燃料电池催化微环境改性研究进展

IF 7.4 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Shuqi Yu  (, ), Yao Wang  (, ), Zidong Wei  (, )
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引用次数: 0

摘要

氢燃料电池以其高能量转换效率和零碳排放在解决能源危机和环境污染方面发挥着至关重要的作用,当氢来自可再生能源供电的电解水。反应的核心在于催化反应界面。在这个界面上,催化剂、水环境、离子种类和离聚物之间的复杂相互作用直接决定了催化反应的效率。本文系统总结了催化剂的吸附行为、界面水动力学、离子修饰和离子-电极相互作用等四个关键界面影响因素。对催化剂工程、界面水结构优化、离子基功能化和界面强化等关键调控策略进行了深入总结。提出了未来的发展方向,重点是原位表征、多相界面工程、非贵金属催化剂耐久性增强和机器学习驱动的多尺度建模,旨在使燃料电池成为可持续能源系统的基石。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Recent achievements on the modification of microenvironment for fuel cell catalysis

Hydrogen fuel cells with high energy conversion efficiency and zero carbon emissions play a critical role in addressing energy crises and environmental pollution, when the hydrogen is derived from renewable energy-powered water electrolysis. The core of the reaction lies in the catalytic reaction interface. At this interface, the complex interactions among catalysts, aqueous environments, ion species, and ionomers directly determine the efficiency of the catalytic reaction. This review systematically summarized four key interfacial influencing factors, including adsorption behavior of catalysts, interfacial water dynamics, ion modification, and ionomer-electrode interactions. It provided an in-depth summary of key regulation strategies such as catalyst engineering, interfacial water structure optimization, ionic group functionalization, and interface reinforcement. Furthermore, future development directions are proposed, focusing on in-situ characterization, multiphase interface engineering, durability enhancement of non-precious metal catalysts, and machine learning-driven multiscale modeling, aiming to establish fuel cells as a cornerstone of sustainable energy systems.

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来源期刊
Science China Materials
Science China Materials Materials Science-General Materials Science
CiteScore
11.40
自引率
7.40%
发文量
949
期刊介绍: Science China Materials (SCM) is a globally peer-reviewed journal that covers all facets of materials science. It is supervised by the Chinese Academy of Sciences and co-sponsored by the Chinese Academy of Sciences and the National Natural Science Foundation of China. The journal is jointly published monthly in both printed and electronic forms by Science China Press and Springer. The aim of SCM is to encourage communication of high-quality, innovative research results at the cutting-edge interface of materials science with chemistry, physics, biology, and engineering. It focuses on breakthroughs from around the world and aims to become a world-leading academic journal for materials science.
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