{"title":"利用荧光定位技术对硅中单G中心进行纳米定位和原位增强","authors":"Yu-Hang Ma, Nai-Jie Guo, Wei Liu, Xiao-Dong Zeng, Lin-Ke Xie, Jun-You Liu, Ya-Qi Wu, Yi-Tao Wang, Zhao-An Wang, Jia-Ming Ren, Chun Ao, Haifei Lu, Jian-Shun Tang*, Chuan-Feng Li* and Guang-Can Guo, ","doi":"10.1021/acsphotonics.5c01247","DOIUrl":null,"url":null,"abstract":"<p >Silicon-based semiconductor nanofabrication technology has achieved a remarkable level of sophistication and maturity, and color centers in silicon naturally inherit this advantage. Besides, their emissions appear in telecommunication bands, which makes them play a crucial role in the construction of a quantum network. To address the challenge of weak spontaneous emission, different optical cavities are fabricated to enhance the emission rate. However, the relative location between cavity and emitter is random, which greatly reduces the success probability of enhancement. Here, we report on a fluorescence-localization technique (FLT) for precisely locating a single G center in silicon and embedding it in the center of a circular Bragg grating cavity in situ, achieving 240-times improvement of the success probability. We observe a 30-fold enhancement of luminescence, 2.5-fold acceleration of the emission from a single G center, corresponding to a Purcell factor exceeding 11. Our findings pave the way for large-scale integration of quantum light sources.</p>","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"12 9","pages":"5240–5247"},"PeriodicalIF":6.7000,"publicationDate":"2025-08-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Nanoscale Positioning and In Situ Enhancement of Single G Center in Silicon Using a Fluorescence-Localization Technique\",\"authors\":\"Yu-Hang Ma, Nai-Jie Guo, Wei Liu, Xiao-Dong Zeng, Lin-Ke Xie, Jun-You Liu, Ya-Qi Wu, Yi-Tao Wang, Zhao-An Wang, Jia-Ming Ren, Chun Ao, Haifei Lu, Jian-Shun Tang*, Chuan-Feng Li* and Guang-Can Guo, \",\"doi\":\"10.1021/acsphotonics.5c01247\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Silicon-based semiconductor nanofabrication technology has achieved a remarkable level of sophistication and maturity, and color centers in silicon naturally inherit this advantage. Besides, their emissions appear in telecommunication bands, which makes them play a crucial role in the construction of a quantum network. To address the challenge of weak spontaneous emission, different optical cavities are fabricated to enhance the emission rate. However, the relative location between cavity and emitter is random, which greatly reduces the success probability of enhancement. Here, we report on a fluorescence-localization technique (FLT) for precisely locating a single G center in silicon and embedding it in the center of a circular Bragg grating cavity in situ, achieving 240-times improvement of the success probability. We observe a 30-fold enhancement of luminescence, 2.5-fold acceleration of the emission from a single G center, corresponding to a Purcell factor exceeding 11. Our findings pave the way for large-scale integration of quantum light sources.</p>\",\"PeriodicalId\":23,\"journal\":{\"name\":\"ACS Photonics\",\"volume\":\"12 9\",\"pages\":\"5240–5247\"},\"PeriodicalIF\":6.7000,\"publicationDate\":\"2025-08-29\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Photonics\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsphotonics.5c01247\",\"RegionNum\":1,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Photonics","FirstCategoryId":"101","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsphotonics.5c01247","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Nanoscale Positioning and In Situ Enhancement of Single G Center in Silicon Using a Fluorescence-Localization Technique
Silicon-based semiconductor nanofabrication technology has achieved a remarkable level of sophistication and maturity, and color centers in silicon naturally inherit this advantage. Besides, their emissions appear in telecommunication bands, which makes them play a crucial role in the construction of a quantum network. To address the challenge of weak spontaneous emission, different optical cavities are fabricated to enhance the emission rate. However, the relative location between cavity and emitter is random, which greatly reduces the success probability of enhancement. Here, we report on a fluorescence-localization technique (FLT) for precisely locating a single G center in silicon and embedding it in the center of a circular Bragg grating cavity in situ, achieving 240-times improvement of the success probability. We observe a 30-fold enhancement of luminescence, 2.5-fold acceleration of the emission from a single G center, corresponding to a Purcell factor exceeding 11. Our findings pave the way for large-scale integration of quantum light sources.
期刊介绍:
Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.