在圣母大学生产加速器质谱236U参考标准

IF 1.4 3区 物理与天体物理 Q3 INSTRUMENTS & INSTRUMENTATION
T.L. Bailey , N. Cabanas , I. Russell , D. Lund , G. Mulcahy , C. Bacall , R. Cox , C.J. Dye , W. Peeler , F. Rivero , P. Collon
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引用次数: 0

摘要

236U是铀的稀有同位素,自然存在于矿石中,丰度为236U/238U<;1×10−9。探测它和测量同位素比率的能力的应用范围从核取证和防扩散到能源生产和环境保护。目前,加速器质谱法(AMS)是唯一一种足够灵敏的技术,可以准确测量236U/238U同位素比,因为它们存在于天然矿石中,范围为236U/238U=10−12−10−9。一些医疗辅助队的设施已经证明有能力进行这些测量。从历史上看,由于缺乏涵盖自然发生的236U/238U丰度范围的商业参考标准,因此需要使用绝对测量,而使用AMS是出了名的困难,导致测量的不确定性增加,并且依赖于系统效应的知识。为减轻这些问题,医疗辅助队各设施已制订各自的参考标准。利用为其他形式的质谱法准备的参考标准品,通过低本底天然铀的稀释,建立了一系列适合的AMS标准品。将讨论用于生产和表征这些材料的技术以及使用AMS对它们进行分析。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Producing 236U reference standards for Accelerator Mass Spectrometry at the University of Notre Dame
236U is a rare isotope of uranium, naturally occurring in ores with an abundance of 236U/238U<1×109. The ability to detect it and make isotopic ratio measurements has applications ranging from nuclear forensics and nonproliferation to energy production and environmental protection. Currently, Accelerator Mass Spectrometry (AMS) is the only technique sensitive enough to accurately measure 236U/238U isotopic ratios as they exist in naturally occurring ores in the range of 236U/238U=1012109. Some AMS facilities have demonstrated their capabilities to make these measurements. Historically, the lack of commercially available reference standards covering the range of naturally occurring 236U/238U abundances has necessitated the use of absolute measurements, notoriously difficult to do using AMS, resulting in increased uncertainties in measurements and a reliance on knowledge of systematic effects. To mitigate these issues, various AMS facilities have sought to develop their own reference standards. Using a reference standard prepared for other forms of mass spectrometry, a series of AMS suitable standards was created through dilution with low-background natural uranium. The techniques used to produce and characterize these materials as well as analysis of them using AMS will be discussed.
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来源期刊
CiteScore
2.80
自引率
7.70%
发文量
231
审稿时长
1.9 months
期刊介绍: Section B of Nuclear Instruments and Methods in Physics Research covers all aspects of the interaction of energetic beams with atoms, molecules and aggregate forms of matter. This includes ion beam analysis and ion beam modification of materials as well as basic data of importance for these studies. Topics of general interest include: atomic collisions in solids, particle channelling, all aspects of collision cascades, the modification of materials by energetic beams, ion implantation, irradiation - induced changes in materials, the physics and chemistry of beam interactions and the analysis of materials by all forms of energetic radiation. Modification by ion, laser and electron beams for the study of electronic materials, metals, ceramics, insulators, polymers and other important and new materials systems are included. Related studies, such as the application of ion beam analysis to biological, archaeological and geological samples as well as applications to solve problems in planetary science are also welcome. Energetic beams of interest include atomic and molecular ions, neutrons, positrons and muons, plasmas directed at surfaces, electron and photon beams, including laser treated surfaces and studies of solids by photon radiation from rotating anodes, synchrotrons, etc. In addition, the interaction between various forms of radiation and radiation-induced deposition processes are relevant.
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