[赣西某矿区土壤重金属污染特征、来源分析及健康风险评价]。

Q2 Environmental Science
Fen Hu, Lie Jiang, Qiao-Hong Chen, Bao-Nan He
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引用次数: 0

摘要

探讨赣西附近某煤矿集中区土壤重金属污染特征、来源及可能的人体健康风险。采用Nemerow指数法评价研究区土壤重金属污染特征,基于自组织神经网络(SOM)描述土壤重金属污染特征的相关性,采用PMF模型对土壤重金属污染进行追踪,采用EPA建立的暴露风险模型进行健康风险评价。结果表明:6种土壤重金属平均含量在0.25 ~ 47.47 mg·kg-1之间,均高于江西省土壤环境背景值;只有Cd平均值高于GB15618-2018的风险筛查值,所有重金属变异系数均较高。Nemerow污染评价表明,研究区周边土壤重金属污染严重,以As、Hg、Cd为典型代表。SOM-K聚类结果表明,Cu、Ni、Cd相关性好,Cu、As、Hg相关性强,Pb与其他元素差异明显。健康风险评价表明,手口食入是研究区土壤重金属的主要暴露途径。研究区儿童存在非致癌性和致癌性健康风险,成人存在致癌性健康风险,儿童暴露于健康风险的程度高于成人。儿童和成人综合非致癌风险指数(HI)分别为1.52E+00和2.41E-01。儿童和成人的综合致癌风险指数(TCR)分别为4.48E-05和2.85E-05。为研究区健康风险的主要贡献指标。来源分析表明,研究区土壤重金属来源受工业降尘源、自然源、煤炭污染源、交通运输源和农业生产源的影响,其贡献率分别为25.62%、22.00%、17.88%、17.84%和16.66%。主要受人为因素影响,这与研究区土壤重金属变异系数较高的结果一致。研究结果可为研究区土壤重金属污染的防治提供理论依据。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
[Pollution Characteristics, Source Analysis, and Health Risk Assessment of Heavy Metals of Soil in a Certain Coal Mining Area of Western Jiangxi Province].

To explore the pollution characteristics, sources, and possible human health risks of soil heavy metals in a coal mine concentration area near western Jiangxi. The Nemerow index method was used to evaluate the characteristics of soil heavy metal pollution in the study area, the correlation of soil heavy metal pollution characteristics was described based on a self-organizing neural network (SOM), the PMF model was used to trace the soil heavy metal pollution, and the exposure risk model established by EPA was used for health risk assessment. The results showed that the average content of heavy metals in the six soils ranged from 0.25 to 47.47 mg·kg-1, which were all higher than the soil environmental background value in Jiangxi Province. Only the mean Cd content was higher than the risk screening value in GB15618-2018, and all heavy metal coefficients of variation were relatively high. The Nemerow pollution assessment indicated that the soil around the study area was severely polluted by heavy metals, especially As, Hg, and Cd as typical representatives. SOM-K clustering showed that Cu, Ni, and Cd had good correlation; Cu, As, and Hg had strong correlation; and Pb had obvious differences with other elements. The health risk assessment showed that the hand-mouth ingestion was the main exposure route of heavy metals in soil in the study area. Children in the study area had non-carcinogenic and carcinogenic health risks, while adults had carcinogenic health risks, and children were more exposed to health risks than adults. The comprehensive non-carcinogenic risk indexes (HI) for children and adults were 1.52E+00 and 2.41E-01, respectively. Additionally, the comprehensive carcinogenic risk index (TCR) for children and adults was 4.48E-05 and 2.85E-05, respectively. As was the main contribution index of health risk in the study area. The source analysis showed that the heavy metal sources in the soil of the study area were influenced by industrial dust fall sources, natural sources, coal pollution sources, transportation sources, and agricultural production sources, and their contribution rates were 25.62%, 22.00%, 17.88%, 17.84%, and 16.66%, respectively. It was mainly affected by human factors, which was consistent with the result of the high variation coefficient of soil heavy metals in the study area. The research results can provide theoretical basis for the prevention and control of heavy metal pollution in the soil of the study area.

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环境科学
环境科学 Environmental Science-Environmental Science (all)
CiteScore
4.40
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0.00%
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15329
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