双通道AsH3供气和H2载气流速变化下金属-有机化学气相沉积InAs/GaAs量子点的生长行为

IF 3.4 2区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
HoSung Kim, Mireu Lee, Dae-Myeong Geum* and Young-Ho Ko*, 
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引用次数: 0

摘要

在这项研究中,我们全面研究了双通道砷(AsH3)供应和不同的氢(H2)载气流速对金属有机气相沉积(MOCVD)中InAs/GaAs量子点(QDs)生长的影响。与传统的单通道配置相比,双通道AsH3供应的实施导致了更稳定和均匀的QD增长,主要是由于V/III比的突然变化。此外,研究发现H2流速对量子点尺寸分布和光学性能起着关键作用。值得注意的是,在中等H2流量为100 sccm时,量子点尺寸均匀性增强,光致发光(PL)强度增强。这些发现为在MOCVD生长过程中通过精确控制AsH3供应配置和H2载气流量来获得高质量的InAs/GaAs量子点提供了有价值的见解。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Growth Behaviors of InAs/GaAs Quantum Dots Using Metal–Organic Chemical Vapor Deposition with Dual-Channel AsH3 Supply and H2 Carrier Gas Flow Rate Variation

Growth Behaviors of InAs/GaAs Quantum Dots Using Metal–Organic Chemical Vapor Deposition with Dual-Channel AsH3 Supply and H2 Carrier Gas Flow Rate Variation

In this study, we conducted a comprehensive investigation into the effects of a dual-channel arsine (AsH3) supply and varying hydrogen (H2) carrier gas flow rates on the growth of InAs/GaAs quantum dots (QDs) via metal–organic vapor deposition (MOCVD). The implementation of a dual-channel AsH3 supply resulted in more stable and uniform QD growth compared with the conventional single-channel configuration, primarily due to the abrupt change in the V/III ratio. Moreover, the H2 flow rate was found to play a critical role in determining the QD size distribution and optical performance. Notably, at a moderate H2 flow rate of 100 sccm, enhanced QD size uniformity and increased photoluminescence (PL) intensity were observed. These findings provide valuable insights into achieving high-quality InAs/GaAs QDs through precise control of the AsH3 supply configuration and H2 carrier gas flow during the MOCVD growth process.

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来源期刊
Crystal Growth & Design
Crystal Growth & Design 化学-材料科学:综合
CiteScore
6.30
自引率
10.50%
发文量
650
审稿时长
1.9 months
期刊介绍: The aim of Crystal Growth & Design is to stimulate crossfertilization of knowledge among scientists and engineers working in the fields of crystal growth, crystal engineering, and the industrial application of crystalline materials. Crystal Growth & Design publishes theoretical and experimental studies of the physical, chemical, and biological phenomena and processes related to the design, growth, and application of crystalline materials. Synergistic approaches originating from different disciplines and technologies and integrating the fields of crystal growth, crystal engineering, intermolecular interactions, and industrial application are encouraged.
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