金属负载生物炭用于低排放和长效沥青

IF 7.3 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Yi Zhou, Chunhui Shen, Teng Wang, Feng Wang and Yongjie Xue*, 
{"title":"金属负载生物炭用于低排放和长效沥青","authors":"Yi Zhou,&nbsp;Chunhui Shen,&nbsp;Teng Wang,&nbsp;Feng Wang and Yongjie Xue*,&nbsp;","doi":"10.1021/acssuschemeng.5c04405","DOIUrl":null,"url":null,"abstract":"<p >Volatile organic compound (VOC) emissions and premature aging of asphalt pose significant environmental and resource management challenges. This study evaluates metal-loaded biochar (Fe, Zn, and Cu) as a sustainable modifier to reduce VOC emissions and enhance asphalt durability. Fe-loaded biochar achieved up to a 73.7% reduction in VOCs, with Fe and Zn particularly effective against aromatic and long-chain alkanes, and Cu targeting small molecular alkanes. Rheological analyses indicate that metal-loaded biochar increases asphalt stiffness and deformation resistance. Moreover, both short-term and UV aging tests demonstrate that biochar modification improves antiaging performance, attributed to the adsorption of polar compounds and stabilization of aging byproducts. By extending pavement lifespan and reducing the need for repaving, this dual-function approach promotes resource conservation and supports a transition toward greener, more sustainable infrastructure practices.</p>","PeriodicalId":25,"journal":{"name":"ACS Sustainable Chemistry & Engineering","volume":"13 36","pages":"14834–14843"},"PeriodicalIF":7.3000,"publicationDate":"2025-09-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Metal-Loaded Biochar for Low-Emission and Long-Lasting Asphalt\",\"authors\":\"Yi Zhou,&nbsp;Chunhui Shen,&nbsp;Teng Wang,&nbsp;Feng Wang and Yongjie Xue*,&nbsp;\",\"doi\":\"10.1021/acssuschemeng.5c04405\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Volatile organic compound (VOC) emissions and premature aging of asphalt pose significant environmental and resource management challenges. This study evaluates metal-loaded biochar (Fe, Zn, and Cu) as a sustainable modifier to reduce VOC emissions and enhance asphalt durability. Fe-loaded biochar achieved up to a 73.7% reduction in VOCs, with Fe and Zn particularly effective against aromatic and long-chain alkanes, and Cu targeting small molecular alkanes. Rheological analyses indicate that metal-loaded biochar increases asphalt stiffness and deformation resistance. Moreover, both short-term and UV aging tests demonstrate that biochar modification improves antiaging performance, attributed to the adsorption of polar compounds and stabilization of aging byproducts. By extending pavement lifespan and reducing the need for repaving, this dual-function approach promotes resource conservation and supports a transition toward greener, more sustainable infrastructure practices.</p>\",\"PeriodicalId\":25,\"journal\":{\"name\":\"ACS Sustainable Chemistry & Engineering\",\"volume\":\"13 36\",\"pages\":\"14834–14843\"},\"PeriodicalIF\":7.3000,\"publicationDate\":\"2025-09-03\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Sustainable Chemistry & Engineering\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acssuschemeng.5c04405\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Sustainable Chemistry & Engineering","FirstCategoryId":"92","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acssuschemeng.5c04405","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

挥发性有机化合物(VOC)的排放和沥青的过早老化对环境和资源管理提出了重大挑战。本研究评估了金属负载生物炭(铁、锌和铜)作为一种可持续改性剂,以减少挥发性有机化合物的排放,提高沥青的耐久性。含铁生物炭的挥发性有机化合物减少率高达73.7%,其中铁和锌对芳香和长链烷烃特别有效,铜对小分子烷烃特别有效。流变学分析表明,金属负载生物炭增加了沥青的刚度和抗变形能力。此外,短期和紫外线老化试验都表明,生物炭改性提高了抗老化性能,这是由于极性化合物的吸附和老化副产物的稳定。通过延长路面寿命和减少重新铺设的需求,这种双重功能的方法促进了资源节约,并支持向更绿色、更可持续的基础设施实践过渡。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Metal-Loaded Biochar for Low-Emission and Long-Lasting Asphalt

Metal-Loaded Biochar for Low-Emission and Long-Lasting Asphalt

Volatile organic compound (VOC) emissions and premature aging of asphalt pose significant environmental and resource management challenges. This study evaluates metal-loaded biochar (Fe, Zn, and Cu) as a sustainable modifier to reduce VOC emissions and enhance asphalt durability. Fe-loaded biochar achieved up to a 73.7% reduction in VOCs, with Fe and Zn particularly effective against aromatic and long-chain alkanes, and Cu targeting small molecular alkanes. Rheological analyses indicate that metal-loaded biochar increases asphalt stiffness and deformation resistance. Moreover, both short-term and UV aging tests demonstrate that biochar modification improves antiaging performance, attributed to the adsorption of polar compounds and stabilization of aging byproducts. By extending pavement lifespan and reducing the need for repaving, this dual-function approach promotes resource conservation and supports a transition toward greener, more sustainable infrastructure practices.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
ACS Sustainable Chemistry & Engineering
ACS Sustainable Chemistry & Engineering CHEMISTRY, MULTIDISCIPLINARY-ENGINEERING, CHEMICAL
CiteScore
13.80
自引率
4.80%
发文量
1470
审稿时长
1.7 months
期刊介绍: ACS Sustainable Chemistry & Engineering is a prestigious weekly peer-reviewed scientific journal published by the American Chemical Society. Dedicated to advancing the principles of green chemistry and green engineering, it covers a wide array of research topics including green chemistry, green engineering, biomass, alternative energy, and life cycle assessment. The journal welcomes submissions in various formats, including Letters, Articles, Features, and Perspectives (Reviews), that address the challenges of sustainability in the chemical enterprise and contribute to the advancement of sustainable practices. Join us in shaping the future of sustainable chemistry and engineering.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信