水动力控制的河岸沉积物中有机磷的非生物循环。

IF 11.3 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL
Guoqiang Zhao*, , , Cai Li, , , Jianyan Wang, , , Qunqun Liu, , , Chongsen Duan, , , Jikang You, , , Fei Liu, , and , Huacheng Xu*, 
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引用次数: 0

摘要

有机磷(OP)是沉积物中主要的磷库,可转化为生物可利用的磷酸盐。尽管生物活性被认为是OP去磷酸化的主要驱动因素,但氧化还原振荡下的非生物机制仍未得到解释。在这里,我们证明了水文扰动驱动的氧化还原波动可以介导op中的非生物磷酸盐释放。通过实验室模拟和对天然河岸沉积物的分析,我们证明了活性氧(ROS)的暗生产对这一过程至关重要。羟基自由基(•OH)介导的氧化是主要的去磷酸化途径,超氧化物(O2•-)和过氧化氢(H2O2)是关键的中间体。氧化还原振荡增强沉积OP进入溶解相的动员,从而加速其ros介导的去磷酸化。对天然沉积物的研究证实,氧化还原振荡过程中产生的ROS驱动非生物OP矿化,反应速率受沉积物电子交换容量和铁形态控制。这些结果揭示了一个以前未被认识到的OP转化的非生物途径,该途径与酶水解、光降解和矿物催化降解一起作用。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Hydrodynamically Controlled Abiotic Recycling of Organic Phosphorus in Riparian Sediments

Hydrodynamically Controlled Abiotic Recycling of Organic Phosphorus in Riparian Sediments

Organic phosphorus (OP), a major phosphorus pool in sediments, can be converted into bioavailable phosphate. Although biological activity is considered the primary driver of OP dephosphorylation, the abiotic mechanism under redox oscillations remains unexplained. Here, we show that hydrological perturbation-driven redox fluctuations can mediate abiotic phosphate release from OP. Through laboratory simulations and analyses of natural riparian sediments, we demonstrate that the dark production of reactive oxygen species (ROS) is essential for this process. Hydroxyl radical (OH)-mediated oxidation emerges as the dominant dephosphorylation pathway, with superoxide (O2•-) and hydrogen peroxide (H2O2) acting as key intermediates. Redox oscillations enhance the mobilization of sedimentary OP into the dissolved phase, thereby accelerating its ROS-mediated dephosphorylation. Investigations of natural sediments confirm that ROS produced during redox oscillations drive abiotic OP mineralization, with reaction rates controlled by sediment electron-exchange capacity and iron speciation. These results reveal a previously unrecognized abiotic pathway for OP transformation that operates alongside enzymatic hydrolysis, photodegradation, and mineral-catalyzed degradation.

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来源期刊
环境科学与技术
环境科学与技术 环境科学-工程:环境
CiteScore
17.50
自引率
9.60%
发文量
12359
审稿时长
2.8 months
期刊介绍: Environmental Science & Technology (ES&T) is a co-sponsored academic and technical magazine by the Hubei Provincial Environmental Protection Bureau and the Hubei Provincial Academy of Environmental Sciences. Environmental Science & Technology (ES&T) holds the status of Chinese core journals, scientific papers source journals of China, Chinese Science Citation Database source journals, and Chinese Academic Journal Comprehensive Evaluation Database source journals. This publication focuses on the academic field of environmental protection, featuring articles related to environmental protection and technical advancements.
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