基于SnTe的超宽带非线性霍尔整流器

IF 34.9 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Fanrui Hu, Pengnan Zhao, Lihuan Yang, Shishun Zhao, Jiayu Lei, Weijian Li, Jiamin Lai, Zhonghai Yu, Hanbum Park, Chengquan Wong, Raghav Sharma, Goki Eda, Shengyuan A. Yang, Xiaohong Xu, Fei Wang, Hyunsoo Yang
{"title":"基于SnTe的超宽带非线性霍尔整流器","authors":"Fanrui Hu, Pengnan Zhao, Lihuan Yang, Shishun Zhao, Jiayu Lei, Weijian Li, Jiamin Lai, Zhonghai Yu, Hanbum Park, Chengquan Wong, Raghav Sharma, Goki Eda, Shengyuan A. Yang, Xiaohong Xu, Fei Wang, Hyunsoo Yang","doi":"10.1038/s41565-025-01993-2","DOIUrl":null,"url":null,"abstract":"<p>The rapid expansion of self-powered electronics in the Internet of Things, 6G communication and millimetre-wave systems calls for rectifiers capable of operating across ultrabroadband frequencies and at extremely low input power levels. However, conventional rectifiers based on semiconductor junctions face fundamental limitations such as parasitic capacitance and threshold voltages, preventing effective operation under broadband and ambient radio-frequency conditions. Here we present an ultrabroadband, zero-bias rectifier based on the nonlinear Hall effect in wafer-scale (001)-oriented topological crystalline insulator SnTe thin film. This material exhibits a large second-order conductivity of ~0.004 Ω⁻<sup>1</sup> V⁻<sup>1</sup>, surpassing that of other wafer-scale materials. The nonlinear Hall effect arises primarily from a Berry curvature dipole, evidenced by angular-resolved transport measurements and first-principles calculations. The device demonstrates rectification from 23 MHz to 1 THz, with sensitivity down to –60 dBm in key radio-frequency bands, without any external bias. Rectified output power is scalable through series- and parallel-array topologies and can be enhanced using rectenna designs. As a proof of concept, we achieve the wireless powering of a thermistor using harvested radio-frequency energy, validating the potential of this material platform and nonlinear Hall effect for next-generation energy-autonomous microsystems.</p>","PeriodicalId":18915,"journal":{"name":"Nature nanotechnology","volume":"8 1","pages":""},"PeriodicalIF":34.9000,"publicationDate":"2025-08-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Ultrabroadband nonlinear Hall rectifier using SnTe\",\"authors\":\"Fanrui Hu, Pengnan Zhao, Lihuan Yang, Shishun Zhao, Jiayu Lei, Weijian Li, Jiamin Lai, Zhonghai Yu, Hanbum Park, Chengquan Wong, Raghav Sharma, Goki Eda, Shengyuan A. Yang, Xiaohong Xu, Fei Wang, Hyunsoo Yang\",\"doi\":\"10.1038/s41565-025-01993-2\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>The rapid expansion of self-powered electronics in the Internet of Things, 6G communication and millimetre-wave systems calls for rectifiers capable of operating across ultrabroadband frequencies and at extremely low input power levels. However, conventional rectifiers based on semiconductor junctions face fundamental limitations such as parasitic capacitance and threshold voltages, preventing effective operation under broadband and ambient radio-frequency conditions. Here we present an ultrabroadband, zero-bias rectifier based on the nonlinear Hall effect in wafer-scale (001)-oriented topological crystalline insulator SnTe thin film. This material exhibits a large second-order conductivity of ~0.004 Ω⁻<sup>1</sup> V⁻<sup>1</sup>, surpassing that of other wafer-scale materials. The nonlinear Hall effect arises primarily from a Berry curvature dipole, evidenced by angular-resolved transport measurements and first-principles calculations. The device demonstrates rectification from 23 MHz to 1 THz, with sensitivity down to –60 dBm in key radio-frequency bands, without any external bias. Rectified output power is scalable through series- and parallel-array topologies and can be enhanced using rectenna designs. As a proof of concept, we achieve the wireless powering of a thermistor using harvested radio-frequency energy, validating the potential of this material platform and nonlinear Hall effect for next-generation energy-autonomous microsystems.</p>\",\"PeriodicalId\":18915,\"journal\":{\"name\":\"Nature nanotechnology\",\"volume\":\"8 1\",\"pages\":\"\"},\"PeriodicalIF\":34.9000,\"publicationDate\":\"2025-08-11\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nature nanotechnology\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1038/s41565-025-01993-2\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nature nanotechnology","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1038/s41565-025-01993-2","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

