基于多层优化微腔量子点随机激光器的杂化等离子体耦合

IF 3.6 3区 物理与天体物理 Q2 OPTICS
Muhammad Ali Khan , Naeem Iqbal , Siqi Chang , Gohar Aziz , Junhua Tong , Xiaoyu Shi , Zhiyang Xu , Xiaomei Gao , Anwer Hayat , Tianrui Zhai
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引用次数: 0

摘要

由于效率低,基于随机激光的器件的发展仍然是一个关键的挑战。本文研究了以银纳米粒子和量子点为散射介质和增益介质的多层随机激光腔在镀银玻璃基板上的性能。聚乙烯醇作为增益和散射之间的间隔层,使等离子体激子耦合的工程;其厚度变化对聚二甲基硅氧烷(PDMS)保护层下的激光阈值和斜率效率有显著影响。当间隔层厚度从0 nm变化到137 nm时,RL波长从~ 636.5 nm红移到~ 645.4 nm,这是由于在等离子体-激子相互作用的影响下,有效折射率的变化也增强了辐射复合。最佳间隔层厚度为105 nm有助于将阈值降低到20 μJ/cm2,强调了混合等离子体耦合下能量约束和激光效率的改善。随机激光光谱的幂傅里叶变换分析辅助了该方法。这些发现为在先进光子应用中开发波长选择性等离子体-激子混合激光系统提供了一个紧凑的策略。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Hybrid plasmonic coupling through multilayer optimum microcavity based quantum dots random laser
The development of random laser-based devices remains a key challenge due to their low efficiency. This study investigates the performance of multilayered random laser cavities encompassing silver nanoparticles and quantum dots as scatters and gain mediums respectively on silver film coated glass substrate. Polyvinyl alcohol as a spacer layer between gain and scatters enables the engineering of plasmon–exciton couplings; its thickness variation significantly influences the lasing threshold and slope efficiency under protective coating of Polydimethylsiloxane (PDMS). RL wavelength is red shifted from 636.5 nm to 645.4 nm under variation of spacer thickness from 0 nm to 137 nm attributed to variation in effective refractive index under the influence of plasmon–exciton interaction which enhanced radiative recombination as well. An optimal spacer thickness of 105 nm assisted in lowering the threshold value to 20 μJ/cm2, underscoring improved energy confinement and lasing efficiency under hybrid plasmonic coupling. The power Fourier transform analysis of the random lasing spectra assisted the presented approach. These findings provide a compact strategy for developing wavelength-selective plasmon–exciton hybrid lasing systems in advanced photonic applications.
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来源期刊
Journal of Luminescence
Journal of Luminescence 物理-光学
CiteScore
6.70
自引率
13.90%
发文量
850
审稿时长
3.8 months
期刊介绍: The purpose of the Journal of Luminescence is to provide a means of communication between scientists in different disciplines who share a common interest in the electronic excited states of molecular, ionic and covalent systems, whether crystalline, amorphous, or liquid. We invite original papers and reviews on such subjects as: exciton and polariton dynamics, dynamics of localized excited states, energy and charge transport in ordered and disordered systems, radiative and non-radiative recombination, relaxation processes, vibronic interactions in electronic excited states, photochemistry in condensed systems, excited state resonance, double resonance, spin dynamics, selective excitation spectroscopy, hole burning, coherent processes in excited states, (e.g. coherent optical transients, photon echoes, transient gratings), multiphoton processes, optical bistability, photochromism, and new techniques for the study of excited states. This list is not intended to be exhaustive. Papers in the traditional areas of optical spectroscopy (absorption, MCD, luminescence, Raman scattering) are welcome. Papers on applications (phosphors, scintillators, electro- and cathodo-luminescence, radiography, bioimaging, solar energy, energy conversion, etc.) are also welcome if they present results of scientific, rather than only technological interest. However, papers containing purely theoretical results, not related to phenomena in the excited states, as well as papers using luminescence spectroscopy to perform routine analytical chemistry or biochemistry procedures, are outside the scope of the journal. Some exceptions will be possible at the discretion of the editors.
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