手性磷酸催化环亚胺还原对映选择性合成雷沙吉兰的研究。

IF 3.3 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Hayate Ishizuka, Toma Osawa, Yuta Shimizu, Hideyuki Sogo, Ryoya Imaizumi, Naohisa Shiba, Ayato Nureki, Taisei Matoba, Minami Odagi, Kazuo Nagasawa
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引用次数: 0

摘要

甲磺酸雷沙吉兰是临床上用于治疗帕金森病的单胺氧化酶B抑制剂。传统的合成依赖于光学分辨率,这限制了效率和可扩展性。为了克服这些挑战,我们开发了一种环丙基亚胺中间体的不对称转移氢化(ATH)对映选择性合成路线。虽然环亚胺由于其刚性结构而难以还原,但使用含Hantzsch酯的手性磷酸催化剂克服了这一挑战,从而提供了高收率和对映选择性的手性胺。该方法成功地扩展到克级,甲磺酸雷沙吉兰的对映体过量率为96%。此外,这种方法显示出广泛的底物相容性,强调了它在环亚胺衍生物的不对称还原中的一般效用。我们的策略为合成雷沙吉兰和结构相关的旋光性胺的现有方法提供了一种实用且可扩展的替代方法。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Enantioselective Gram-Scale Synthesis of Rasagiline via Chiral Phosphoric Acid-Catalyzed Reduction of Cyclic Imine.

Rasagiline mesylate is a monoamine oxidase B inhibitor used clinically for treating Parkinson's disease. Conventional synthesis relies on optical resolution, which limits efficiency and scalability. To overcome these challenges, we developed an enantioselective synthesis route using asymmetric transfer hydrogenation (ATH) of a cyclic propargyl imine intermediate. Although cyclic imines are difficult to reduce due to their rigid structures, this challenge was overcome using a chiral phosphoric acid catalyst with a Hantzsch ester, affording chiral amines in high yield and enantioselectivity. The method was successfully scaled to the gram level, affording rasagiline mesylate with >96% enantiomeric excess. Furthermore, this approach showed broad substrate compatibility, underscoring its general utility in the asymmetric reduction of cyclic imine derivatives. Our strategy offers a practical and scalable alternative to existing methods for the synthesis of rasagiline and structurally related optically active amines.

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来源期刊
Chemistry - An Asian Journal
Chemistry - An Asian Journal 化学-化学综合
CiteScore
7.00
自引率
2.40%
发文量
535
审稿时长
1.3 months
期刊介绍: Chemistry—An Asian Journal is an international high-impact journal for chemistry in its broadest sense. The journal covers all aspects of chemistry from biochemistry through organic and inorganic chemistry to physical chemistry, including interdisciplinary topics. Chemistry—An Asian Journal publishes Full Papers, Communications, and Focus Reviews. A professional editorial team headed by Dr. Theresa Kueckmann and an Editorial Board (headed by Professor Susumu Kitagawa) ensure the highest quality of the peer-review process, the contents and the production of the journal. Chemistry—An Asian Journal is published on behalf of the Asian Chemical Editorial Society (ACES), an association of numerous Asian chemical societies, and supported by the Gesellschaft Deutscher Chemiker (GDCh, German Chemical Society), ChemPubSoc Europe, and the Federation of Asian Chemical Societies (FACS).
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