聚酰胺6水解、醇解、氨解和酸解的分子研究。

IF 2.8 2区 化学 Q3 CHEMISTRY, PHYSICAL
Zhengyi Wan, Yilun Huang*, Liangyu Xiang, Jiawei Zhao, Zhihui Song, Huasheng Feng, Shijun Zhang and Changjiang Wu*, 
{"title":"聚酰胺6水解、醇解、氨解和酸解的分子研究。","authors":"Zhengyi Wan,&nbsp;Yilun Huang*,&nbsp;Liangyu Xiang,&nbsp;Jiawei Zhao,&nbsp;Zhihui Song,&nbsp;Huasheng Feng,&nbsp;Shijun Zhang and Changjiang Wu*,&nbsp;","doi":"10.1021/acs.jpca.5c02954","DOIUrl":null,"url":null,"abstract":"<p >Recycling emerges as a pivotal strategy to mitigate plastic waste, particularly for polyamides. This study delves into the chemical recycling of polyamide 6 (PA6) using quantum chemistry calculations. We investigate the molecular mechanisms of hydrolysis, alcoholysis, and ammonolysis as well as acidolysis with acetic acid. Our findings elucidate a two-step process in PA6 recycling: depolymerization and cyclization. PA6 is degraded to 6-aminocaproic acid and its derivatives in the depolymerization step, and these intermediates are then turned into ε-caprolactam in the cyclization step. Each step has several reaction pathways with different energy profiles. In pure solvents, depolymerization is identified as the rate-limiting step. The introduction of acetic acid changes the rate-limiting step and effectively lowers the energy barrier, enhancing the recycling process. Computational results align with prior experimental data and offer a plausible molecular explanation of polyamide recycling. These insights are vital for devising more efficient and sustainable chemical recycling methods for polyamides.</p>","PeriodicalId":59,"journal":{"name":"The Journal of Physical Chemistry A","volume":"129 32","pages":"7345–7351"},"PeriodicalIF":2.8000,"publicationDate":"2025-08-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Molecular Insights into Hydrolysis, Alcoholysis, Ammonolysis, and Acidolysis of Polyamide 6\",\"authors\":\"Zhengyi Wan,&nbsp;Yilun Huang*,&nbsp;Liangyu Xiang,&nbsp;Jiawei Zhao,&nbsp;Zhihui Song,&nbsp;Huasheng Feng,&nbsp;Shijun Zhang and Changjiang Wu*,&nbsp;\",\"doi\":\"10.1021/acs.jpca.5c02954\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Recycling emerges as a pivotal strategy to mitigate plastic waste, particularly for polyamides. This study delves into the chemical recycling of polyamide 6 (PA6) using quantum chemistry calculations. We investigate the molecular mechanisms of hydrolysis, alcoholysis, and ammonolysis as well as acidolysis with acetic acid. Our findings elucidate a two-step process in PA6 recycling: depolymerization and cyclization. PA6 is degraded to 6-aminocaproic acid and its derivatives in the depolymerization step, and these intermediates are then turned into ε-caprolactam in the cyclization step. Each step has several reaction pathways with different energy profiles. In pure solvents, depolymerization is identified as the rate-limiting step. The introduction of acetic acid changes the rate-limiting step and effectively lowers the energy barrier, enhancing the recycling process. Computational results align with prior experimental data and offer a plausible molecular explanation of polyamide recycling. These insights are vital for devising more efficient and sustainable chemical recycling methods for polyamides.</p>\",\"PeriodicalId\":59,\"journal\":{\"name\":\"The Journal of Physical Chemistry A\",\"volume\":\"129 32\",\"pages\":\"7345–7351\"},\"PeriodicalIF\":2.8000,\"publicationDate\":\"2025-08-05\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"The Journal of Physical Chemistry A\",\"FirstCategoryId\":\"1\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acs.jpca.5c02954\",\"RegionNum\":2,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"The Journal of Physical Chemistry A","FirstCategoryId":"1","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.jpca.5c02954","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0

摘要

回收利用成为减少塑料废物,特别是聚酰胺的关键战略。本研究利用量子化学计算深入研究了聚酰胺6 (PA6)的化学回收。我们研究了水解、醇解、氨解以及醋酸酸解的分子机制。我们的研究结果阐明了PA6回收的两步过程:解聚和环化。PA6在解聚过程中降解为6-氨基己酸及其衍生物,这些中间体在环化过程中转化为ε-己内酰胺。每一步都有几个具有不同能量分布的反应途径。在纯溶剂中,解聚被确定为限速步骤。醋酸的引入改变了限速步骤,有效地降低了能垒,提高了回收效率。计算结果与先前的实验数据一致,并提供了聚酰胺回收的合理分子解释。这些见解对于设计更有效和可持续的聚酰胺化学回收方法至关重要。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Molecular Insights into Hydrolysis, Alcoholysis, Ammonolysis, and Acidolysis of Polyamide 6

Molecular Insights into Hydrolysis, Alcoholysis, Ammonolysis, and Acidolysis of Polyamide 6

Recycling emerges as a pivotal strategy to mitigate plastic waste, particularly for polyamides. This study delves into the chemical recycling of polyamide 6 (PA6) using quantum chemistry calculations. We investigate the molecular mechanisms of hydrolysis, alcoholysis, and ammonolysis as well as acidolysis with acetic acid. Our findings elucidate a two-step process in PA6 recycling: depolymerization and cyclization. PA6 is degraded to 6-aminocaproic acid and its derivatives in the depolymerization step, and these intermediates are then turned into ε-caprolactam in the cyclization step. Each step has several reaction pathways with different energy profiles. In pure solvents, depolymerization is identified as the rate-limiting step. The introduction of acetic acid changes the rate-limiting step and effectively lowers the energy barrier, enhancing the recycling process. Computational results align with prior experimental data and offer a plausible molecular explanation of polyamide recycling. These insights are vital for devising more efficient and sustainable chemical recycling methods for polyamides.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
The Journal of Physical Chemistry A
The Journal of Physical Chemistry A 化学-物理:原子、分子和化学物理
CiteScore
5.20
自引率
10.30%
发文量
922
审稿时长
1.3 months
期刊介绍: The Journal of Physical Chemistry A is devoted to reporting new and original experimental and theoretical basic research of interest to physical chemists, biophysical chemists, and chemical physicists.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信