纳米流体润湿反转效应增强微通道内流动的机理研究

IF 4.3 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
ACS Omega Pub Date : 2025-08-01 DOI:10.1021/acsomega.5c02720
Xiaoxiao Dou, Guangwen Zhang, Xuqing Lang, Ripeng Zhang and Chun Wang*, 
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引用次数: 0

摘要

纳米流体可以诱导固液界面的润湿逆转,这有望增强通道内的流动。在本文中,我们评估了纳米流体在固体表面诱导润湿转变的性能,并研究了改善流动的机制。首先,对接触角的实验测试表明,表面活性剂-纳米颗粒复合溶液处理的固体表面具有较高的亲水性。分别研究了纳米颗粒和表面活性剂对降低接触角的影响。阐述了分离压力引起固液界面油膜分离的基本机理。为了验证润湿逆转对流动的促进作用,我们利用自行设计的三维微通道模型进行了流动测试实验。通过实验和数值模拟相结合的方法,阐明了纳米流体在微通道中的润湿反转效应对流动效率、流动轨迹和流动介质体积分布的影响机理。清洗效率分析表明,表面活性纳米颗粒复合溶液广泛分布在模型中大多数微通道中。阐述了该溶液诱导润湿反转以提高流动效率的机理。本研究通过实验与数值模拟相结合的方法系统地阐明了纳米流体中润湿逆转的机理,为理解表面活性纳米颗粒复合溶液在多相界面上的流动行为提供了重要的基础。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Study on the Mechanism of the Nanofluid Wetting Inversion Effect Enhancing the Flow in Microchannels

Nanofluids can induce a reversal of wetting at the solid–liquid interface, which is expected to enhance flow within channels. In this paper, we evaluate the performance of nanofluids in inducing wetting transitions on solid surfaces and investigate the mechanisms that improve flow. First, the experimental tests on contact angles demonstrate that solid surfaces treated with surfactant–nanoparticle composite solutions exhibit high hydrophilicity. The effects of nanoparticles and surfactants on reducing the contact angle are separately investigated. The basic mechanism of solid–liquid interface oil film separation caused by the separation pressure is elaborated. To verify the promoting effect of wetting reversal on flow, we conducted flow testing experiments using a self-designed 3D microchannel model. The mechanism by which the wetting reversal effect of nanofluids in microchannels affects flow efficiency, flow trajectory, and distribution of the flow medium volume is elucidated through a combination of experimental and numerical simulation methods. The analysis of cleaning efficiency reveals that the surface-active nanoparticle composite solution is widely distributed throughout most microchannels in the model. The mechanism by which this solution induces wetting inversion to improve the flow efficiency is elaborated. This study systematically clarifies the mechanism of wetting reversal in nanofluids by combining experiments with numerical simulations, providing an important foundation for understanding the flow behavior of surface-active nanoparticle composite solutions at multiphase interfaces.

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来源期刊
ACS Omega
ACS Omega Chemical Engineering-General Chemical Engineering
CiteScore
6.60
自引率
4.90%
发文量
3945
审稿时长
2.4 months
期刊介绍: ACS Omega is an open-access global publication for scientific articles that describe new findings in chemistry and interfacing areas of science, without any perceived evaluation of immediate impact.
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