Yueguang Wang , Zifeng Huang , Di Zhang , Meining Li , Xinyan Wen , Xin Lei , Ziwei Ye , Jie Pang
{"title":"以魔芋葡甘露聚糖和κ-卡拉胶制备的高性能多功能生物凝胶传感器","authors":"Yueguang Wang , Zifeng Huang , Di Zhang , Meining Li , Xinyan Wen , Xin Lei , Ziwei Ye , Jie Pang","doi":"10.1016/j.carbpol.2025.124215","DOIUrl":null,"url":null,"abstract":"<div><div>In this study, a novel multifunctional biosensor was developed based on the synergistic cross-linking of Konjac glucomannan (KGM) and κ-Carrageenan (KC). This biosensor exhibits high sensitivity for detecting triple signals: temperature, humidity, and strain. This matrix demonstrates excellent mechanical toughness (elongation at break >300 %) and a low Young's modulus (173.017 ± 1.51 kPa). This material exhibits a high thermal sensitivity of 1.67 %°C<sup>−1</sup> in temperature detection, and a linear response range of −15 % to 45 % was achieved within the temperature range of 4–40 °C. For humidity sensing, it provides a three-stage linear response with sensitivities of −89.75 %/% RH (0–40 % RH), −182.21 %/% RH (40–75 % RH), and −53.45 %/% RH (75–95 % RH). In terms of the strain sensing performance, this material demonstrates excellent wide-range detection capability (1–350 % strain), with a response value of approximately 875 %, and it also has high sensitivity (GF = 2.54 ± 0.06). Compared with traditional biomass-based gel sensors, the response limit of this sensor has been significantly increased while maintaining higher sensitivity. Experiments confirmed that the sensor can be monitored via resistance signals and exhibits stable performance (>2000 cycles) in flexible wearable applications such as human breathing monitoring and joint motion tracking, offering an innovative solution for intelligent medical monitoring and environmentally friendly electronic skin development.</div></div>","PeriodicalId":261,"journal":{"name":"Carbohydrate Polymers","volume":"368 ","pages":"Article 124215"},"PeriodicalIF":12.5000,"publicationDate":"2025-08-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"High performance multifunctional bio-gel sensor prepared with konjac glucomannan and κ-carrageenan\",\"authors\":\"Yueguang Wang , Zifeng Huang , Di Zhang , Meining Li , Xinyan Wen , Xin Lei , Ziwei Ye , Jie Pang\",\"doi\":\"10.1016/j.carbpol.2025.124215\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>In this study, a novel multifunctional biosensor was developed based on the synergistic cross-linking of Konjac glucomannan (KGM) and κ-Carrageenan (KC). This biosensor exhibits high sensitivity for detecting triple signals: temperature, humidity, and strain. This matrix demonstrates excellent mechanical toughness (elongation at break >300 %) and a low Young's modulus (173.017 ± 1.51 kPa). This material exhibits a high thermal sensitivity of 1.67 %°C<sup>−1</sup> in temperature detection, and a linear response range of −15 % to 45 % was achieved within the temperature range of 4–40 °C. For humidity sensing, it provides a three-stage linear response with sensitivities of −89.75 %/% RH (0–40 % RH), −182.21 %/% RH (40–75 % RH), and −53.45 %/% RH (75–95 % RH). In terms of the strain sensing performance, this material demonstrates excellent wide-range detection capability (1–350 % strain), with a response value of approximately 875 %, and it also has high sensitivity (GF = 2.54 ± 0.06). Compared with traditional biomass-based gel sensors, the response limit of this sensor has been significantly increased while maintaining higher sensitivity. Experiments confirmed that the sensor can be monitored via resistance signals and exhibits stable performance (>2000 cycles) in flexible wearable applications such as human breathing monitoring and joint motion tracking, offering an innovative solution for intelligent medical monitoring and environmentally friendly electronic skin development.</div></div>\",\"PeriodicalId\":261,\"journal\":{\"name\":\"Carbohydrate Polymers\",\"volume\":\"368 \",\"pages\":\"Article 124215\"},\"PeriodicalIF\":12.5000,\"publicationDate\":\"2025-08-14\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Carbohydrate Polymers\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0144861725010008\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, APPLIED\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Carbohydrate Polymers","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0144861725010008","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, APPLIED","Score":null,"Total":0}
High performance multifunctional bio-gel sensor prepared with konjac glucomannan and κ-carrageenan
In this study, a novel multifunctional biosensor was developed based on the synergistic cross-linking of Konjac glucomannan (KGM) and κ-Carrageenan (KC). This biosensor exhibits high sensitivity for detecting triple signals: temperature, humidity, and strain. This matrix demonstrates excellent mechanical toughness (elongation at break >300 %) and a low Young's modulus (173.017 ± 1.51 kPa). This material exhibits a high thermal sensitivity of 1.67 %°C−1 in temperature detection, and a linear response range of −15 % to 45 % was achieved within the temperature range of 4–40 °C. For humidity sensing, it provides a three-stage linear response with sensitivities of −89.75 %/% RH (0–40 % RH), −182.21 %/% RH (40–75 % RH), and −53.45 %/% RH (75–95 % RH). In terms of the strain sensing performance, this material demonstrates excellent wide-range detection capability (1–350 % strain), with a response value of approximately 875 %, and it also has high sensitivity (GF = 2.54 ± 0.06). Compared with traditional biomass-based gel sensors, the response limit of this sensor has been significantly increased while maintaining higher sensitivity. Experiments confirmed that the sensor can be monitored via resistance signals and exhibits stable performance (>2000 cycles) in flexible wearable applications such as human breathing monitoring and joint motion tracking, offering an innovative solution for intelligent medical monitoring and environmentally friendly electronic skin development.
期刊介绍:
Carbohydrate Polymers stands as a prominent journal in the glycoscience field, dedicated to exploring and harnessing the potential of polysaccharides with applications spanning bioenergy, bioplastics, biomaterials, biorefining, chemistry, drug delivery, food, health, nanotechnology, packaging, paper, pharmaceuticals, medicine, oil recovery, textiles, tissue engineering, wood, and various aspects of glycoscience.
The journal emphasizes the central role of well-characterized carbohydrate polymers, highlighting their significance as the primary focus rather than a peripheral topic. Each paper must prominently feature at least one named carbohydrate polymer, evident in both citation and title, with a commitment to innovative research that advances scientific knowledge.