) and photoresponsivity (6.4/7.2 times) under 365/280 nm UV illumination. Moreover, it can reliably mimic computational capabilities with unusual adaptivity for skin-inspired nociceptor functions, achieving an unusual neural blocking degree of approximately 52%. This work presents a new approach for designing complex bionic functions in 2D materials for advanced neuromorphic photoelectronics.

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来源期刊
The Journal of Physical Chemistry Letters
The Journal of Physical Chemistry Letters CHEMISTRY, PHYSICAL-NANOSCIENCE & NANOTECHNOLOGY
CiteScore
9.60
自引率
7.00%
发文量
1519
审稿时长
1.6 months
期刊介绍: The Journal of Physical Chemistry (JPC) Letters is devoted to reporting new and original experimental and theoretical basic research of interest to physical chemists, biophysical chemists, chemical physicists, physicists, material scientists, and engineers. An important criterion for acceptance is that the paper reports a significant scientific advance and/or physical insight such that rapid publication is essential. Two issues of JPC Letters are published each month.
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