通过超分子脱羧的手性诱导和记忆。

IF 16.9 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Jun.-Prof. Dr. Robert Hein, Dr. Eric Sidler, Dr. Yohan Gisbert, Prof. Dr. Ben L. Feringa
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引用次数: 0

摘要

手性是自然界固有的,分子手性的控制一直处于化学科学的前沿。引入基本的新原理来打破对称,从而形成特定的对映体,这在许多科学领域都具有重要的意义,尤其具有挑战性。本文提出了一种螺旋手性动态分子开关,其对映体通过单一对称亚稳态连接,该亚稳态可以通过光或氧化还原刺激填充。在结合的手性客体铵的存在下,前手性态的松弛导致通过概念上独特的超分子脱羧过程优先形成特定的对映体。重要的是,即使在没有客体的情况下,形成的宿主对映体也是稳定的,从而实现可逆和稳定的手性信息传递,而宿主的氧化导致对光不敏感的对映体富集,从而允许正交手性记忆。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Chiral Induction and Memory via Supramolecular Deracemization

Chiral Induction and Memory via Supramolecular Deracemization

Chirality is intrinsic to nature, and control of molecular chirality remains at the forefront of the chemical sciences. The introduction of fundamentally new principles to break symmetry, leading to the formation of a specific enantiomer, is particularly challenging with important implications in numerous scientific fields. Herein we present a helically chiral dynamic molecular switch whose enantiomers are connected via a single symmetric metastable state that can be populated via light or redox stimuli. Relaxation of the prochiral state in the presence of a bound chiral ammonium guest results in the preferential formation of a specific enantiomer through a conceptually unique supramolecular deracemization process. Importantly, the formed host enantiomer is stable even in the absence of guest, enabling reversible and stable chiral information transfer, while oxidation of the host results in an enantioenriched dication that is insensitive to light, allowing orthogonal chiral memory.

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来源期刊
CiteScore
26.60
自引率
6.60%
发文量
3549
审稿时长
1.5 months
期刊介绍: Angewandte Chemie, a journal of the German Chemical Society (GDCh), maintains a leading position among scholarly journals in general chemistry with an impressive Impact Factor of 16.6 (2022 Journal Citation Reports, Clarivate, 2023). Published weekly in a reader-friendly format, it features new articles almost every day. Established in 1887, Angewandte Chemie is a prominent chemistry journal, offering a dynamic blend of Review-type articles, Highlights, Communications, and Research Articles on a weekly basis, making it unique in the field.
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