{"title":"基于银三角形纳米片的维生素C快速灵敏检测增强多比色传感器","authors":"Indah Nursyamsi Handayani , Nursama Heru Apriantoro , Amanda Aurelia , Muhammad Rizki Nugroho , Yudhistira Tirtayasri Amrillah , Ferry Anggoro Ardy Nugroho , Adhi Harmoko Saputro , Vivi Fauzia","doi":"10.1016/j.optmat.2025.117487","DOIUrl":null,"url":null,"abstract":"<div><div>Colorimetric sensors have emerged as promising alternatives for vitamin C detection due to their simplicity, speed, and ease of use. However, conventional single-color indicators often suffer from limited sensitivity and are challenging for naked-eye detection. This study presents a simple, rapid, and reliable multi-colorimetric method for vitamin C detection using silver triangular nanoplates (AgTNPs) as the sensing platform. By investigating the effect of varying potassium chloride (KCl) concentrations (2, 4, 8, and 10 mM), the results reveal that an optimal KCl concentration of 8 mM significantly enhances the sensor's performance. The enhanced sensor achieved a high sensitivity of 4.57 nm/μM ± 0.35 nm/μM with a correlation coefficient of 96 %, and lowest LOD was 0.52 μM enabling accurate quantification of vitamin C across a concentration range of 0–40 μM. Furthermore, the sensor demonstrated an ultra-fast response time (as low as 27 s), making it suitable for real-time applications. To further improve usability, a novel visual detection approach using Euclidean distance (<span><math><mrow><mi>d</mi></mrow></math></span>) analysis was introduced, facilitating direct visual observation of vitamin C concentrations. The sensor achieved Euclidean distance values exceeding 0.020 units for vitamin C concentrations above 20 μM, providing a clear and distinguishable color change visible to the naked eye. These findings establish the enhanced AgTNP-based colorimetric sensor as a highly effective tool for vitamin C detection in food samples, offering a practical solution for quality control and nutritional analysis.</div></div>","PeriodicalId":19564,"journal":{"name":"Optical Materials","volume":"168 ","pages":"Article 117487"},"PeriodicalIF":4.2000,"publicationDate":"2025-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Enhanced multi-colorimetric sensor based on silver triangular nanoplates for rapid and sensitive vitamin C detection\",\"authors\":\"Indah Nursyamsi Handayani , Nursama Heru Apriantoro , Amanda Aurelia , Muhammad Rizki Nugroho , Yudhistira Tirtayasri Amrillah , Ferry Anggoro Ardy Nugroho , Adhi Harmoko Saputro , Vivi Fauzia\",\"doi\":\"10.1016/j.optmat.2025.117487\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Colorimetric sensors have emerged as promising alternatives for vitamin C detection due to their simplicity, speed, and ease of use. However, conventional single-color indicators often suffer from limited sensitivity and are challenging for naked-eye detection. This study presents a simple, rapid, and reliable multi-colorimetric method for vitamin C detection using silver triangular nanoplates (AgTNPs) as the sensing platform. By investigating the effect of varying potassium chloride (KCl) concentrations (2, 4, 8, and 10 mM), the results reveal that an optimal KCl concentration of 8 mM significantly enhances the sensor's performance. The enhanced sensor achieved a high sensitivity of 4.57 nm/μM ± 0.35 nm/μM with a correlation coefficient of 96 %, and lowest LOD was 0.52 μM enabling accurate quantification of vitamin C across a concentration range of 0–40 μM. Furthermore, the sensor demonstrated an ultra-fast response time (as low as 27 s), making it suitable for real-time applications. To further improve usability, a novel visual detection approach using Euclidean distance (<span><math><mrow><mi>d</mi></mrow></math></span>) analysis was introduced, facilitating direct visual observation of vitamin C concentrations. The sensor achieved Euclidean distance values exceeding 0.020 units for vitamin C concentrations above 20 μM, providing a clear and distinguishable color change visible to the naked eye. These findings establish the enhanced AgTNP-based colorimetric sensor as a highly effective tool for vitamin C detection in food samples, offering a practical solution for quality control and nutritional analysis.</div></div>\",\"PeriodicalId\":19564,\"journal\":{\"name\":\"Optical Materials\",\"volume\":\"168 \",\"pages\":\"Article 117487\"},\"PeriodicalIF\":4.2000,\"publicationDate\":\"2025-09-05\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Optical Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S092534672500847X\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Optical Materials","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S092534672500847X","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Enhanced multi-colorimetric sensor based on silver triangular nanoplates for rapid and sensitive vitamin C detection
Colorimetric sensors have emerged as promising alternatives for vitamin C detection due to their simplicity, speed, and ease of use. However, conventional single-color indicators often suffer from limited sensitivity and are challenging for naked-eye detection. This study presents a simple, rapid, and reliable multi-colorimetric method for vitamin C detection using silver triangular nanoplates (AgTNPs) as the sensing platform. By investigating the effect of varying potassium chloride (KCl) concentrations (2, 4, 8, and 10 mM), the results reveal that an optimal KCl concentration of 8 mM significantly enhances the sensor's performance. The enhanced sensor achieved a high sensitivity of 4.57 nm/μM ± 0.35 nm/μM with a correlation coefficient of 96 %, and lowest LOD was 0.52 μM enabling accurate quantification of vitamin C across a concentration range of 0–40 μM. Furthermore, the sensor demonstrated an ultra-fast response time (as low as 27 s), making it suitable for real-time applications. To further improve usability, a novel visual detection approach using Euclidean distance () analysis was introduced, facilitating direct visual observation of vitamin C concentrations. The sensor achieved Euclidean distance values exceeding 0.020 units for vitamin C concentrations above 20 μM, providing a clear and distinguishable color change visible to the naked eye. These findings establish the enhanced AgTNP-based colorimetric sensor as a highly effective tool for vitamin C detection in food samples, offering a practical solution for quality control and nutritional analysis.
期刊介绍:
Optical Materials has an open access mirror journal Optical Materials: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review.
The purpose of Optical Materials is to provide a means of communication and technology transfer between researchers who are interested in materials for potential device applications. The journal publishes original papers and review articles on the design, synthesis, characterisation and applications of optical materials.
OPTICAL MATERIALS focuses on:
• Optical Properties of Material Systems;
• The Materials Aspects of Optical Phenomena;
• The Materials Aspects of Devices and Applications.
Authors can submit separate research elements describing their data to Data in Brief and methods to Methods X.