Rui Dong , Wangquan Ye , Luyu Yang , Zhenghao Guo , Ye Tian , Yuan Lu , Ronger Zheng
{"title":"基于双轴激光扫描振镜系统的无平移LIBS成像","authors":"Rui Dong , Wangquan Ye , Luyu Yang , Zhenghao Guo , Ye Tian , Yuan Lu , Ronger Zheng","doi":"10.1016/j.sab.2025.107290","DOIUrl":null,"url":null,"abstract":"<div><div>Conventional laser-induced breakdown spectroscopy (LIBS) imaging systems typically rely on motorized translation stages to move samples. However, stage-dependent architectures have limitations in non-destructive, large-area imaging, especially when analyzing immobilized specimens under <em>in situ</em> conditions. In this work, we replaced the traditional sample translation method with a beam deflection approach, utilizing a dual-axis laser scanning galvanometer system to adjust the deflection direction of the light beam. A telecentric F-theta field lens was introduced to correct field curvature and geometric distortions, enabling efficient scanning of stationary samples without mechanical translation. We applied the system to measure a pure copper target and a copper–silver composite target, with a scanning area of 32 mm<span><math><mrow><mspace></mspace><mo>×</mo><mspace></mspace></mrow></math></span>32 mm, to evaluate its imaging performance. The plasma images reveal a noticeable center-symmetric pattern influenced by scanning angles. Moreover, spectral peak intensities at different wavelengths show markedly distinct distributions, demonstrating the wavelength-dependent interaction mechanisms. This phenomenon was explained using interference theory, thereby enabling correction of the spatial distribution of spectral intensity. This methodology provides a practical design framework for stationary-sample scanning systems, demonstrating measurable application potential in <em>in situ</em> analytics.</div></div>","PeriodicalId":21890,"journal":{"name":"Spectrochimica Acta Part B: Atomic Spectroscopy","volume":"233 ","pages":"Article 107290"},"PeriodicalIF":3.8000,"publicationDate":"2025-08-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Translation-free LIBS imaging based on a dual-axis laser scanning galvanometer system\",\"authors\":\"Rui Dong , Wangquan Ye , Luyu Yang , Zhenghao Guo , Ye Tian , Yuan Lu , Ronger Zheng\",\"doi\":\"10.1016/j.sab.2025.107290\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Conventional laser-induced breakdown spectroscopy (LIBS) imaging systems typically rely on motorized translation stages to move samples. However, stage-dependent architectures have limitations in non-destructive, large-area imaging, especially when analyzing immobilized specimens under <em>in situ</em> conditions. In this work, we replaced the traditional sample translation method with a beam deflection approach, utilizing a dual-axis laser scanning galvanometer system to adjust the deflection direction of the light beam. A telecentric F-theta field lens was introduced to correct field curvature and geometric distortions, enabling efficient scanning of stationary samples without mechanical translation. We applied the system to measure a pure copper target and a copper–silver composite target, with a scanning area of 32 mm<span><math><mrow><mspace></mspace><mo>×</mo><mspace></mspace></mrow></math></span>32 mm, to evaluate its imaging performance. The plasma images reveal a noticeable center-symmetric pattern influenced by scanning angles. Moreover, spectral peak intensities at different wavelengths show markedly distinct distributions, demonstrating the wavelength-dependent interaction mechanisms. This phenomenon was explained using interference theory, thereby enabling correction of the spatial distribution of spectral intensity. This methodology provides a practical design framework for stationary-sample scanning systems, demonstrating measurable application potential in <em>in situ</em> analytics.</div></div>\",\"PeriodicalId\":21890,\"journal\":{\"name\":\"Spectrochimica Acta Part B: Atomic Spectroscopy\",\"volume\":\"233 \",\"pages\":\"Article 107290\"},\"PeriodicalIF\":3.8000,\"publicationDate\":\"2025-08-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Spectrochimica Acta Part B: Atomic Spectroscopy\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0584854725001752\",\"RegionNum\":2,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"SPECTROSCOPY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Spectrochimica Acta Part B: Atomic Spectroscopy","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0584854725001752","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"SPECTROSCOPY","Score":null,"Total":0}
Translation-free LIBS imaging based on a dual-axis laser scanning galvanometer system
Conventional laser-induced breakdown spectroscopy (LIBS) imaging systems typically rely on motorized translation stages to move samples. However, stage-dependent architectures have limitations in non-destructive, large-area imaging, especially when analyzing immobilized specimens under in situ conditions. In this work, we replaced the traditional sample translation method with a beam deflection approach, utilizing a dual-axis laser scanning galvanometer system to adjust the deflection direction of the light beam. A telecentric F-theta field lens was introduced to correct field curvature and geometric distortions, enabling efficient scanning of stationary samples without mechanical translation. We applied the system to measure a pure copper target and a copper–silver composite target, with a scanning area of 32 mm32 mm, to evaluate its imaging performance. The plasma images reveal a noticeable center-symmetric pattern influenced by scanning angles. Moreover, spectral peak intensities at different wavelengths show markedly distinct distributions, demonstrating the wavelength-dependent interaction mechanisms. This phenomenon was explained using interference theory, thereby enabling correction of the spatial distribution of spectral intensity. This methodology provides a practical design framework for stationary-sample scanning systems, demonstrating measurable application potential in in situ analytics.
期刊介绍:
Spectrochimica Acta Part B: Atomic Spectroscopy, is intended for the rapid publication of both original work and reviews in the following fields:
Atomic Emission (AES), Atomic Absorption (AAS) and Atomic Fluorescence (AFS) spectroscopy;
Mass Spectrometry (MS) for inorganic analysis covering Spark Source (SS-MS), Inductively Coupled Plasma (ICP-MS), Glow Discharge (GD-MS), and Secondary Ion Mass Spectrometry (SIMS).
Laser induced atomic spectroscopy for inorganic analysis, including non-linear optical laser spectroscopy, covering Laser Enhanced Ionization (LEI), Laser Induced Fluorescence (LIF), Resonance Ionization Spectroscopy (RIS) and Resonance Ionization Mass Spectrometry (RIMS); Laser Induced Breakdown Spectroscopy (LIBS); Cavity Ringdown Spectroscopy (CRDS), Laser Ablation Inductively Coupled Plasma Atomic Emission Spectroscopy (LA-ICP-AES) and Laser Ablation Inductively Coupled Plasma Mass Spectrometry (LA-ICP-MS).
X-ray spectrometry, X-ray Optics and Microanalysis, including X-ray fluorescence spectrometry (XRF) and related techniques, in particular Total-reflection X-ray Fluorescence Spectrometry (TXRF), and Synchrotron Radiation-excited Total reflection XRF (SR-TXRF).
Manuscripts dealing with (i) fundamentals, (ii) methodology development, (iii)instrumentation, and (iv) applications, can be submitted for publication.