Chen Zhang , Yan Gao , Ruyue Cui , Hanxi Zhang , Jinhua Tian , Yujie Tang , Lei Yang , Chaofan Feng , Pietro Patimisco , Angelo Sampaolo , Vincenzo Spagnolo , Xukun Yin , Lei Dong , Hongpeng Wu
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Enhancing photoacoustic trace gas detection via a CNN–transformer denoising framework
We present a novel approach for gas concentration measurement using a differential resonant photoacoustic cell combined with a deep learning-based signal denoising model. This method addresses the persistent challenge of noise interference in 2 f signals at low gas concentrations, where conventional processing methods struggle to maintain signal fidelity. To resolve this, we propose a deep learning model that integrates 1D Convolutional Neural Networks (1D CNNs) for local feature extraction and Transformer networks for capturing global dependencies. The model was trained using synthetic signals with added noise to simulate real-world conditions, ensuring robustness and adaptability. Applied to experimental 2 f signals, the model demonstrated excellent noise suppression capabilities, enhancing the signal-to-noise ratio (SNR) of 500 ppb acetylene signals by a factor of approximately 70. Furthermore, the determination coefficient (R²) improved, reflecting better accuracy and linearity in signal reconstruction. These results underscore the model's potential for improving detection sensitivity and reliability in trace gas measurements, marking a significant advancement in spectroscopic signal processing for gas detection.
PhotoacousticsPhysics and Astronomy-Atomic and Molecular Physics, and Optics
CiteScore
11.40
自引率
16.50%
发文量
96
审稿时长
53 days
期刊介绍:
The open access Photoacoustics journal (PACS) aims to publish original research and review contributions in the field of photoacoustics-optoacoustics-thermoacoustics. This field utilizes acoustical and ultrasonic phenomena excited by electromagnetic radiation for the detection, visualization, and characterization of various materials and biological tissues, including living organisms.
Recent advancements in laser technologies, ultrasound detection approaches, inverse theory, and fast reconstruction algorithms have greatly supported the rapid progress in this field. The unique contrast provided by molecular absorption in photoacoustic-optoacoustic-thermoacoustic methods has allowed for addressing unmet biological and medical needs such as pre-clinical research, clinical imaging of vasculature, tissue and disease physiology, drug efficacy, surgery guidance, and therapy monitoring.
Applications of this field encompass a wide range of medical imaging and sensing applications, including cancer, vascular diseases, brain neurophysiology, ophthalmology, and diabetes. Moreover, photoacoustics-optoacoustics-thermoacoustics is a multidisciplinary field, with contributions from chemistry and nanotechnology, where novel materials such as biodegradable nanoparticles, organic dyes, targeted agents, theranostic probes, and genetically expressed markers are being actively developed.
These advanced materials have significantly improved the signal-to-noise ratio and tissue contrast in photoacoustic methods.