{"title":"具有超宽量程和高灵敏度的仿生离子电子压力传感器。","authors":"Zijun Pan, , , Bolong Qin, , , Zhanghao Lin, , , Haowei Kong, , , Senrong Ye, , , Haohan Wu, , , Chenchen Bian, , , Gengzhe Shen*, , , Yeqing Chen, , , Chi Zhang, , , Weijia Yang, , and , Xin He*, ","doi":"10.1021/acssensors.5c02041","DOIUrl":null,"url":null,"abstract":"<p >The trade-off between sensitivity and detection range has limited the performance of flexible pressure sensors, hindering their deployment in advanced human–machine interfaces and precision healthcare monitoring. Inspired by the ion-mediated electrogenesis of electric eels, we report a bioinspired iontronic pressure sensor (IPS) that overcomes this bottleneck by coupling MXene-functionalized electrodes with a hierarchical silica aerogel/ionic liquid (ILA) dielectric. This architecture enables pressure-driven, reversible ion migration within the porous dielectric and enhances electrical double-layer (EDL) formation at the electrode-dielectric interface. As a result, the IPS delivers an ultrawide detection range of up to 5.8 MPa, a high sensitivity of 26,845 kPa<sup>–1</sup> within 400 kPa, rapid response/recovery times of 5 ms/6 ms, outstanding durability over 10,000 loading cycles, and intrinsic flame retardancy. These distinctive capabilities allow monitoring of subtle physiological signals and complex human motions even under harsh conditions. This bioinspired approach enables the development of advanced flexible pressure sensors, thereby paving the way for advancements in adaptive robotics, intelligent wearables, and advanced healthcare diagnostics.</p>","PeriodicalId":24,"journal":{"name":"ACS Sensors","volume":"10 9","pages":"6991–7001"},"PeriodicalIF":9.1000,"publicationDate":"2025-08-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Bioinspired Iontronic Pressure Sensor with Ultrawide Range and High Sensitivity\",\"authors\":\"Zijun Pan, , , Bolong Qin, , , Zhanghao Lin, , , Haowei Kong, , , Senrong Ye, , , Haohan Wu, , , Chenchen Bian, , , Gengzhe Shen*, , , Yeqing Chen, , , Chi Zhang, , , Weijia Yang, , and , Xin He*, \",\"doi\":\"10.1021/acssensors.5c02041\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >The trade-off between sensitivity and detection range has limited the performance of flexible pressure sensors, hindering their deployment in advanced human–machine interfaces and precision healthcare monitoring. Inspired by the ion-mediated electrogenesis of electric eels, we report a bioinspired iontronic pressure sensor (IPS) that overcomes this bottleneck by coupling MXene-functionalized electrodes with a hierarchical silica aerogel/ionic liquid (ILA) dielectric. This architecture enables pressure-driven, reversible ion migration within the porous dielectric and enhances electrical double-layer (EDL) formation at the electrode-dielectric interface. As a result, the IPS delivers an ultrawide detection range of up to 5.8 MPa, a high sensitivity of 26,845 kPa<sup>–1</sup> within 400 kPa, rapid response/recovery times of 5 ms/6 ms, outstanding durability over 10,000 loading cycles, and intrinsic flame retardancy. These distinctive capabilities allow monitoring of subtle physiological signals and complex human motions even under harsh conditions. This bioinspired approach enables the development of advanced flexible pressure sensors, thereby paving the way for advancements in adaptive robotics, intelligent wearables, and advanced healthcare diagnostics.</p>\",\"PeriodicalId\":24,\"journal\":{\"name\":\"ACS Sensors\",\"volume\":\"10 9\",\"pages\":\"6991–7001\"},\"PeriodicalIF\":9.1000,\"publicationDate\":\"2025-08-21\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Sensors\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acssensors.5c02041\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, ANALYTICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Sensors","FirstCategoryId":"92","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acssensors.5c02041","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, ANALYTICAL","Score":null,"Total":0}
Bioinspired Iontronic Pressure Sensor with Ultrawide Range and High Sensitivity
The trade-off between sensitivity and detection range has limited the performance of flexible pressure sensors, hindering their deployment in advanced human–machine interfaces and precision healthcare monitoring. Inspired by the ion-mediated electrogenesis of electric eels, we report a bioinspired iontronic pressure sensor (IPS) that overcomes this bottleneck by coupling MXene-functionalized electrodes with a hierarchical silica aerogel/ionic liquid (ILA) dielectric. This architecture enables pressure-driven, reversible ion migration within the porous dielectric and enhances electrical double-layer (EDL) formation at the electrode-dielectric interface. As a result, the IPS delivers an ultrawide detection range of up to 5.8 MPa, a high sensitivity of 26,845 kPa–1 within 400 kPa, rapid response/recovery times of 5 ms/6 ms, outstanding durability over 10,000 loading cycles, and intrinsic flame retardancy. These distinctive capabilities allow monitoring of subtle physiological signals and complex human motions even under harsh conditions. This bioinspired approach enables the development of advanced flexible pressure sensors, thereby paving the way for advancements in adaptive robotics, intelligent wearables, and advanced healthcare diagnostics.
期刊介绍:
ACS Sensors is a peer-reviewed research journal that focuses on the dissemination of new and original knowledge in the field of sensor science, particularly those that selectively sense chemical or biological species or processes. The journal covers a broad range of topics, including but not limited to biosensors, chemical sensors, gas sensors, intracellular sensors, single molecule sensors, cell chips, and microfluidic devices. It aims to publish articles that address conceptual advances in sensing technology applicable to various types of analytes or application papers that report on the use of existing sensing concepts in new ways or for new analytes.