Yi Zhou, Chunhui Shen, Teng Wang, Feng Wang and Yongjie Xue*,
{"title":"金属负载生物炭用于低排放和长效沥青","authors":"Yi Zhou, Chunhui Shen, Teng Wang, Feng Wang and Yongjie Xue*, ","doi":"10.1021/acssuschemeng.5c04405","DOIUrl":null,"url":null,"abstract":"<p >Volatile organic compound (VOC) emissions and premature aging of asphalt pose significant environmental and resource management challenges. This study evaluates metal-loaded biochar (Fe, Zn, and Cu) as a sustainable modifier to reduce VOC emissions and enhance asphalt durability. Fe-loaded biochar achieved up to a 73.7% reduction in VOCs, with Fe and Zn particularly effective against aromatic and long-chain alkanes, and Cu targeting small molecular alkanes. Rheological analyses indicate that metal-loaded biochar increases asphalt stiffness and deformation resistance. Moreover, both short-term and UV aging tests demonstrate that biochar modification improves antiaging performance, attributed to the adsorption of polar compounds and stabilization of aging byproducts. By extending pavement lifespan and reducing the need for repaving, this dual-function approach promotes resource conservation and supports a transition toward greener, more sustainable infrastructure practices.</p>","PeriodicalId":25,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"13 36","pages":"14834–14843"},"PeriodicalIF":7.3000,"publicationDate":"2025-09-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Metal-Loaded Biochar for Low-Emission and Long-Lasting Asphalt\",\"authors\":\"Yi Zhou, Chunhui Shen, Teng Wang, Feng Wang and Yongjie Xue*, \",\"doi\":\"10.1021/acssuschemeng.5c04405\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Volatile organic compound (VOC) emissions and premature aging of asphalt pose significant environmental and resource management challenges. This study evaluates metal-loaded biochar (Fe, Zn, and Cu) as a sustainable modifier to reduce VOC emissions and enhance asphalt durability. Fe-loaded biochar achieved up to a 73.7% reduction in VOCs, with Fe and Zn particularly effective against aromatic and long-chain alkanes, and Cu targeting small molecular alkanes. Rheological analyses indicate that metal-loaded biochar increases asphalt stiffness and deformation resistance. Moreover, both short-term and UV aging tests demonstrate that biochar modification improves antiaging performance, attributed to the adsorption of polar compounds and stabilization of aging byproducts. By extending pavement lifespan and reducing the need for repaving, this dual-function approach promotes resource conservation and supports a transition toward greener, more sustainable infrastructure practices.</p>\",\"PeriodicalId\":25,\"journal\":{\"name\":\"ACS Sustainable Chemistry & Engineering\",\"volume\":\"13 36\",\"pages\":\"14834–14843\"},\"PeriodicalIF\":7.3000,\"publicationDate\":\"2025-09-03\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Sustainable Chemistry & Engineering\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acssuschemeng.5c04405\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Sustainable Chemistry & Engineering","FirstCategoryId":"92","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acssuschemeng.5c04405","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Metal-Loaded Biochar for Low-Emission and Long-Lasting Asphalt
Volatile organic compound (VOC) emissions and premature aging of asphalt pose significant environmental and resource management challenges. This study evaluates metal-loaded biochar (Fe, Zn, and Cu) as a sustainable modifier to reduce VOC emissions and enhance asphalt durability. Fe-loaded biochar achieved up to a 73.7% reduction in VOCs, with Fe and Zn particularly effective against aromatic and long-chain alkanes, and Cu targeting small molecular alkanes. Rheological analyses indicate that metal-loaded biochar increases asphalt stiffness and deformation resistance. Moreover, both short-term and UV aging tests demonstrate that biochar modification improves antiaging performance, attributed to the adsorption of polar compounds and stabilization of aging byproducts. By extending pavement lifespan and reducing the need for repaving, this dual-function approach promotes resource conservation and supports a transition toward greener, more sustainable infrastructure practices.
期刊介绍:
ACS Sustainable Chemistry & Engineering is a prestigious weekly peer-reviewed scientific journal published by the American Chemical Society. Dedicated to advancing the principles of green chemistry and green engineering, it covers a wide array of research topics including green chemistry, green engineering, biomass, alternative energy, and life cycle assessment.
The journal welcomes submissions in various formats, including Letters, Articles, Features, and Perspectives (Reviews), that address the challenges of sustainability in the chemical enterprise and contribute to the advancement of sustainable practices. Join us in shaping the future of sustainable chemistry and engineering.