Siyang Peng, Xuan Zheng, Sheng Li, Bin Lao, Yamin Han, Zhaoliang Liao, Hongsheng Zheng, Yumeng Yang, Tianye Yu, Peitao Liu, Yan Sun, Xing-Qiu Chen, Shouzhong Peng, Weisheng Zhao, Run-Wei Li, Zhiming Wang
{"title":"轨道霍尔效应的非常规缩放","authors":"Siyang Peng, Xuan Zheng, Sheng Li, Bin Lao, Yamin Han, Zhaoliang Liao, Hongsheng Zheng, Yumeng Yang, Tianye Yu, Peitao Liu, Yan Sun, Xing-Qiu Chen, Shouzhong Peng, Weisheng Zhao, Run-Wei Li, Zhiming Wang","doi":"10.1038/s41563-025-02326-3","DOIUrl":null,"url":null,"abstract":"<p>Orbital torque is a promising approach for electrically controlling magnetization in spintronic devices. However, unravelling the underlying mechanisms governing the orbital Hall effect (OHE), especially the role of extrinsic scattering and its scaling with conductivity (<i>σ</i><sub><i>xx</i></sub>), is crucial for realizing the full potential of orbital torque in energy-efficient spintronic devices. Here, using SrRuO<sub>3</sub> as a model system, we discover an unconventional scaling of orbital Hall conductivity (<span>\\({\\sigma }_{{\\rm{OH}}}\\)</span>) with tunable <i>σ</i><sub><i>xx</i></sub>. <span>\\({\\sigma }_{{\\rm{OH}}}\\)</span> remains constant at high <i>σ</i><sub><i>xx</i></sub> but exhibits a striking enhancement as <i>σ</i><sub><i>xx</i></sub> decreases, contrasting with spin Hall effect suppression at low <i>σ</i><sub><i>xx</i></sub>. This behaviour underscores the Dyakonov–Perel-like orbital relaxation mechanism as key to unconventional OHE. Leveraging this scaling, we achieve enhanced orbital torque via concurrent increases in orbital Hall conductivity and orbital Hall angle, demonstrating threefold power reduction in spin–orbit torque switching with moderate <i>σ</i><sub><i>xx</i></sub> reduction. Our work highlights the dominant role of extrinsic disorder scattering in unconventional OHE and establishes a transformative paradigm for energy-efficient spintronics.</p>","PeriodicalId":19058,"journal":{"name":"Nature Materials","volume":"14 1","pages":""},"PeriodicalIF":38.5000,"publicationDate":"2025-08-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Unconventional scaling of the orbital Hall effect\",\"authors\":\"Siyang Peng, Xuan Zheng, Sheng Li, Bin Lao, Yamin Han, Zhaoliang Liao, Hongsheng Zheng, Yumeng Yang, Tianye Yu, Peitao Liu, Yan Sun, Xing-Qiu Chen, Shouzhong Peng, Weisheng Zhao, Run-Wei Li, Zhiming Wang\",\"doi\":\"10.1038/s41563-025-02326-3\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Orbital torque is a promising approach for electrically controlling magnetization in spintronic devices. However, unravelling the underlying mechanisms governing the orbital Hall effect (OHE), especially the role of extrinsic scattering and its scaling with conductivity (<i>σ</i><sub><i>xx</i></sub>), is crucial for realizing the full potential of orbital torque in energy-efficient spintronic devices. Here, using SrRuO<sub>3</sub> as a model system, we discover an unconventional scaling of orbital Hall conductivity (<span>\\\\({\\\\sigma }_{{\\\\rm{OH}}}\\\\)</span>) with tunable <i>σ</i><sub><i>xx</i></sub>. <span>\\\\({\\\\sigma }_{{\\\\rm{OH}}}\\\\)</span> remains constant at high <i>σ</i><sub><i>xx</i></sub> but exhibits a striking enhancement as <i>σ</i><sub><i>xx</i></sub> decreases, contrasting with spin Hall effect suppression at low <i>σ</i><sub><i>xx</i></sub>. This behaviour underscores the Dyakonov–Perel-like orbital relaxation mechanism as key to unconventional OHE. Leveraging this scaling, we achieve enhanced orbital torque via concurrent increases in orbital Hall conductivity and orbital Hall angle, demonstrating threefold power reduction in spin–orbit torque switching with moderate <i>σ</i><sub><i>xx</i></sub> reduction. Our work highlights the dominant role of extrinsic disorder scattering in unconventional OHE and establishes a transformative paradigm for energy-efficient spintronics.</p>\",\"PeriodicalId\":19058,\"journal\":{\"name\":\"Nature Materials\",\"volume\":\"14 1\",\"pages\":\"\"},\"PeriodicalIF\":38.5000,\"publicationDate\":\"2025-08-15\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nature Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1038/s41563-025-02326-3\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nature Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1038/s41563-025-02326-3","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Orbital torque is a promising approach for electrically controlling magnetization in spintronic devices. However, unravelling the underlying mechanisms governing the orbital Hall effect (OHE), especially the role of extrinsic scattering and its scaling with conductivity (σxx), is crucial for realizing the full potential of orbital torque in energy-efficient spintronic devices. Here, using SrRuO3 as a model system, we discover an unconventional scaling of orbital Hall conductivity (\({\sigma }_{{\rm{OH}}}\)) with tunable σxx. \({\sigma }_{{\rm{OH}}}\) remains constant at high σxx but exhibits a striking enhancement as σxx decreases, contrasting with spin Hall effect suppression at low σxx. This behaviour underscores the Dyakonov–Perel-like orbital relaxation mechanism as key to unconventional OHE. Leveraging this scaling, we achieve enhanced orbital torque via concurrent increases in orbital Hall conductivity and orbital Hall angle, demonstrating threefold power reduction in spin–orbit torque switching with moderate σxx reduction. Our work highlights the dominant role of extrinsic disorder scattering in unconventional OHE and establishes a transformative paradigm for energy-efficient spintronics.
期刊介绍:
Nature Materials is a monthly multi-disciplinary journal aimed at bringing together cutting-edge research across the entire spectrum of materials science and engineering. It covers all applied and fundamental aspects of the synthesis/processing, structure/composition, properties, and performance of materials. The journal recognizes that materials research has an increasing impact on classical disciplines such as physics, chemistry, and biology.
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