水溶液中重力偏置离子迁移。

IF 3.8 2区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
Jooyoung Im, J Carlos Santamarina
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引用次数: 0

摘要

假设水合离子的重力偏漂可以忽略不计,因此在分析和设计中不考虑。在这项研究中,我们重新评估了重力对水合离子在水溶液中迁移的影响,通过在不同的飞行持续时间内对六种氯盐溶液进行控制离心加速度。由此得到的数据表明,离子迁移取决于g水平和持续时间,这为引力偏差提供了明确的证据。根据测量到的移动量,在延伸数米或在长达一个世纪的时间尺度上运行的系统中,不应忽视重力引起的影响。认识到重力驱动的迁移有可能改变设计范式,从工业过程到核废料的地质储存。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Gravitation-biased ion migration in aqueous solutions.

The gravity-biased drift of hydrated ions is assumed negligible and therefore disregarded in analysis and design. In this study, we reassess the impact of gravity on hydrated ion migration in aqueous solutions by subjecting six chloride salt solutions to controlled centrifugal acceleration across varying flight durations. The resulting data show that ion migration depends on both g-level and duration, providing clear evidence of gravitational bias. Based on the measured mobilities, gravity-induced effects should not be overlooked in systems extending over several meters or operating on century-long timescales. Recognizing gravity-driven migration has the potential to shift design paradigms, from industrial processes to the geological storage of nuclear waste.

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来源期刊
Scientific Reports
Scientific Reports Natural Science Disciplines-
CiteScore
7.50
自引率
4.30%
发文量
19567
审稿时长
3.9 months
期刊介绍: We publish original research from all areas of the natural sciences, psychology, medicine and engineering. You can learn more about what we publish by browsing our specific scientific subject areas below or explore Scientific Reports by browsing all articles and collections. Scientific Reports has a 2-year impact factor: 4.380 (2021), and is the 6th most-cited journal in the world, with more than 540,000 citations in 2020 (Clarivate Analytics, 2021). •Engineering Engineering covers all aspects of engineering, technology, and applied science. It plays a crucial role in the development of technologies to address some of the world''s biggest challenges, helping to save lives and improve the way we live. •Physical sciences Physical sciences are those academic disciplines that aim to uncover the underlying laws of nature — often written in the language of mathematics. It is a collective term for areas of study including astronomy, chemistry, materials science and physics. •Earth and environmental sciences Earth and environmental sciences cover all aspects of Earth and planetary science and broadly encompass solid Earth processes, surface and atmospheric dynamics, Earth system history, climate and climate change, marine and freshwater systems, and ecology. It also considers the interactions between humans and these systems. •Biological sciences Biological sciences encompass all the divisions of natural sciences examining various aspects of vital processes. The concept includes anatomy, physiology, cell biology, biochemistry and biophysics, and covers all organisms from microorganisms, animals to plants. •Health sciences The health sciences study health, disease and healthcare. This field of study aims to develop knowledge, interventions and technology for use in healthcare to improve the treatment of patients.
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