邻苯二甲酸酯在中国新装修住宅地板材料中的存在、迁移行为及环境负担

IF 3.9 3区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES
Toxics Pub Date : 2025-06-20 DOI:10.3390/toxics13070517
Ying Zhang, Li-Bo Chen, Hao-Yang Shen, Zi-Chao Wu, Ning-Zheng Zhu, Chong-Jing Gao, Ying Guo
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引用次数: 0

摘要

邻苯二甲酸酯(PAEs)是一类合成的半挥发性有机化合物,广泛应用于装饰材料中。然而,它们的具体发生、迁移行为以及对这些材料的环境影响——这些材料构成了住宅环境中最大的表面积——仍然没有得到充分的了解。本研究调查了中国家庭常用地板中PAEs的分布、排放动态和环境负担。结果表明,PAEs在地板中分布广泛,总浓度为1220 ~ 166,000 ng/g(中位数为14,100 ng/g)。实木地板(55,900 ng/g)的PAE含量明显高于工程地板(22,600 ng/g)和强化地板(4000 ng/g) (p < 0.05)。迁移实验表明,实木地板具有连续释放PAE的趋势,强化木地板具有明显的PAE吸收能力,而工程地板具有释放和吸收的双重特性。初始PAE浓度是影响迁移速率的主要因素,地板类型和基材密度也有不同程度的影响。新装修的中国家庭地板中PAEs造成的环境负担范围为3.63 × 109 ng至3.45 × 1011 ng,中位数为1.23 × 1010 ng。东部和西南地区家庭PAE负担最高,南部地区最低。住宅面积、房间数量、家庭收入和装修预算等社会经济因素对地板产生的PAEs的环境负担有显著影响。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Occurrence, Migration Behavior, and Environmental Burden of Phthalate Esters in Flooring Materials Used in Newly Renovated Chinese Homes.

Phthalic acid esters (PAEs), a class of synthetic semi-volatile organic compounds, are extensively incorporated into decorative materials. However, their specific occurrence, migration behaviors, and environmental impact on these materials-which comprise the largest surface areas in residential settings-remain insufficiently understood. This study investigated the distribution, emission dynamics, and environmental burdens of PAEs in flooring commonly used in Chinese households. The results showed that PAEs are widespread in flooring, with total concentrations ranging from 1220 to 166,000 ng/g (14,100 ng/g, median value). Solid wood flooring (55,900 ng/g) exhibited significantly higher PAE levels compared to engineered flooring (22,600 ng/g) and laminate flooring (4000 ng/g) (p < 0.05). Migration experiments revealed that solid wood flooring tended to continuously release PAEs, laminate flooring showed a pronounced capacity for PAE absorption, and engineered flooring exhibited both release and absorption behaviors. The initial PAE concentration is the dominant factor influencing migration rates, while the flooring type and substrate density also contribute to varying degrees. The estimated environmental burdens of PAEs resulting from flooring in newly renovated Chinese households ranged from 3.63 × 109 ng to 3.45 × 1011 ng, with a median value of 1.23 × 1010 ng. Households in the eastern and southwestern regions exhibited the highest PAE burdens, while the southern region showed the lowest. Socioeconomic factors such as residential floor area, number of rooms, household income, and renovation budget significantly influenced the environmental burden of PAEs derived from flooring.

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来源期刊
Toxics
Toxics Chemical Engineering-Chemical Health and Safety
CiteScore
4.50
自引率
10.90%
发文量
681
审稿时长
6 weeks
期刊介绍: Toxics (ISSN 2305-6304) is an international, peer-reviewed, open access journal which provides an advanced forum for studies related to all aspects of toxic chemicals and materials. It publishes reviews, regular research papers, and short communications. Our aim is to encourage scientists to publish their experimental and theoretical results in detail. There is, therefore, no restriction on the maximum length of the papers, although authors should write their papers in a clear and concise way. The full experimental details must be provided so that the results can be reproduced. Electronic files or software regarding the full details of calculations and experimental procedure can be deposited as supplementary material, if it is not possible to publish them along with the text.
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