质子束辐照下Cr、Si、Mg共掺Al2O3陶瓷板的热释光性能

IF 3.6 3区 物理与天体物理 Q2 OPTICS
Ayano Okubo , Yutaro Mori , Tomonori Isobe , Takeji Sakae , Yusuke Koba , Weishan Chang , Kiyomitsu Shinsho
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引用次数: 0

摘要

本研究评估了Cr、Si和Mg共掺杂Al2O3 (Al2O3:Cr、Si、Mg)陶瓷板在200 MeV质子束照射下的热释光(TL)性能,旨在评估其在质子治疗中的高分辨率二维剂量学潜力。光谱测量显示,在693 nm处有一个主要的TL发射峰,对应于Cr3+离子2E→4A2跃迁。无论剂量和线性能量转移(LET)如何,发光曲线的峰值温度和形状都是一致的,这表明了陷阱和复合中心的稳定性。TL响应与吸收剂量呈良好的线性关系,与电离室测量值在±1.5%范围内一致,对LET的依赖性最小。此外,使用大面积(200 mm × 200 mm) TL陶瓷板获得二维剂量分布图。TL成像测量的离轴比和百分比深度剂量分布与标准剂量计测量结果吻合较好(±1 ~ 6%),空间分辨率达到156 μm。这些结果表明,Al2O3:Cr,Si,Mg陶瓷适用于精确,可重复使用和高分辨率的质子剂量测定,为粒子治疗的质量保证提供了传统的基于薄膜或电离的探测器的有希望的替代方案。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Thermoluminescence properties of Cr, Si, and Mg co-doped Al2O3 ceramics plates under proton beam irradiation
This study evaluates the thermoluminescence (TL) properties of Cr, Si, and Mg co-doped Al2O3 (Al2O3:Cr,Si,Mg) ceramic plates under 200 MeV proton beam irradiation, aiming to assess their potential for high-resolution two-dimensional dosimetry in proton therapy. Spectral measurements revealed a dominant TL emission peak at 693 nm, corresponding to the 2E → 4A2 transition of Cr3+ ions. The glow curves exhibited consistent peak temperature and shape regardless of dose and linear energy transfer (LET), indicating the stability of the trap and recombination centers. The TL response showed excellent linearity with absorbed dose, agreeing within ±1.5 % with ionization chamber measurements, and demonstrated minimal dependence on LET. Furthermore, large-area (200 mm × 200 mm) TL ceramic plates were used to obtain two-dimensional dose distribution maps. The off-axis ratio and percent depth dose distributions measured using TL imaging were in good agreement (within ±1–6 %) with those obtained from standard dosimeters, and the spatial resolution reached 156 μm. These results suggest that Al2O3:Cr,Si,Mg ceramics are suitable for accurate, reusable, and high-resolution proton dosimetry, offering a promising alternative to conventional film- or ionization-based detectors for quality assurance in particle therapy.
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来源期刊
Journal of Luminescence
Journal of Luminescence 物理-光学
CiteScore
6.70
自引率
13.90%
发文量
850
审稿时长
3.8 months
期刊介绍: The purpose of the Journal of Luminescence is to provide a means of communication between scientists in different disciplines who share a common interest in the electronic excited states of molecular, ionic and covalent systems, whether crystalline, amorphous, or liquid. We invite original papers and reviews on such subjects as: exciton and polariton dynamics, dynamics of localized excited states, energy and charge transport in ordered and disordered systems, radiative and non-radiative recombination, relaxation processes, vibronic interactions in electronic excited states, photochemistry in condensed systems, excited state resonance, double resonance, spin dynamics, selective excitation spectroscopy, hole burning, coherent processes in excited states, (e.g. coherent optical transients, photon echoes, transient gratings), multiphoton processes, optical bistability, photochromism, and new techniques for the study of excited states. This list is not intended to be exhaustive. Papers in the traditional areas of optical spectroscopy (absorption, MCD, luminescence, Raman scattering) are welcome. Papers on applications (phosphors, scintillators, electro- and cathodo-luminescence, radiography, bioimaging, solar energy, energy conversion, etc.) are also welcome if they present results of scientific, rather than only technological interest. However, papers containing purely theoretical results, not related to phenomena in the excited states, as well as papers using luminescence spectroscopy to perform routine analytical chemistry or biochemistry procedures, are outside the scope of the journal. Some exceptions will be possible at the discretion of the editors.
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