Cheng Xu, Ting-Yi Chen, Chun-Pu Tsai, Dongxiao Li, Hong Zhou, Wei-Chang Li* and Chengkuo Lee*,
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Unraveling the Far-Field Coupling of Multilayered Chiral Metamaterials for CMOS-Enabled Midinfrared Imaging
Three-dimensional (3D) chiral metamaterials are structures with broken out-of-plane symmetry. With intrinsic chirality, they present larger circular dichroism (CD) signals than the 2D chiral metamaterials. Among all types of 3D metamaterials, multilayer-stacked metamaterials stand out, as they have the potential for large-scale fabrication. To date, tremendous work has focused on improving the CD signal by trying different patterns and materials. However, they lack a general theoretical framework to bridge the in-plane pattern design and out-of-plane layer design. Besides, most attempts have been made on longer wavelengths, such as THz and GHz ranges, as resonator dimensions are challenging in shorter wavelengths. In this work, leveraging both in-plane rotation and out-of-plane twist designs, we explore the far-field coupling mechanism using temporal coupled-mode theory and discuss the mechanism behind the multilayered chiral metamaterials. Moreover, enabled by a standard CMOS fabrication process, we demonstrate multilayered chiral metamaterials in the mid-infrared regime. Furthermore, by arranging the achiral and chiral cells accordingly at different wavelengths, a 5 × 5 array is demonstrated for mid-infrared imaging. Our work has the potential to be used for free-space communication, optical encryption, and sensing applications.
期刊介绍:
ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.