在物联网、6G通信和毫米波系统中,自供电电子设备的迅速发展需要能够在超宽带频率和极低输入功率水平下工作的整流器。然而,基于半导体结的传统整流器面临寄生电容和阈值电压等基本限制,无法在宽带和环境射频条件下有效运行。在这里,我们提出了一种基于非线性霍尔效应的超宽带零偏置整流器,这种整流器是基于晶圆尺度(001)取向拓扑晶体绝缘体SnTe薄膜的。这种材料的二阶电导率高达~0.004 Ω毒血症(⁻1 V毒血症),超过了其他晶圆级材料。非线性霍尔效应主要是由贝里曲率偶极子引起的,角分辨输运测量和第一性原理计算证明了这一点。该器件演示了从23 MHz到1 THz的整流,在关键射频频段的灵敏度低至-60 dBm,没有任何外部偏置。整流输出功率可通过串联和并联阵列拓扑进行扩展,并可使用整流天线设计进行增强。作为概念验证,我们利用收集的射频能量实现了热敏电阻的无线供电,验证了这种材料平台和下一代能量自主微系统的非线性霍尔效应的潜力。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Ultrabroadband nonlinear Hall rectifier using SnTe

Ultrabroadband nonlinear Hall rectifier using SnTe

The rapid expansion of self-powered electronics in the Internet of Things, 6G communication and millimetre-wave systems calls for rectifiers capable of operating across ultrabroadband frequencies and at extremely low input power levels. However, conventional rectifiers based on semiconductor junctions face fundamental limitations such as parasitic capacitance and threshold voltages, preventing effective operation under broadband and ambient radio-frequency conditions. Here we present an ultrabroadband, zero-bias rectifier based on the nonlinear Hall effect in wafer-scale (001)-oriented topological crystalline insulator SnTe thin film. This material exhibits a large second-order conductivity of ~0.004 Ω⁻1 V⁻1, surpassing that of other wafer-scale materials. The nonlinear Hall effect arises primarily from a Berry curvature dipole, evidenced by angular-resolved transport measurements and first-principles calculations. The device demonstrates rectification from 23 MHz to 1 THz, with sensitivity down to –60 dBm in key radio-frequency bands, without any external bias. Rectified output power is scalable through series- and parallel-array topologies and can be enhanced using rectenna designs. As a proof of concept, we achieve the wireless powering of a thermistor using harvested radio-frequency energy, validating the potential of this material platform and nonlinear Hall effect for next-generation energy-autonomous microsystems.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Nature nanotechnology
Nature nanotechnology 工程技术-材料科学:综合
CiteScore
59.70
自引率
0.80%
发文量
196
审稿时长
4-8 weeks
期刊介绍: Nature Nanotechnology is a prestigious journal that publishes high-quality papers in various areas of nanoscience and nanotechnology. The journal focuses on the design, characterization, and production of structures, devices, and systems that manipulate and control materials at atomic, molecular, and macromolecular scales. It encompasses both bottom-up and top-down approaches, as well as their combinations. Furthermore, Nature Nanotechnology fosters the exchange of ideas among researchers from diverse disciplines such as chemistry, physics, material science, biomedical research, engineering, and more. It promotes collaboration at the forefront of this multidisciplinary field. The journal covers a wide range of topics, from fundamental research in physics, chemistry, and biology, including computational work and simulations, to the development of innovative devices and technologies for various industrial sectors such as information technology, medicine, manufacturing, high-performance materials, energy, and environmental technologies. It includes coverage of organic, inorganic, and hybrid materials.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信