综合分析主要天气型态及强影响台风路径,揭示热带气旋在何处及如何影响中国长三角地区的区域臭氧污染

IF 3.7 2区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES
Mengzhu Xi , Yi Luo , Yichen Li , Danyang Ma , Lingyun Feng , Shuxian Zhang , Shitong Chen , Min Xie
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引用次数: 0

摘要

长三角地区是典型的经济发达、人口密集的沿海城市群。在温暖季节,当热带气旋登陆时,长三角通常会受到极端天气的影响。然而,当tc离长三角不远时,长三角也会受到严重的臭氧污染。有报道称,TCs的外围流动与长三角地区的区域性O3污染有关。然而,tc的轨迹和位置,以及它们的作用机制,仍然不清楚。本研究试图通过对主要天气模式(SWPs)和高影响TC路径的综合分析,揭示TC如何以及在何处导致长三角区域的臭氧污染。天气模式方面,采用NCEP再分析资料和t型主成分分析(PCT)方法对2018 - 2021年长三角850 hPa位势高度场进行了客观分类。通过整合长三角同期大气污染观测资料和气象资料,系统分析了不同SWPs下的O3污染特征及其形成机制。同时,对TC轨迹数据进行轨迹聚类分析,探讨不同路径TC对长三角地区O3污染的作用机制。结果表明:长三角地区O3浓度总体在6月和9月达到峰值,区域O3污染通常发生在tc登陆前和tc消散后;长三角的社会福利项目可分为七类。其中SWP3和SWP4是会受到tc影响的swp,而具有相似环流情况的SWP6和SWP7则不受tc影响。在SWP3和SWP4中,tc是非常重要的天气系统。此外,基于不同SWPs下的O3污染分类和TC轨迹聚类分析,揭示了TC轨迹和中心位置对长三角区域O3污染的影响。在SWP3下,TCs的路径通常为西北转向,其中心位于(130°-135°E, 20°-30°N)区域时,对长三角地区的O3污染水平最高。西太平洋副热带高压(WPSH)所引致的下降气流及周边的低压气流使长三角上空的空气更加停滞。大气污染物的积累以及温度升高导致的化学反应更加强烈是造成区域性O3污染的主要原因。而在SWP4中,TCs一般为西进路径,当TCs位于(125°-130°E, 10°-16°N)区域时,长三角区域O3污染强度较强。由于SWP4下强tc的外围平流气流,更多的臭氧从内陆污染地区输送到长三角。长三角在SWP4下比在SWP3下由tc引起的向下气流较少。这些发现为TCs与沿海地区O3污染之间相互作用的复杂机制提供了新的视角。为沿海城市严重O3污染的预测、预警和针对性防治提供重要科学依据,为优化区域空气质量管理策略、制定更精准的污染防治措施提供重要指导。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Comprehensive analysis of prevailing weather patterns and high-impact typhoon tracks to reveal where and how tropical cyclone affects regional ozone pollution in the Yangtze River Delta region, China
The Yangtze River Delta (YRD) region is a typical economically developed and densely populated coastal city cluster. During warm seasons, the YRD generally suffers from extreme weather when tropical cyclones (TCs) make landfall. However, the YRD is also affected by severe ozone (O3) pollution when TCs are not far away. It has been reported that the peripheral flow of TCs is related to the regional O3 pollution over the YRD. Nevertheless, the tracks and locations of TCs, as well as the mechanisms of their effects, are still unclear. This study tries to reveal how and where TCs cause regional O3 pollution in the YRD based on a comprehensive analysis of prevailing synoptic weather patterns (SWPs) and high-impact TC tracks. For weather patterns, the NCEP reanalysis data and the Principal Component Analysis in T-mode (PCT) analysis method were adopted to objectively classify the 850 hPa geopotential height field in the YRD from 2018 to 2021. By integrating the air pollution observation data and the meteorological data in the YRD of the same period, a systematic analysis of the O3 pollution characteristics and their formation mechanism under different SWPs was conducted. Meanwhile, trajectory clustering analysis was conducted on TC track data to investigate the mechanisms of TCs with different paths on O3 pollution in the YRD. The results indicate that O3 concentration in the YRD generally peaks in June and September, and regional O3 pollution usually occurs before TCs land and after TCs dissipate. The SWPs in the YRD can be categorized into seven categories. Among them, SWP3 and SWP4 are SWPs that will be affected by TCs, while SWP6 and SWP7, which have similar circulation situations, are not affected by TCs. TCs are very important weather systems in SWP3 and SWP4. Furthermore, based on O3 pollution classification under different SWPs and TC track clustering analysis, how TC trajectories and central locations affect regional O3 pollution over the YRD is revealed. Under SWP3, TCs usually have the northwest-turning track, and cause the highest O3 pollution levels in the YRD when their centers are located in the area of (130°–135°E, 20°–30°N). Downdrafts caused by western Pacific subtropical high (WPSH) and the peripheral downward airflows of TCs make the air more stagnant over the YRD. The accumulation of air pollutants, as well as more intensive chemical reactions due to higher temperature, are the main cause of regional O3 pollution. For SWP4, however, TCs generally have the westward track, and regional O3 pollution in the YRD occurs when TCs are located over the area of (125°–130°E, 10°–16°N) with stronger intensities. More O3 is transported from inland polluted areas to the YRD due to the peripheral advection airflows of the strong TCs under SWP4. There are fewer downward airflows caused by TCs when the YRD is under SWP4 than under SWP3. These findings provide a new perspective on the intricate mechanisms underlying the interactions between TCs and coastal region O3 pollution. They also provide an important scientific basis for the prediction, early warning, and targeted prevention and control of severe O3 pollution in coastal cities, while also offering crucial guidance for optimizing regional air quality management strategies and formulating more precise pollution prevention and control measures.
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来源期刊
Atmospheric Environment
Atmospheric Environment 环境科学-环境科学
CiteScore
9.40
自引率
8.00%
发文量
458
审稿时长
53 days
期刊介绍: Atmospheric Environment has an open access mirror journal Atmospheric Environment: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review. Atmospheric Environment is the international journal for scientists in different disciplines related to atmospheric composition and its impacts. The journal publishes scientific articles with atmospheric relevance of emissions and depositions of gaseous and particulate compounds, chemical processes and physical effects in the atmosphere, as well as impacts of the changing atmospheric composition on human health, air quality, climate change, and ecosystems.
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