{"title":"动态CO2电还原过程中Cu(100)的表面修饰与选择性的联系","authors":"","doi":"10.1038/s41929-025-01403-9","DOIUrl":null,"url":null,"abstract":"The response of a well-defined Cu pre-catalyst surface to dynamic pulsed electrocatalytic CO2 reduction conditions is unveiled using a correlated spatially resolved spectro-microscopy approach. The observed structural changes are key to understanding the increased selectivity towards ethanol and ethylene under these conditions.","PeriodicalId":18845,"journal":{"name":"Nature Catalysis","volume":"8 9","pages":"870-871"},"PeriodicalIF":44.6000,"publicationDate":"2025-08-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Linking surface modifications of Cu(100) to selectivity during dynamic CO2 electroreduction\",\"authors\":\"\",\"doi\":\"10.1038/s41929-025-01403-9\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The response of a well-defined Cu pre-catalyst surface to dynamic pulsed electrocatalytic CO2 reduction conditions is unveiled using a correlated spatially resolved spectro-microscopy approach. The observed structural changes are key to understanding the increased selectivity towards ethanol and ethylene under these conditions.\",\"PeriodicalId\":18845,\"journal\":{\"name\":\"Nature Catalysis\",\"volume\":\"8 9\",\"pages\":\"870-871\"},\"PeriodicalIF\":44.6000,\"publicationDate\":\"2025-08-25\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nature Catalysis\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.nature.com/articles/s41929-025-01403-9\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nature Catalysis","FirstCategoryId":"92","ListUrlMain":"https://www.nature.com/articles/s41929-025-01403-9","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Linking surface modifications of Cu(100) to selectivity during dynamic CO2 electroreduction
The response of a well-defined Cu pre-catalyst surface to dynamic pulsed electrocatalytic CO2 reduction conditions is unveiled using a correlated spatially resolved spectro-microscopy approach. The observed structural changes are key to understanding the increased selectivity towards ethanol and ethylene under these conditions.
期刊介绍:
Nature Catalysis serves as a platform for researchers across chemistry and related fields, focusing on homogeneous catalysis, heterogeneous catalysis, and biocatalysts, encompassing both fundamental and applied studies. With a particular emphasis on advancing sustainable industries and processes, the journal provides comprehensive coverage of catalysis research, appealing to scientists, engineers, and researchers in academia and industry.
Maintaining the high standards of the Nature brand, Nature Catalysis boasts a dedicated team of professional editors, rigorous peer-review processes, and swift publication times, ensuring editorial independence and quality. The journal publishes work spanning heterogeneous catalysis, homogeneous catalysis, and biocatalysis, covering areas such as catalytic synthesis, mechanisms, characterization, computational studies, nanoparticle catalysis, electrocatalysis, photocatalysis, environmental catalysis, asymmetric catalysis, and various forms of organocatalysis.