Shangwei Zhou , Wenjia Du , Bastian Mager , Paul R. Shearing , Thomas S. Miller , Rhodri Jervis
{"title":"1秒内批量诊断电池","authors":"Shangwei Zhou , Wenjia Du , Bastian Mager , Paul R. Shearing , Thomas S. Miller , Rhodri Jervis","doi":"10.1016/j.joule.2025.102099","DOIUrl":null,"url":null,"abstract":"<div><div>As demand grows for scalable and sustainable energy storage, fast and affordable diagnostics are urgently needed, especially for factory-level cell sorting and second-life assessments. Electrochemical impedance spectroscopy (EIS) is widely used but remains too slow, complex, and costly for large-scale use. This work introduces a multi-channel and multi-frequency electrical excitation response (MMER) technique that captures comparable impedance-related information at a fraction of the time and cost. MMER can diagnose entire battery modules in 1 s, regardless of cell count. It uses a binary multi-frequency excitation signal, implemented on simple hardware such as programmable logic devices. Unlike EIS, MMER avoids frequency-domain transformation and impedance fitting. Instead, it compares raw voltage responses under a shared excitation current to reveal performance variations. Experiments show MMER tracks cell health in line with EIS while reducing test time by over 99%. It supports real-time diagnostics even during high-rate cycling and extends to other electrochemical systems.</div></div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"9 9","pages":"Article 102099"},"PeriodicalIF":35.4000,"publicationDate":"2025-09-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Batch diagnosis of batteries within one second\",\"authors\":\"Shangwei Zhou , Wenjia Du , Bastian Mager , Paul R. Shearing , Thomas S. Miller , Rhodri Jervis\",\"doi\":\"10.1016/j.joule.2025.102099\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>As demand grows for scalable and sustainable energy storage, fast and affordable diagnostics are urgently needed, especially for factory-level cell sorting and second-life assessments. Electrochemical impedance spectroscopy (EIS) is widely used but remains too slow, complex, and costly for large-scale use. This work introduces a multi-channel and multi-frequency electrical excitation response (MMER) technique that captures comparable impedance-related information at a fraction of the time and cost. MMER can diagnose entire battery modules in 1 s, regardless of cell count. It uses a binary multi-frequency excitation signal, implemented on simple hardware such as programmable logic devices. Unlike EIS, MMER avoids frequency-domain transformation and impedance fitting. Instead, it compares raw voltage responses under a shared excitation current to reveal performance variations. Experiments show MMER tracks cell health in line with EIS while reducing test time by over 99%. It supports real-time diagnostics even during high-rate cycling and extends to other electrochemical systems.</div></div>\",\"PeriodicalId\":343,\"journal\":{\"name\":\"Joule\",\"volume\":\"9 9\",\"pages\":\"Article 102099\"},\"PeriodicalIF\":35.4000,\"publicationDate\":\"2025-09-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Joule\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2542435125002806\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Joule","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2542435125002806","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
As demand grows for scalable and sustainable energy storage, fast and affordable diagnostics are urgently needed, especially for factory-level cell sorting and second-life assessments. Electrochemical impedance spectroscopy (EIS) is widely used but remains too slow, complex, and costly for large-scale use. This work introduces a multi-channel and multi-frequency electrical excitation response (MMER) technique that captures comparable impedance-related information at a fraction of the time and cost. MMER can diagnose entire battery modules in 1 s, regardless of cell count. It uses a binary multi-frequency excitation signal, implemented on simple hardware such as programmable logic devices. Unlike EIS, MMER avoids frequency-domain transformation and impedance fitting. Instead, it compares raw voltage responses under a shared excitation current to reveal performance variations. Experiments show MMER tracks cell health in line with EIS while reducing test time by over 99%. It supports real-time diagnostics even during high-rate cycling and extends to other electrochemical systems.
期刊介绍:
Joule is a sister journal to Cell that focuses on research, analysis, and ideas related to sustainable energy. It aims to address the global challenge of the need for more sustainable energy solutions. Joule is a forward-looking journal that bridges disciplines and scales of energy research. It connects researchers and analysts working on scientific, technical, economic, policy, and social challenges related to sustainable energy. The journal covers a wide range of energy research, from fundamental laboratory studies on energy conversion and storage to global-level analysis. Joule aims to highlight and amplify the implications, challenges, and opportunities of novel energy research for different groups in the field.