{"title":"高效稳定的纯蓝色钙钛矿发光二极管,用于高色纯度高级显示器","authors":"Gi-Jeong Park, Kyoung-Been Shin and Min-Ho Park*, ","doi":"10.1021/acsaelm.5c01342","DOIUrl":null,"url":null,"abstract":"<p >Metal halide perovskite light-emitting diodes (PeLEDs) have garnered substantial attention owing to their exceptional optoelectronic properties, enabling rapid advancements in red and green devices with external quantum efficiencies (EQEs) approaching 30%. However, blue PeLEDs continue to lag behind in both efficiency and spectral stability, posing a critical barrier to achieving full-color, ultrahigh-definition displays. Although sky-blue PeLEDs (470–490 nm) have demonstrated relatively high efficiencies, their emission spectra have failed to meet the stringent chromaticity requirements defined by Rec.2020 and NTSC standards. Deep-blue emitters (440–460 nm), however, raise safety concerns owing to potential photobiological hazards, such as retinal damage. These limitations underscore the urgent need for pure-blue PeLEDs (460–470 nm) that offer an optimal balance between spectral accuracy, device safety, and performance. In this paper, we explore strategies aimed at improving the spectral stability and emission efficiency of pure-blue PeLEDs. Specifically, we highlight the impact of dimensional engineering and ion substitution on enhancing spectral stability and discuss additive engineering, ligand engineering, and interface engineering as key approaches for boosting emission efficiency. Together, these strategies offer a comprehensive framework for addressing the critical limitations of pure-blue PeLEDs and advancing their integration into next-generation display technologies.</p>","PeriodicalId":3,"journal":{"name":"ACS Applied Electronic Materials","volume":"7 17","pages":"7963–7973"},"PeriodicalIF":4.7000,"publicationDate":"2025-08-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Efficient and Stable Pure-Blue Perovskite Light-Emitting Diodes for High-Color-Purity Advanced Displays\",\"authors\":\"Gi-Jeong Park, Kyoung-Been Shin and Min-Ho Park*, \",\"doi\":\"10.1021/acsaelm.5c01342\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Metal halide perovskite light-emitting diodes (PeLEDs) have garnered substantial attention owing to their exceptional optoelectronic properties, enabling rapid advancements in red and green devices with external quantum efficiencies (EQEs) approaching 30%. However, blue PeLEDs continue to lag behind in both efficiency and spectral stability, posing a critical barrier to achieving full-color, ultrahigh-definition displays. Although sky-blue PeLEDs (470–490 nm) have demonstrated relatively high efficiencies, their emission spectra have failed to meet the stringent chromaticity requirements defined by Rec.2020 and NTSC standards. Deep-blue emitters (440–460 nm), however, raise safety concerns owing to potential photobiological hazards, such as retinal damage. These limitations underscore the urgent need for pure-blue PeLEDs (460–470 nm) that offer an optimal balance between spectral accuracy, device safety, and performance. In this paper, we explore strategies aimed at improving the spectral stability and emission efficiency of pure-blue PeLEDs. Specifically, we highlight the impact of dimensional engineering and ion substitution on enhancing spectral stability and discuss additive engineering, ligand engineering, and interface engineering as key approaches for boosting emission efficiency. Together, these strategies offer a comprehensive framework for addressing the critical limitations of pure-blue PeLEDs and advancing their integration into next-generation display technologies.</p>\",\"PeriodicalId\":3,\"journal\":{\"name\":\"ACS Applied Electronic Materials\",\"volume\":\"7 17\",\"pages\":\"7963–7973\"},\"PeriodicalIF\":4.7000,\"publicationDate\":\"2025-08-27\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Electronic Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsaelm.5c01342\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, ELECTRICAL & ELECTRONIC\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Electronic Materials","FirstCategoryId":"88","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsaelm.5c01342","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ELECTRICAL & ELECTRONIC","Score":null,"Total":0}
Efficient and Stable Pure-Blue Perovskite Light-Emitting Diodes for High-Color-Purity Advanced Displays
Metal halide perovskite light-emitting diodes (PeLEDs) have garnered substantial attention owing to their exceptional optoelectronic properties, enabling rapid advancements in red and green devices with external quantum efficiencies (EQEs) approaching 30%. However, blue PeLEDs continue to lag behind in both efficiency and spectral stability, posing a critical barrier to achieving full-color, ultrahigh-definition displays. Although sky-blue PeLEDs (470–490 nm) have demonstrated relatively high efficiencies, their emission spectra have failed to meet the stringent chromaticity requirements defined by Rec.2020 and NTSC standards. Deep-blue emitters (440–460 nm), however, raise safety concerns owing to potential photobiological hazards, such as retinal damage. These limitations underscore the urgent need for pure-blue PeLEDs (460–470 nm) that offer an optimal balance between spectral accuracy, device safety, and performance. In this paper, we explore strategies aimed at improving the spectral stability and emission efficiency of pure-blue PeLEDs. Specifically, we highlight the impact of dimensional engineering and ion substitution on enhancing spectral stability and discuss additive engineering, ligand engineering, and interface engineering as key approaches for boosting emission efficiency. Together, these strategies offer a comprehensive framework for addressing the critical limitations of pure-blue PeLEDs and advancing their integration into next-generation display technologies.
期刊介绍:
ACS Applied Electronic Materials is an interdisciplinary journal publishing original research covering all aspects of electronic materials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials science, engineering, optics, physics, and chemistry into important applications of electronic materials. Sample research topics that span the journal's scope are inorganic, organic, ionic and polymeric materials with properties that include conducting, semiconducting, superconducting, insulating, dielectric, magnetic, optoelectronic, piezoelectric, ferroelectric and thermoelectric.
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CAS
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