对电池树突生长机制的洞察:结合机器学习和计算研究

Zirui Zhao, Junchao Xia, Si Wu, Xiaoke Wang, Guanping Xu, Yinghao Zhu, Jing Sun, Hai-Feng Li
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引用次数: 0

摘要

近年来,由于电池具有高能量密度、低成本和环境适应性,研究人员越来越多地寻求电池作为一种高效、经济的能量存储和供应解决方案。然而,树突生长的问题已经成为电池发展的一个重大障碍。在充放电过程中,过度的枝晶生长会导致电池短路、电化学性能下降、循环寿命缩短和异常放热事件。因此,了解树突生长过程已成为研究人员面临的关键挑战。在这项研究中,我们使用组合机器学习方法,特别是二维人工卷积神经网络(CNN)模型,以及计算方法来研究电池中的枝晶生长机制。我们开发了两种不同的计算机模型来预测电池中的树突生长。CNN-1模型采用标准的CNN技术进行树突生长预测,而CNN-2则集成了额外的物理参数来增强模型的鲁棒性。我们的研究结果表明,CNN-2显著提高了预测精度,为物理因素对树突生长的影响提供了更深入的见解。该改进模型有效地捕捉了枝晶形成的动态特性,具有较高的精度和灵敏度。这些发现有助于开发更安全、更可靠的储能系统。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Insights Into Dendritic Growth Mechanisms in Batteries: A Combined Machine Learning and Computational Study

Insights Into Dendritic Growth Mechanisms in Batteries: A Combined Machine Learning and Computational Study

In recent years, researchers have increasingly sought batteries as an efficient and cost-effective solution for energy storage and supply, owing to their high energy density, low cost, and environmental resilience. However, the issue of dendrite growth has emerged as a significant obstacle in battery development. Excessive dendrite growth during charging and discharging processes can lead to battery short-circuiting, degradation of electrochemical performance, reduced cycle life, and abnormal exothermic events. Consequently, understanding the dendrite growth process has become a key challenge for researchers. In this study, we investigated dendrite growth mechanisms in batteries using a combined machine learning approach, specifically a two-dimensional artificial convolutional neural network (CNN) model, along with computational methods. We developed two distinct computer models to predict dendrite growth in batteries. The CNN-1 model employs standard CNN techniques for dendritic growth prediction, while CNN-2 integrates additional physical parameters to enhance model robustness. Our results demonstrate that CNN-2 significantly enhances prediction accuracy, offering deeper insights into the impact of physical factors on dendritic growth. This improved model effectively captures the dynamic nature of dendrite formation, exhibiting high accuracy and sensitivity. These findings contribute to the advancement of safer and more reliable energy storage systems.

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