金属衬底上Ge光栅/SrTiO3 /VO2混合元结构的角度稳健和可调谐中红外吸收

IF 3.3 3区 化学 Q2 CHEMISTRY, INORGANIC & NUCLEAR
Xin Cui, Yangyang Dai, Fenglin Xian, Liming Qian and Gaige Zheng
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引用次数: 0

摘要

我们提出了一种动态可调且角度鲁棒的中红外吸收器,该吸收器基于由顶层Ge光栅、超薄SrTiO3极性介电层、热致变色VO2薄膜和金属衬底组成的混合元结构。系统的光学响应采用严格的耦合波分析(RCWA)建模,揭示了在横磁(TM)极化下宽入射角(0°-80°)范围内的宽带和高效吸收。吸收行为受多种共振机制的相互作用控制,包括Ge光栅中的引导模共振(GMR), \ce{SrTiO3}层中的声子-极化子\textcolor{red}{(PhP)}激发,以及绝缘VO2促进的类腔模式。通过改变光栅周期(p=6-10 μm)、填充系数(f=0.4-0.7)以及SrTiO3和VO2的厚度等结构参数,绘制出优化性能的设计空间。数值结果证实了强场约束和模式杂化对观察到的角稳定性和可调性的影响。该理论框架为设计具有热调制、可重构光学和红外光子电路应用潜力的有源中红外元结构提供了重要见解。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Angle-robust and tunable mid-infrared absorption in a Ge grating/SrTiO3/VO2 hybrid metastructure on a metallic substrate

Angle-robust and tunable mid-infrared absorption in a Ge grating/SrTiO3/VO2 hybrid metastructure on a metallic substrate

We propose a dynamically tunable and angle-robust mid-infrared (mid-IR) absorber based on a hybrid metastructure composed of a top-layer Ge grating, an ultrathin SrTiO3 polar dielectric layer, a thermochromic VO2 film, and a metallic substrate. The optical response of the system is modeled using rigorous coupled-wave analysis (RCWA), revealing broadband and high-efficiency absorption across a wide range of incident angles (0°–80°) under transverse-magnetic (TM) polarization. The absorption behavior is governed by the interplay of multiple resonant mechanisms, including guided-mode resonance (GMR) in the Ge grating, phonon–polariton (PhP) excitation in the SrTiO3 layer, and cavity-like modes facilitated by the insulating VO2. By varying structural parameters such as the grating period (p = 6–10 μm), fill factor (f = 0.4–0.7), and the thicknesses of SrTiO3 and VO2, we map the design space for optimized performance. Numerical results confirm that strong field confinement and mode hybridization are responsible for the observed angular stability and tunability. This theoretical framework provides critical insights for the design of active mid-IR metastructures with application potential in thermal modulation, reconfigurable optics, and infrared photonic circuitry.

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来源期刊
Dalton Transactions
Dalton Transactions 化学-无机化学与核化学
CiteScore
6.60
自引率
7.50%
发文量
1832
审稿时长
1.5 months
期刊介绍: Dalton Transactions is a journal for all areas of inorganic chemistry, which encompasses the organometallic, bioinorganic and materials chemistry of the elements, with applications including synthesis, catalysis, energy conversion/storage, electrical devices and medicine. Dalton Transactions welcomes high-quality, original submissions in all of these areas and more, where the advancement of knowledge in inorganic chemistry is significant.
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